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1. 发明授权

US07731837B2 Oxidatively regenerable adsorbents for sulfur removal 失效
标题翻译：用于除硫的氧化可再生吸附剂
公开(公告)号：US07731837B2
公开(公告)日：2010-06-08
申请号：US11899964
申请日：2007-09-07
申请人： Chunshan Song , Xiaoliang Ma , Shingo Watanabe , Fuxia Sun
发明人： Chunshan Song , Xiaoliang Ma , Shingo Watanabe , Fuxia Sun
IPC分类号： C10G29/00
CPC分类号： C10G29/16 , B01D53/02 , B01D2253/112 , B01D2256/24 , B01D2257/30 , B01J20/0207 , B01J20/0211 , B01J20/06 , C01F17/0018 , C01F17/0043 , C01G3/00 , C01G5/00 , C01G7/00 , C01G21/006 , C01G23/00 , C01G23/002 , C01G23/003 , C01G23/04 , C01G23/047 , C01G25/02 , C01G31/02 , C01G37/02 , C01G39/02 , C01G41/02 , C01G45/02 , C01G49/02 , C01G51/04 , C01G53/04 , C01G55/004 , C01P2002/54 , C01P2004/80 , C01P2006/80
摘要： Compositions and processes are disclosed for removing sulfur and sulfur compounds from hydrocarbon fuel feedstocks. The feedstock is contacted with a regenerable sorbent such as a compound of the formula TixCeyO2 where 0
摘要翻译：公开了从烃燃料原料中除去硫和硫化合物的组合物和方法。原料与可再生的吸附剂接触，例如式TixCeyO2的化合物，其中0

2. 发明授权

US6156693A Method for preparing a highly active, unsupported high-surface-area ub . MoS.s2 catalyst 有权
标题翻译：制备高活性，未负载的高表面积MoS2催化剂的方法
公开(公告)号：US6156693A
公开(公告)日：2000-12-05
申请号：US413121
申请日：1999-10-06
申请人： Chunshan Song , Yoshiharu Yoneyama , Madhusudan Reddy Kondam
发明人： Chunshan Song , Yoshiharu Yoneyama , Madhusudan Reddy Kondam
IPC分类号： B01J27/051 , C01G39/06 , B01J27/05 , C01B17/00
CPC分类号： B01J27/051 , C01G39/06
摘要： The present invention is a new and simple method of decomposing ammonium tetrathiomolybdate (ATTM) in an organic solvent with added water under H.sub.2 pressure. Model compound reactions of 4-(1-naphthylmethyl)bibenzyl (NMBB) were carried out at 350-425.degree. C. under H.sub.2 pressure in order to examine the activity of the Mo sulfide catalysts generated from ATTM with and without added water for C--C bond cleavage and hydrogenation of aromatic ring. The Mo sulfide catalysts generated from ATTM with added water were much more effective for C--C bond cleavage and hydrogenation of aromatic moieties at 350-425.degree. C. than those from ATTM alone. Two-step tests revealed that the addition of water is effective for generating highly active Mo sulfide catalyst from ATTM, but water itself does not promote catalytic conversion. Removal of water after the decomposition of ATTM with added water at 350-400.degree. C. under H.sub.2 pressure by hot purging gives highly active Mo sulfide catalyst.
摘要翻译：本发明是一种在H2压力下加入水分解有机溶剂中四硫代钼酸铵（ATTM）的新型简单方法。在氢气压力下，在350-425℃下进行4-（1-萘基甲基）联苄（NMBB）的模型化合物反应，以便检测由ATTM生成的硫化钼催化剂的活性，并且不加入水分用于CC键芳环的裂解和氢化。由ATTM生成的添加水的Mo硫化物催化剂在350-425℃比单独的ATTM对C-C键断裂和芳烃部分氢化更有效。两步测试表明，添加水对于从ATTM产生高活性的硫化钼催化剂是有效的，但是水本身不能促进催化转化。在氢气压力下通过热吹扫在350-400℃加入ATTM分解后除去水，得到高活性的硫化钼催化剂。

