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1. 发明申请

WO2004081116A1 ORIENTED THERMOPLASTIC ELASTOMER FILM AND PROCESS FOR PRODUCING THE SAME 审中-公开
标题翻译：面向热塑性弹性体膜及其制造方法
公开(公告)号：WO2004081116A1
公开(公告)日：2004-09-23
申请号：PCT/US2003/006560
申请日：2003-03-06
申请人： EXXONMOBIL CHEMICAL PATENTS, INC. , THE YOKOHAMA RUBBER CO., LTD. , SOEDA, Yoshihiro , TSOU, Andy, Haishung , CARAWAY, Joyce, Foshee
发明人： SOEDA, Yoshihiro , TSOU, Andy, Haishung , CARAWAY, Joyce, Foshee
IPC分类号： C08L77/00
CPC分类号： C08L77/06 , C08L23/283 , C08L77/00 , C08L77/02 , Y10T428/249921 , Y10T428/254 , Y10T428/26 , Y10T428/268 , Y10T428/269 , C08L2666/20 , C08L2666/06 , C08L2666/08 , C08L2666/04
摘要： An oriented thermoplastic elastomer film having reduced permeability and improved fatigue resistance comprising a dynamically vulcanized polymer blend of (A) a halogenated isobutylene elastomer and (B) polyamide, the film is produced by casting or blowing the above polymer blend under the condition such that a shear rate at a die lip for casting or blowing is regulated to control the molecular arrangement in the film, whereby the planar birefringemence (PBR) of the resultant film becomes greater or equal to 0.002 and a production process of the same.
摘要翻译：一种具有降低的渗透性和改善的耐疲劳性的定向热塑性弹性体膜，其包含（A）卤代异丁烯弹性体和（B）聚酰胺的动态硫化聚合物共混物，该膜通过在上述聚合物共混物的浇铸或吹塑条件下制备，调节用于铸造或吹塑的模唇的剪切速率以控制膜中的分子排列，由此所得膜的平面双折射率（PBR）变得大于或等于0.002，并且其制造方法。

2. 发明申请

WO2004081108A1 THERMOPLASTIC ELASTOMER COMPOSITION WITH AN IMPROVED RUBBER PELLETIZATION PROCESS 审中-公开
标题翻译：具有改进橡胶剥离工艺的热塑性弹性体组合物
公开(公告)号：WO2004081108A1
公开(公告)日：2004-09-23
申请号：PCT/US2003/006702
申请日：2003-03-06
申请人： THE YOKOHAMA RUBBER CO., LTD. , EXXONMOBIL CHEMICAL PATENTS, INC. , SOEDA, Yoshihiro , TSOU, Andy, Haishung , CARAWAY, Joyce, Foshee
发明人： SOEDA, Yoshihiro , TSOU, Andy, Haishung , CARAWAY, Joyce, Foshee
IPC分类号： C08L23/28
CPC分类号： C08L77/06 , C08L23/283 , C08L77/00 , C08L77/02 , C08L2312/00 , C08L2666/20 , C08L2666/08 , C08L2666/04 , C08L2666/06
摘要： A thermoplastic elastomer composition having improved durability, heat resistant andflexibility comprising a dynamically vulcanized blend of (A) a halogenated isobutylene elastomer, (B) polyamide and (C) an antioxidant having a melting temperature more than 70°C and less than 200°C, wherein the elastomer (A) is dispersed as a domain in a continuous phase of the polyamide (B) and the dynamically vulcanized blend of the components (A) and (B) is dynamically vulcanized in the presence of the antioxidant (C)as an anti-blocking agent.
摘要翻译：具有改进的耐久性，耐热性和柔韧性的热塑性弹性体组合物，其包含（A）卤化异丁烯弹性体，（B）聚酰胺和（C）熔融温度大于70℃且小于200℃的抗氧化剂的动态硫化混合物其中弹性体（A）以聚酰胺（B）的连续相的形式分散，组分（A）和（B）的动态硫化共混物在抗氧化剂（C）的存在下动态硫化为防粘剂。

