Method for generating quantum-entangled photon pairs转让专利
申请号 : US11587003
文献号 : US07683361B2
文献日 : 2010-03-23
发明人 : Keiichi Edamatsu , Tadashi Itoh
申请人 : Keiichi Edamatsu , Tadashi Itoh
摘要 :
权利要求 :
The invention claimed is:
说明书 :
This application is the US national phase of international application PCT/JP2004/016249 filed 2 Nov. 2004, which designated the U.S. and claimed priority of JP 2004-124716 filed 20 Apr. 2004, the entire contents of each of which are hereby incorporated by reference.
The present invention relates to a method for generating photon pairs in a quantum entangled state.
Cryptographic techniques in information transmission have been studied in response to recent dramatic advance in information/communication technologies such as electronic commerce transactions, electric mails, etc. Quantum cryptography is one of cryptographic techniques, which draw much attention recently.
The quantum cryptography provides security by means of physical phenomenon by the uncertainty principle of Heisenberg in the quantum theory. According to the uncertainty principle, the state of quantum will be changed once it is observed, wiretapping (observation) of communication will be inevitably detectable. This allows to take measures against the wiretapping, such as shutting down the communication upon the detection of wiretapping. Thus, quantum cryptography makes wiretapping impossible physically. Moreover, the uncertainty principle explains that it is impossible to replicate particles.
Quantum teleportation is one of the key features of quantum cryptography. Quantum teleportation is a technique to transfer quantum information of the particles from one place where the particles exist to another place. The quantum teleportation is realized by information communication between photons by utilizing entanglement of quantum (quantum entanglement). Photon pairs in the quantum entangled state have such a property that once a quantum state of one of the photons is determined, then that of the other can be spontaneously determined. This property is not dependent on a distance between the photons.
Incidentally, optical lithography is utilized as a fine fabricating technique for semiconductors today. Lithography is a technique for forming an image based on an image transferred by exposure to light. In the conventional lithography, a limit of spatial resolution due to light diffraction makes it difficult to make fabrication finer than the order of light wavelength. On the other hand, quantum lithography, that is, a technique to attain a finer fabrication than the classical diffraction limit in the conventional technique by utilizing a phenomenon that de Broglie wavelength becomes shorter in a multiphoton in the quantum entangled state, has been proposed and studied. (see “A. N. Boto, P. Kok, D. S. Abrams, S. L. Braunstein, C. P. Williams, and J. P. Dowing, ‘Physical Review Letters’ 85 (2000) p. 2733-2736” and “D. V. Strekalov and J. P. Dowing, ‘J. Mod. Opt’ 49 (2002), p. 519.”).
In the quantum teleportation and quantum lithography, photon pairs in the quantum entangled state are inevitably required.
So far, parametric down-conversion (PDC) by using a nonlinear crystal has been used frequently to generate photon pairs in the quantum entangled state. (See P. G. Kwiat, K. Mattle, H. Weinfurter, and A. eilinger, “Physical Review Letters” 75 (1995) p. 4337-4341), and “P. G. Kwiat, E. Waks, A. G. White, I. Appelbaum, and P. H. Eberhard, “Physical Review A” 60, Number 2 (1999), R773-R776”.
Meanwhile, generation of quantum-entangled photon pairs by using a semiconductor has been proposed recently. Especially, cascade light emission occurring in quantum dots by biexciton is disclosed in “C. Santoni, D. Fattal, M. Pelton, G. G. Solomon, and Y. Yamamoto, “Physical Review B” 66 (2002) 045308”.
Moreover, in “S. Savasta, G. Martino, R. Girlanda, ‘Solid State Communications’ 111 (1999) p. 495-500”, hyper parametric scattering (hyper Raman scattering), which is in resonance with biexciton in a semiconductor crystal, is theoretically pointed out.
However, in the parametric down-conversion, a pair of quantum-entangled photons is generated from a parent photon (pump photon) via second-order non-linear process. Thus, wavelengths of the photons thus generated are double that of the parent photon. Therefore, the parametric down-conversion is difficult to generate photon pairs in a short wavelength range, and inapplicable to generation of the quantum entanglement of multiphotons, quantum lithography, and the like.
Moreover, “C. Santoni, D. Fattal, M. Pelton, G. G. Solomon, and Y. Yamamoto, “Physical Review B” 66 (2002) 045308” discusses that structural asymmetry of quantum dots prevents generation of entangled photon pairs for polarization.
Furthermore, “S. Savasta, G. Martino, R. Girlanda,’ Solid State Communications’ 111 (1999) p. 495-500”, is disclosure of a theory and leaves it uncertain whether the contents thereof can be reduced to practice or not. Moreover, this literature also discusses temporal correlation of the generated photon pairs, but does not disclose the quantum entanglement regarding polarization.