3. 发明授权

US5523505A Zeolite-catalyzed isomerization of sym-octahydrophenanthrene to sym-octahydroanthracene 失效
标题翻译：对称八氢菲的沸石催化异构化与对映八氢蒽
公开(公告)号：US5523505A
公开(公告)日：1996-06-04
申请号：US290648
申请日：1994-08-15
申请人： Chunshan Song
发明人： Chunshan Song
IPC分类号： C07C5/27 , C07C5/22
CPC分类号： C07C5/2708 , C07C2103/24 , C07C2529/08
摘要： An environmentally benign catalytic process for the production of sym-octahydroanthracene (sym-OHA) from sym-octahydrophenanthrene (sym-OHP) by ring-shift isomerization. Proton-form moralenite or partially dealuminated proton-form mordenite are effective catalysts for the selective formation of sym-OHA from sym-OHP. Y-zeolite and metal-ion exchanged Y-zeolites display lower selectivity towards Sym-OHA. The use of certain solvents can further improve the performance of the Y-zeolites and mordenites, particularly the selectivity of Y-zeolite catalysts. The sym-OHA is an useful product and can be converted by existing methods to various anthracene derivatives which are industrial chemicals in demand.
摘要翻译：通过环移异构化从sym八氢菲（sym-OHP）生产对称八氢蒽（sym-OHA）的环境友好的催化方法。质子形式的光子沸石或部分脱铝的质子型丝光沸石是从sym-OHP选择性形成sym-OHA的有效催化剂。 Y-沸石和金属离子交换的Y-沸石对Sym-OHA的选择性较低。使用某些溶剂可以进一步提高Y-沸石和丝光沸石的性能，特别是Y-沸石催化剂的选择性。 sym-OHA是一种有用的产品，可以通过现有方法转化为需要的工业化学品的各种蒽衍生物。

4. 发明申请

US20080265212A1 Sulfur-tolerant and carbon-resistant catalysts 有权
标题翻译：耐硫和耐碳催化剂
公开(公告)号：US20080265212A1
公开(公告)日：2008-10-30
申请号：US12007983
申请日：2008-01-17
申请人： Chunshan Song , James J. Strohm , Jian Zheng , Weidong Gu , Chao Xie , Xiaoxing Wang
发明人： Chunshan Song , James J. Strohm , Jian Zheng , Weidong Gu , Chao Xie , Xiaoxing Wang
IPC分类号： B01J21/04 , C01B3/26
CPC分类号： B01J37/0207 , B01J21/04 , B01J23/60 , B01J23/62 , B01J23/6525 , B01J23/89 , B01J23/8913 , B01J23/892 , B01J23/894 , B01J23/8946 , B01J23/896 , B01J37/0009 , B01J37/0236 , C01B3/38 , C01B3/382 , C01B3/40 , C01B2203/0233 , C01B2203/0244 , C01B2203/066 , C01B2203/1047 , C01B2203/1058 , C01B2203/1082 , C01B2203/1211 , Y02P20/52
摘要： The invention relates to novel bimetallic and trimetallic catalysts, their manufacture and use in both steam reforming and oxidative steam reforming of liquid fuels such as jet fuels, diesel fuels and gasoline to produce synthesis gas and/or hydrogen for fuel cell applications. The invention further relates to manufacture of synthesis gas and/or hydrogen gas for chemicals synthesis and fuel processing. The catalysts have high sulfur tolerance and carbon resistance when used in steam reforming and/or oxidative steam reforming of heavy hydrocarbon fuels.
摘要翻译：本发明涉及新颖的双金属和三金属催化剂，它们在液体燃料例如喷气燃料，柴油燃料和汽油的蒸汽重整和氧化蒸汽重整中用于燃料电池应用产生合成气和/或氢气的制造和应用。本发明还涉及用于化学品合成和燃料处理的合成气和/或氢气的制造。当用于重烃燃料的蒸汽重整和/或氧化蒸汽重整中时，催化剂具有高耐硫和耐碳性。