3. 发明申请

WO2007111584A1 THERMOPLASTIC ELASTOMER COMPOSITION HAVING EXCELLENT LOW TEMPERATURE PROPERTY 审中-公开
标题翻译：热塑性弹性体组合物具有极佳的低温性能
公开(公告)号：WO2007111584A1
公开(公告)日：2007-10-04
申请号：PCT/US2006/011002
申请日：2006-03-24
申请人： THE YOKOHAMA RUBBER CO., LTD. , EXXONMOBIL CHEMICAL PATENTS INC. , SOEDA, Yoshihiro , TSOU, Andy Haishung , HARA, Yuichi , MEASMER, Matthew, Brian
发明人： SOEDA, Yoshihiro , TSOU, Andy Haishung , HARA, Yuichi , MEASMER, Matthew, Brian
IPC分类号： C08L23/28 , C08L23/22 , B60C1/00
CPC分类号： B60C1/0008 , C08L21/00 , C08L23/22 , C08L23/28 , C08L51/06 , C08L77/00 , C08L77/02 , C08L77/06 , C08L2205/02 , C08L2205/22 , C08L2666/20 , C08L2666/08
摘要： A thermoplastic elastomer composition a thermoplastic elastomer composed of at least partially , vulcanized first rubber component discretely dispersed in a polyamide matrix and a secondary rubber component, which is different from the first rubber component, having a glass transition temperature Tg of -30°C or less.
摘要翻译：一种热塑性弹性体组合物，由至少部分硫化的离散分散在聚酰胺基体中的硫化的第一橡胶组分和与玻璃化转变温度Tg为-30℃的与第一橡胶组分不同的第二橡胶组分组成的热塑性弹性体，或减。

4. 发明申请

WO2007081323A1 LAMINATE OF THERMOPLASTIC POLYMER COMPOSITION HAVING LOW AIR PERMEABILITY AND PNEUMATIC TIRE USING SAME AS INNER LINER 审中-公开
标题翻译：具有低空气渗透性和气动轮胎的热塑性聚合物组合物的层压体使用同一内衬
公开(公告)号：WO2007081323A1
公开(公告)日：2007-07-19
申请号：PCT/US2006/000588
申请日：2006-01-10
申请人： THE YOKOHAMA RUBBER CO., LTD. , EXXONMOBIL CHEMICAL PATENTS INC. , SOEDA, Yoshihiro , MORROKA, Naoyuki , HARA, Yuichi , TSOU, Andy Haishung
发明人： SOEDA, Yoshihiro , MORROKA, Naoyuki , HARA, Yuichi , TSOU, Andy Haishung
IPC分类号： B60C1/00 , B32B25/08
CPC分类号： B60C1/0008 , B29C47/0023 , B29C47/065 , B29C47/26 , B32B7/10 , B32B25/08 , B32B25/14 , B32B27/08 , B32B27/302 , B32B27/306 , B32B27/32 , B32B27/34 , B32B2270/00 , B32B2274/00 , B32B2307/54 , B32B2307/7242 , B32B2605/00 , Y10T428/24975 , Y10T428/249981 , Y10T428/249982 , Y10T428/31725 , Y10T428/31855 , Y10T428/31931
摘要： A laminate (C) of a thermoplastic polymer composition comprising: a thermoplastic resin composition (A) having an permeation coefficient of 10 x 10 -12 cc•cm/cm 2 •sec•cmHg or less, laminated with a thermoplastic polymer composition (B) having a melt viscosity of 500 - 2000 Pa•s and a Young's modulus at a room temperature of 1 - 400 MPa, wherein the thickness of a layer of the thermoplastic resin composition (A) is 0.05 - 10 µm and the air permeation coefficient of the laminate (C) of 20 x 10 -12 cc • cm/cm 2 • sec • cmHg or less, and a pneumatic tire using the above laminate (C) as an inner liner.
摘要翻译： 1.一种热塑性聚合物组合物的层压体（C），其包含：具有10×10 -6 cm 3 / cm 2以上的渗透系数的热塑性树脂组合物（A）以下，将热塑性树脂组合物（A）的层的厚度与熔融粘度为500〜2000Pa·s的热塑性聚合物组合物（B）和室温为1〜400MPa的杨氏模量层叠，为0.05〜10μm，层压体（C）的透气系数为20×10 -2 cm 3 / cm 2·sec·cmHg以下，充气轮胎使用上述层压体（C）作为内衬。