The present invention, which is accomplished in view of the aforementioned problems, has an object of attaining a method for generating quantum-entangled photon pairs, in which each photon is in a short wavelength, and which makes it possible to generate quantum-entangled photon pairs regarding polarization.
In order to attain the object, a method according to the present invention for producing a photon pair in quantum entangled state is arranged to include: radiating two parent photons to a semiconductor material, so as to induce two-photon resonance which generates biexciton that has an angular momentum of 0; and splitting the generated biexciton into two photons simultaneously, so as to generate the photon pair.
Here, the “quantum entanglement” is a state in which two particles share one wave function, and determination of a property of one of the particles determines a property of the other particle. The quantum entanglement (ryoshi motsure in Japanese) is also referred to as ryoshi karamiai in Japanese.
According to the above method, two parent photons are radiated to the semiconductor material, so as to generate biexciton. By using this biexciton, the photon pair is generated. Because of this, the photon pair thus generated has a wavelength substantially identical with that of the parent photons. This method makes it possible to easily produce a pair of photons in a shorter wavelength than in the conventional art in which generated photons have a wavelength double of that of parent photons.
Moreover, the biexciton, the intermediate product between the parent photons and the photon pair, has an angular momentum J of 0 (that is, the biexciton is in its ground state at which the biexciton is not polarized). This results in quantum entanglement of the photon pair in terms of polarization, the photon pair being produced by simultaneously splitting the biexciton. That is, this method makes it possible to produce photon pairs in the quantum entangled state in terms of polarization.
The photon pair thus generated is applicable to, e.g., quantum teleportation. That is, the photon pair thus generated is in the state of quantum entangled state in terms of polarization. Thus, determination of the polarization state of one of the photon readily determines the polarization state of the other photon regardless of a distance between the photons. This makes it possible to transfer information instantaneously.
Moreover, the photon pair thus generated is also applicable to, e.g., lithography. In lithography using light, which is a classic electromagnetic wave, a wavelength of the light can be regarded as de Broglie wavelength of one photon. In case of the photon pair in the quantum entangled state, however, the photon pair (a system composed of two photons) has a momentum double of that of the individual photons. Thus, the de Broglie wavelength of the photon pair is a half of the wavelength of one photon. As a result, the lithography using the photon pair can have spatial resolution improved to be double that of the conventional lithography. This attains finer fabrication than before.
For a fuller understanding of the nature and advantages of the invention, reference should be made to the ensuing detailed description taken in conjunction with the accompanying drawings.
The present invention is a method for generating quantum-entangled photon pairs by utilizing resonant hyper parametric scattering in resonance to biexciton (a combination of two exciton) in a semiconductor crystal, the photon pairs being quantum-entangled in terms of energy (frequency), momentum (frequency vector) and polarization.
Firstly, hyper parametric scattering (Resonant Hyper Parametric Scattering: hereinafter RHPS) through which photon pairs are generated is explained.
In Example of the present application, biexciton is generated by inducing two-photon resonance in such a manner that the generated biexciton has angular momentum J=0 (ground state of biexciton). When the angular momentum of biexciton is 0, the scattered photon pair from such biexciton will have angular momentum of 0 in sum. By this, the scattered photon pair falls into the state of quantum entanglement in terms of polarization.
The photon pair in the state of quantum entanglement regarding polarization has a function of a polarization state ψ expressed as follows:
where Li, Ri, Hi, and Li respectively represent the states for left-circular, right-circular, horizontal linear, and vertical linear polarizations of the respective daughter photons i.
The following explains Example which specifically exemplifies the method of the present invention for producing the photon pairs, and evaluation results of the generated photon pairs, referring to
The mode-locked titanium-sapphire laser apparatus 11 is a titanium-sapphire laser apparatus for generating a laser beam in a short pulse. The mode-locked titanium-sapphire laser apparatus 11 outputs a laser beam in a predetermined wavelength, a predetermined pulse width, and a predetermined repetition frequency. The SHG crystal 12 is a crystal of lithium-triborate (LiB3O5:LBO) crystal. The SHG crystal 12 creates a second higher harmonics from the laser beam outputted from the mode-locked titanium-sapphire laser apparatus 11. Then, the created second higher harmonics is radiated to a sample placed in the cryostat 13, which maintains the sample at a low temperature.
The photon pairs from the sample in the cryostat 13 are scattered by RHPS. The condensing lenses 21a and 21b are configured to condense the scattered photons of the photon pairs to the optical fibers 23a and 23b. Before the optical fibers 23a and 23b, the polarizers 22a and 22b are respectively provided, each of which includes a quarter wave plate and a linear polarizer. Polarization state of the photons passing the polarizers 22a and 22b can be changed by configuring the polarizers 22a and 22b as appropriate. The optical fibers 23a and 23b are configured to guide, to the monochromators 24a and 24b, the photons that have passed through the polarizers 22a and 22b.