5. 发明授权

US07022637B2 Selective methylation catalyst, method of catalyst manufacture and methylation process 失效
标题翻译：选择性甲基化催化剂，催化剂制备方法和甲基化方法
公开(公告)号：US07022637B2
公开(公告)日：2006-04-04
申请号：US09771876
申请日：2001-01-29
申请人： Chunshan Song , Jian-Ping Shen , Lawrence D. Lillwitz
发明人： Chunshan Song , Jian-Ping Shen , Lawrence D. Lillwitz
IPC分类号： B01J29/06
CPC分类号： C07C2/864 , B01J29/04 , C07C2/865 , C07C2529/08 , C07C2529/18 , C07C2529/40 , C07C2529/60 , C07C2529/70 , C07C15/24
摘要： Novel catalysts and processes in accordance with the invention can accomplish high selectivity and conversion of naphthalenic compounds such as the conversion of methylnaphthalene (2-MN) or naphthalene to 2,6-dimethylnaphthalene (2,6-DMN). The catalysts are prepared by treating, for example, a ZSM-5-type material with iron in the presence of a halogen such as a fluoride. The resulting catalyst includes iron, as well as a significant portion of aluminum present in the ZSM-5-type starting material. Processes for using the catalysts also are disclosed.
摘要翻译：根据本发明的新型催化剂和方法可以实现萘化合物的高选择性和转化率，例如将甲基萘（2-MN）或萘转化为2,6-二甲基萘（2,6-DMN）。催化剂通过在诸如氟化物的卤素存在下用铁处理例如ZSM-5型材料来制备。所得催化剂包括铁，以及存在于ZSM-5型起始原料中的大部分铝。还公开了使用催化剂的方法。

6. 发明授权

US09387470B2 Sulfur-tolerant and carbon-resistant catalysts 有权
标题翻译：耐硫和耐碳催化剂
公开(公告)号：US09387470B2
公开(公告)日：2016-07-12
申请号：US12007983
申请日：2008-01-17
申请人： Chunshan Song , James J. Strohm , Jian Zheng , Weidong Gu , Chao Xie , Xiaoxing Wang
发明人： Chunshan Song , James J. Strohm , Jian Zheng , Weidong Gu , Chao Xie , Xiaoxing Wang
IPC分类号： B01J23/00 , B01J23/58 , B01J37/02 , B01J23/60 , B01J23/62 , B01J23/652 , B01J23/89 , C01B3/38 , C01B3/40 , B01J21/04 , B01J37/00
CPC分类号： B01J37/0207 , B01J21/04 , B01J23/60 , B01J23/62 , B01J23/6525 , B01J23/89 , B01J23/8913 , B01J23/892 , B01J23/894 , B01J23/8946 , B01J23/896 , B01J37/0009 , B01J37/0236 , C01B3/38 , C01B3/382 , C01B3/40 , C01B2203/0233 , C01B2203/0244 , C01B2203/066 , C01B2203/1047 , C01B2203/1058 , C01B2203/1082 , C01B2203/1211 , Y02P20/52
摘要： The invention relates to novel bimetallic and trimetallic catalysts, their manufacture and use in both steam reforming and oxidative steam reforming of liquid fuels such as jet fuels, diesel fuels and gasoline to produce synthesis gas and/or hydrogen for fuel cell applications. The invention further relates to manufacture of synthesis gas and/or hydrogen gas for chemicals synthesis and fuel processing. The catalysts have high sulfur tolerance and carbon resistance when used in steam reforming and/or oxidative steam reforming of heavy hydrocarbon fuels.
摘要翻译：本发明涉及新颖的双金属和三金属催化剂，它们在液体燃料例如喷气燃料，柴油燃料和汽油的蒸汽重整和氧化蒸汽重整中用于燃料电池应用产生合成气和/或氢气的制造和应用。本发明还涉及用于化学品合成和燃料处理的合成气和/或氢气的制造。当用于重烃燃料的蒸汽重整和/或氧化蒸汽重整中时，催化剂具有高耐硫和耐碳性。