5. 发明申请

WO2007050076A1 LOW PERMEABILITY THERMOPLASTIC ELASTOMER COMPOSITION 审中-公开
标题翻译：低渗透性热塑性弹性体组合物
公开(公告)号：WO2007050076A1
公开(公告)日：2007-05-03
申请号：PCT/US2005/038940
申请日：2005-10-27
申请人： EXXONMOBIL CHEMICAL PATENTS INC. , THE YOKOHAMA RUBBER CO., LTD. , TSOU, Andy, Haishung , SOEDA, Yoshihiro , HARA, Yuichi , MEASMER, Matthew, Brian
发明人： TSOU, Andy, Haishung , SOEDA, Yoshihiro , HARA, Yuichi , MEASMER, Matthew, Brian
IPC分类号： C08L77/00 , B60C1/00
CPC分类号： B60C1/0008 , B60C1/00 , C08L23/26 , C08L23/28 , C08L77/00 , C08L77/02 , C08L77/06 , C08L2205/02 , C08L2205/03 , Y10T428/1352 , Y10T428/1386 , Y10T428/139 , Y10T428/1397 , C08L2666/20 , C08L2666/06
摘要： A thermoplastic elastomer composition possessing superior air impermeability, excellent durability and flexibility. In particular, the composition includes (A) at least one halogenated isobutylene-containing elastomer; and (B) at least one nylon resin having a melting point of about 170 °C to about 260 °C; and (C) a low molecular weight polymeric nylon plasticizer; wherein: (1) the at least one elastomer is present as a dispersed phase of small vulcanized particles in a continuous nylon phase; and (2) the elastomer particles are formed by dynamic vulcanization. Use of a low molecular weight nylon plasticizer provides for improved mixing and rubber dispersion while retaining the high levels of impermeability achievable by the use of nylon resin and halogenated isobutylene-containing elastomer in a dynamically vulcanized composition. Such compositions are particularly useful in applications such as tire innerliners and barrier films or layers as well as hoses.
摘要翻译：具有优异的防空气性，优异的耐久性和柔软性的热塑性弹性体组合物。特别地，组合物包括（A）至少一种含卤代异丁烯的弹性体; 和（B）至少一种熔点为约170℃至约260℃的尼龙树脂; 和（C）低分子量聚合尼龙增塑剂; 其中：（1）所述至少一种弹性体作为连续尼龙相中的小硫化颗粒的分散相存在; 和（2）弹性体颗粒通过动态硫化形成。使用低分子量尼龙增塑剂可提供改进的混合和橡胶分散体，同时保持在动态硫化组合物中使用尼龙树脂和含卤代异丁烯的弹性体可实现的高水平的不渗透性。这样的组合物在诸如轮胎内衬和阻隔膜或层以及软管的应用中特别有用。