Different phase-matching conditions cause the photon pairs to be scattered by RHPS in different directions. Therefore, the condensing lenses 21a and 21b, polarizers 22a and 22b, and optical fibers 23a and 23b are arranged at appropriate positions to satisfy the phase-matching conditions.
The condensed photons are split into monochrome light of a predetermined wavelength via the two monochromators 24a and 24b. The number of photons of light split via the monochromators 24a and 24b is counted by the PMTs 26a and 26b. The time interval analyzer 27 measures temporal correlations of monopulse from the PMTs 26a and 26b with approximately 300 ps resolution. The data processing apparatus 29 is configured to display the data of analysis of the time interval analyzer 27, and perform predetermined data processing of the data.
The monochromator 24a is provided with the CCD 25 for monitoring spectrum of the light introduced into the monochromator 24a. The data processing apparatus 28 is configured to display the spectrum monitored by the CCD 25, and perform predetermined data processing of the spectrum.
In the present Example, a semiconductor monocrystal of cuprous chloride (CuCl) was used as the sample for generating the photon pairs. CuCl, which has a relatively large band gap (approximately 3.4 eV), is suitable for generating photon pairs in a short wavelength such as ultraviolet band. Moreover, CuCl monocrystal has a large binding energy for exciton and biexciton (approximately 200 meV for exciton, and approximately 30 meV for biexciton). Thus, CuCl monocrystal allows both exciton and biexciton to exist therein in a very stable state under low temperature. These properties make the CuCl monocrystal suitable for the experiment of the hyper parametric scattering that is in resonance to the biexciton.
The CuCl monocrystal was placed in the cryostat 13 in which a temperature of 4K was maintained. Moreover, the mode-locked titanium-sapphire laser apparatus 11 was adjusted to output such a laser beam that the pump photons emitted from the SHG crystal 12 was the second higher harmonics of the mode-locked titanium-sapphire laser (i.e., wavelength: 389 nm (ultraviolet band wavelength), pulse width: 8 ps, repetition frequency: 80 MHz). In this Example, the pump photons had a photon energy 3.1861 eV, which corresponds to the energy that is required to generate, in the CuCl monocrystal, biexciton of angular momentum J of 0 by two-photon resonance.
With this configuration, radiation of two pump photons onto the CuCl monocrystal generated one biexciton of angular momentum J=0 in the CuCl monocrystal, as illustrated in
The one of the scattered photon pairs was passed through the condensing lens 21a, polarizer 22a, and optical fiber 23a, and then condensed to the monochromator 24a. Similarly, the other one of the scattered photons was passed through the condensing lens 21b, polarizer 22b, and optical fiber 23b, and then condensed to the monochromator 24b.
On both sides of the Rayleigh scattering light, two peaks having photon energies, which are symmetric to each other with respect to the Rayleigh scattering light, were observed (in
Moreover, in
Peaks other than the peak at the time difference τ=0 were caused between photons having no correlation therebetween. The “photons having no correlation” are emitted from different biexcitons generated by pump pulses continuously introduced into the sample. The peak at the time difference τ=0 also includes a peak component (non-correlation component) between the photons emitted from different biexcitons. The non-correlation peak component has the same quantity as the peaks other than the peak at the time difference τ=0.
As described above, biexciton with angular momentum J=0 was generated in the CuCl monocrystal by two-photon resonance, and the biexciton was spontaneously converted into the photon pairs. From the experiment results shown in
In
In
Furthermore, density matrix of two-photon polarization was worked out by measuring signals obtained in polarization combinations (≧16) of H (horizontal linear polarization), V (vertical linear polarization), R (right-circular polarization), L (left-circular polarization), D (linear polarization at 45°), and D′ (linear polarization at −45°).
As shown in
Fidelity F for the state Ψ is expressed as Equation (2):
F≡Ψ|ρ|Ψ (2),
where ρ is the density matrix measured, and |Ψ> is state vector. In the present Example, it was assumed that the photon pairs had a state vector expressed as Equation (3):
The fidelity F for the observed state was 0.83. This significantly exceeds the classic limit (F=0.5). Thus, it was proved that the observed state held quantum entanglement, which was not attainable classically.
In the literature “S. Savasta, G. Martino, R. Girlanda, ‘Solid State Communications’ 111 (1999) p. 495-500”, scattering by RHPS is theoretically pointed out, but does not show actual generation of photon pairs by experiment. Moreover, this literature does not disclose the feature that biexciton has angular momentum J=0. On the other hand, the inventors of the present invention succeeded, by experiment, to generate photon pairs being correlated with each other in terms of energy, momentum, and time, and holing quantum entanglement in terms of polarization. The inventors of the present invention generated such photon pairs by generating, in a semiconductor crystal, biexciton with angular momentum J=0 (ground state of biexciton).