7. 发明授权

US06451729B1 Method for preparing a highly active, unsupported high surface-area MoS2 catalyst 失效
标题翻译：制备高活性，未负载的高表面积MoS2催化剂的方法
公开(公告)号：US06451729B1
公开(公告)日：2002-09-17
申请号：US09687046
申请日：2000-10-13
申请人： Chunshan Song , Yoshiharu Yoneyama , Madhusudan Reddy Kondam
发明人： Chunshan Song , Yoshiharu Yoneyama , Madhusudan Reddy Kondam
IPC分类号： B01J2705
CPC分类号： B01J27/051 , C01G39/06
摘要： The present invention is a new and simple method of decomposing ammonium tetrathiomolybdate (ATTM) in an organic solvent with added water under H2 pressure. Model compound reactions of 4-(1-naphthylmethyl)bibenzyl (NMBB) were carried out at 350-425° C. under H2 pressure in order to examine the activity of the Mo sulfide catalysts generated from ATTM with and without added water for C—C bond cleavage and hydrogenation of aromatic ring. The Mo sulfide catalysts generated from ATTM with added water were much more effective for C—C bond cleavage and hydrogenation of aromatic moieties at 350-425° C. than those from ATTM alone. Two-step tests revealed that the addition of water is effective for generating highly active Mo sulfide catalyst from ATTM, but water itself does not promote catalytic conversion. Removal of water after the decomposition of ATTM with added water at 350-400° C. under H2 pressure by hot purging gives highly active Mo sulfide catalyst.
摘要翻译：本发明是一种在H2压力下加入水分解有机溶剂中四硫代钼酸铵（ATTM）的新型简单方法。在氢气压力下，在350-425℃下进行4-（1-萘基甲基）联苄（NMBB）的模型化合物反应，以检查由ATTM生成的硫化钼催化剂的活性，并且没有添加水用于CC键芳环的裂解和氢化。从ATTM生成的添加水的Mo硫化物催化剂在350-425℃比单独的ATTM对C-C键断裂和芳烃部分氢化更有效。两步测试表明，添加水对于从ATTM产生高活性的硫化钼催化剂是有效的，但是水本身不能促进催化转化。通过热吹扫在氢气压力下，在350-400℃下加入水分解ATTM后除去水分，得到高活性的硫化钼催化剂。

8. 发明申请

US20090065400A1 Oxidatively regenerable adsorbents for sulfur removal 失效
标题翻译：用于除硫的氧化可再生吸附剂
公开(公告)号：US20090065400A1
公开(公告)日：2009-03-12
申请号：US11899964
申请日：2007-09-07
申请人： Chunshan Song , Xiaoliang Ma , Shingo Watanabe , Fuxia Sun
发明人： Chunshan Song , Xiaoliang Ma , Shingo Watanabe , Fuxia Sun
IPC分类号： C10G29/00 , C01F17/00
CPC分类号： C10G29/16 , B01D53/02 , B01D2253/112 , B01D2256/24 , B01D2257/30 , B01J20/0207 , B01J20/0211 , B01J20/06 , C01F17/0018 , C01F17/0043 , C01G3/00 , C01G5/00 , C01G7/00 , C01G21/006 , C01G23/00 , C01G23/002 , C01G23/003 , C01G23/04 , C01G23/047 , C01G25/02 , C01G31/02 , C01G37/02 , C01G39/02 , C01G41/02 , C01G45/02 , C01G49/02 , C01G51/04 , C01G53/04 , C01G55/004 , C01P2002/54 , C01P2004/80 , C01P2006/80
摘要： Compositions and processes are disclosed for removing sulfur and sulfur compounds from hydrocarbon fuel feedstocks. The feedstock is contacted with a regenerable sorbent such as a compound of the formula TixCeyO2 where 0
摘要翻译：公开了从烃燃料原料中除去硫和硫化合物的组合物和方法。原料与可再生的吸附剂例如式TixCeyO2的化合物接触，其中0

9. 发明申请

US20080264254A1 Novel sorbents and purification and bulk separation of gas streams 审中-公开
公开(公告)号：US20080264254A1
公开(公告)日：2008-10-30
申请号：US12081036
申请日：2008-04-09
申请人： Chunshan Song , Xiaoliang Ma , Xiaoxing Wang
发明人： Chunshan Song , Xiaoliang Ma , Xiaoxing Wang
IPC分类号： B01D53/02 , B01J20/26
CPC分类号： B01D53/02 , B01D53/06 , B01D2253/202 , B01D2256/16 , B01D2257/2045 , B01D2257/2047 , B01D2257/2064 , B01D2257/302 , B01D2257/304 , B01D2257/306 , B01D2257/308 , B01D2257/402 , B01D2257/404 , B01D2257/406 , B01D2257/408 , B01D2257/504 , B01D2257/70 , B01D2258/0208 , B01D2258/05 , B01D2258/06 , B01D2259/40009 , B01D2259/40088 , B01D2259/402 , B01J20/103 , B01J20/16 , B01J20/20 , B01J20/22 , B01J20/26 , B01J20/28057 , B01J20/28069 , B01J20/3092 , B01J20/3204 , B01J20/3242 , B01J20/3272 , B01J20/3425 , B01J20/3458 , B01J20/3483 , B01J2220/42 , C12M47/18 , Y02C10/08 , Y02C20/10 , Y02E50/346 , Y02P20/59
摘要： Porous-material-supported polymer sorbents and process for removal of undesirable gases such as H2S, COS, CO2, N2O, NO, NO2, SO2, SO3, HCl, HF, HCN, NH3, H2O, C2H5OH, CH3OH, HCHO, CHCl3, CH2Cl2, CH3Cl, CS2, C4H4S, CH3SH, and CH3—S—CH3 from various gas streams such as natural gas, coal/biomass gasification gas, biogas, landfill gas, coal mine gas, ammonia syngas, H2 and oxo-syngas, Fe ore reduction gas, reformate gas, refinery process gases, indoor air, fuel cell anode fuel gas and cathode air are disclosed. The sorbents have numerous advantages such as high breakthrough capacity, high sorption/desorption rates, little or no corrosive effect and are easily regenerated. The sorbents may be prepared by loading H2S—, COS—, CO2—, N2O, NO—, NO2—, SO2—, SO3—, HCl—, HF—, HCN—, NH3—, H2O—, C2H5OH—, CH3OH—, HCHO—, CHCl3—, CH2Cl2—, CH3Cl—, CS2—, C4H4S—, CH3SH—, CH3—S—CH3-philic polymer(s) or mixtures thereof, as well as any one or more of H2S—, COS—, CO2—, N2O, NO—, NO2—, SO2—, SO3—, HCl—, HF—, HCN—, NH3—, H2O—, C2H5OH—, CH3OH—, HCHO—, CHCl3—, CH2Cl2—, CH3Cl—, CS2—, C4H4S—, CH3SH—, CH3—S—CH3-philic compound(s) or mixtures thereof on to porous materials such as mesoporous, microporous or macroporous materials. The sorbents may be employed in processes such as one-stage and multi-stage processes to remove and recover H2S, COS, CO2, N2O, NO, NO2, SO2, SO3, HCl, HF, HCN, NH3, H2O, C2H5OH, CH3OH, HCHO, CHCl3, CH2Cl2, CH3Cl, CS2, C4H4S, CH3SH and CH3—S—CH3 from gas streams by use of, such as, fixed-bed sorbers, fluidized-bed sorbers, moving-bed sorbers, and rotating-bed sorbers.

10. 发明授权

US08158843B2 Deep desulfurization of hydrocarbon fuels 有权
标题翻译：碳氢燃料的深度脱硫
公开(公告)号：US08158843B2
公开(公告)日：2012-04-17
申请号：US10365574
申请日：2003-02-11
申请人： Chunshan Song , Xiaoliang Ma , Michael J. Sprague , Velu Subramani
发明人： Chunshan Song , Xiaoliang Ma , Michael J. Sprague , Velu Subramani
IPC分类号： C07C7/12 , C10G29/04
CPC分类号： C10G25/003 , C10G2300/104 , C10G2300/1044 , C10G2300/1051 , C10G2300/1055 , C10G2300/202 , C10G2300/44 , C10G2400/02 , C10G2400/04 , C10G2400/08
摘要： The invention relates to processes for reducing the sulfur content in hydrocarbon fuels such as gasoline, diesel fuel and jet fuel. The invention provides a method and materials for producing ultra low sulfur content transportation fuels for motor vehicles as well as for applications such as fuel cells. The materials and method of the invention may be used at ambient or elevated temperatures and at ambient or elevated pressures without the need for hydrogen.
摘要翻译：本发明涉及降低烃类燃料如汽油，柴油和喷气燃料中的硫含量的方法。本发明提供了用于生产用于机动车辆的超低硫含量运输燃料以及诸如燃料电池的应用的方法和材料。本发明的材料和方法可以在环境温度或升高的温度以及环境或升高的压力下使用，而不需要氢气。

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