Moreover, the wavelength of photons generated by conventional parametric down-conversion disclosed in the literature “C. Santoni, D. Fattal, M. Pelton, G. G. Solomon, and Y. Yamamoto, “Physical Review B” 66 (2002) 045308” is double that of the pump photons. On the other hand, the photons generated in the present Example had a wavelength substantially equal to that of the pump photons. According to the present Example, therefore, it becomes possible to generate quantum-entangled photons in a shorter wavelength than in the conventional art. In the present Example, the wavelength of the generated photons was approximately 390 nm (wavelength of ultraviolet band), which was substantially equal to that of the pump photons.
The photon pairs generated in the above mentioned manner shared one wave function expressed as Equation (1). Let photons of a photon pair sharing one wave function be photon A and photon B, and information to be transmitted from a sender to a receiver be information c, and let the sender have photon A and the receiver have photon B. The photon A and the photon C carrying the information c are caused to be in the state of quantum entanglement in terms of polarization, and observed in a commutable quantity. The quantum information is lost in accordance with the uncertainty principle, but the information carried by the photon C is transferred to photon B that is originally in the state of quantum entanglement with the photon A. That is, information c can be transferred instantaneously. This realizes quantum teleportation.
Moreover, the wavelength λ of light as classical electromagnetic wave can be regarded as de Broglie wavelength of one photon. Consider two photons paired in the state of quantum entanglement in terms of energy, momentum, and polarization, as described above. Let momentum of photons be p, then momentum of a system made up of two photons is 2p. Thus, the de Broglie wavelength λ2 in this system is expressed as:
λ2=h/2p=λ/2.
This is a half of the wavelength of one photon.
In the conventional optical lithography, the limit of the spatial resolution due to light diffraction makes it difficult to realize fabrication as fine as or finer than the order of light wavelength. However, the photon pairs generated by RHPS are correlated with each other in terms of time, energy, and momentum. Thus, the system in which the photons are paired as photon pairs, the de Broglie wavelength is approximately half of the wavelength of each photons. That is, de Broglie wavelength is the approximately half of the wavelength of the pump photons used for generating the biexciton. As a result, the quantum lithography using the quantum-entangled photon pairs has spatial resolution improved to be double that of the classical lithography. In the above embodiment, the wavelength of the photons in the quantum entanglement is approximately 390 nm, then the de Broglie wavelength of the photon pairs is approximately 195 nm. Thus, the use of the photon pairs in the quantum lithography makes it possible to realize fine fabrication of approximately 195 nm.
As described above, a method according to the present invention for producing a photon pair in quantum entangled state is arranged to include: radiating two parent photons to a semiconductor material, so as to induce two-photon resonance which generates biexciton that has an angular momentum of 0; and splitting the generated biexciton into two photons simultaneously, so as to generate the photon pair. With this arrangement, it is possible to generate photon pair in short wavelength and in the quantum entangled state in terms of the polarization.
Furthermore, it is preferable in the method according to the present invention that the semiconductor material be cuprous chloride.
CuCl, which has a relatively large band gap (approximately 3.4 eV), is suitable for generating photon pairs in a short wavelength such as ultraviolet band. Moreover, CuCl has a large binding energy for exciton and biexciton. Thus, CuCl allows both exciton and biexciton to exist therein in a very stable state under low temperature. This arrangement allows stable existence of the biexciton, which is generated as the intermediate product, thereby attaining more reliable generation of photon pair.
Furthermore, it is preferable in the method according to the present invention that the parent photons have a wavelength in the ultraviolet band.
As described above, the wavelength of the photons of the photon pair thus generated is substantially equal to that of the parent photons. Thus, this arrangement allows that the wavelength of the photon pairs thus generated is a short wavelength within the ultraviolet band. For example, the lithography using the photon pair thus generated can realize finer fabrication than can the conventional art.
The invention being thus described, it will be obvious that the same may be varied in many ways. Such variations are not to be regarded as a departure from the spirit and scope of the invention, and all such modifications as would be obvious to one skilled in the art are intended to be included within the scope of the following claims.
According to the present invention, it is possible to generate photon pairs correlated with each other in terms of energy, momentum, and time, and in a quantum entangled state regarding polarization. Because the photon pairs are in the quantum entangled state in terms of polarization, the photon pairs are applicable to quantum information/communication technology such as quantum cryptography, in which quantum teleportation is utilized. Moreover, the photons thus generated is in a short wavelength. This makes the photon pair applicable to quantum imaging technologies such as quantum lithography, which can exceed classical diffraction limit.