6. 发明申请

WO2014039043A1 CONSTRUCTION COMPRISING TIE LAYER 审中-公开
标题翻译：施工包括层层
公开(公告)号：WO2014039043A1
公开(公告)日：2014-03-13
申请号：PCT/US2012/053944
申请日：2012-09-06
申请人： EXXONMOBIL CHEMICAL PATENTS INC. , THE YOKOHAMA RUBBER CO., LTD. , KEUNG, Jay, Kin Ming , RODGERS, Michael, Brendan , SHANNON, Porter, C. , TSOU, Andy, Haishung , HARA, Yuichi , SHIBATA, Hirokazu , SOEDA, Yoshihiro
发明人： KEUNG, Jay, Kin Ming , RODGERS, Michael, Brendan , SHANNON, Porter, C. , TSOU, Andy, Haishung , HARA, Yuichi , SHIBATA, Hirokazu , SOEDA, Yoshihiro
IPC分类号： B32B25/04 , B32B25/08 , B32B25/14 , B32B25/18 , B32B27/00 , B32B27/16 , B32B27/22 , B32B27/34 , B60C1/00 , B60C5/14 , C08L23/28
CPC分类号： B32B25/042 , B32B25/08 , B32B25/14 , B32B25/18 , B32B27/00 , B32B27/16 , B32B27/22 , B32B27/34 , B32B2270/00 , B32B2307/7242 , B32B2605/00 , B60C1/0008 , B60C2005/145 , C08G69/36 , C08K5/0025 , C08K5/01 , C08L23/0815 , C08L23/283 , C08L77/02 , C08L77/06 , C08L2312/00 , C08L2314/06 , C08L2666/68 , C09J4/06 , C09J123/0815 , C09J123/22 , C09J123/283 , C09J193/04
摘要： A layered structure suitable for use in a pneumatic tire as an innerliner is prepared by directly bonding a fluid permeation prevention film and an adhesive tie layer together. Prior to bonding the two layers, the fluid permeation prevention layer is treated to remove any residual plasticizers or oils on the surface of the film. The tie layer comprises a mixture of 100 weight % of at least one halogenated isobutylene containing elastomer and about 1 to about 20 parts per hundred (phr) of at least one tackifier. The fluid permeation prevention film comprises an elastomeric component dispersed in a vulcanized or partially vulcanized state, as a discontinuous phase, in a matrix of the thermoplastic resin component. The two layers of the layered structure may be separately extruded and then adhered to each other or adhered to each other during a calendering operation wherein the adhesive tie layer composition is coated onto the treated film.
摘要翻译：适用于充气轮胎作为内衬的分层结构通过将防流体渗透膜和粘结层直接粘合在一起来制备。在粘合两层之前，处理流体渗透防止层以去除膜表面上的任何残留的增塑剂或油。连接层包含100重量％的至少一种含卤代异丁烯的弹性体和约1至约20份/ 100（phr）的至少一种增粘剂的混合物。防止流体渗透的膜包括在热塑性树脂组分的基质中以硫化或部分硫化状态分散的不连续相的弹性体组分。层压结构的两层可以在压延操作期间被分开挤出，然后彼此粘合或彼此粘合，其中将粘合剂粘合层组合物涂覆到经处理的膜上。

7. 发明申请

WO2008088555A1 POLYAMIDE RESIN COMPOSITION HAVING SUPERIOR EXTENSIBILITY AND FLEXING FATIGUE AND PNEUMATIC TIRE AND HOSE USING THE SAME 审中-公开
标题翻译：具有超强扩展性和柔韧性疲劳的聚酰胺树脂组合物及使用其的气动轮胎和软管
公开(公告)号：WO2008088555A1
公开(公告)日：2008-07-24
申请号：PCT/US2007/060699
申请日：2007-01-18
申请人： THE YOKOHAMA RUBBER CO., LTD. , EXXONMOBIL CHEMICAL PATENTS INC. , SOEDA, Yoshihiro , HARA, Yuichi , MOROOKA, Naoyuki , TSOU, Andy, Haishung
发明人： SOEDA, Yoshihiro , HARA, Yuichi , MOROOKA, Naoyuki , TSOU, Andy, Haishung
IPC分类号： C08L77/00 , C08L77/02 , C08L77/06 , F16L11/04 , B60C1/00
CPC分类号： C08L77/00 , C08L51/04 , C08L51/06 , C08L77/02 , C08L77/06 , C08L2666/14 , C08L2666/02 , C08L2666/06 , C08L2666/24
摘要： A polyamide resin composition, having an excellent extensibility and flexing fatigue, composed of a polyamide resin (A) , as a matrix, and a modifying polymer (C) ,• dispersed therein, having a functional group (B) reactive with the polyamide resin (A) , wherein a tensile stress at break of the modifying polymer (C) is 30 to 70% of the tensile stress at break of the polyamide resin (A) , and a tensile elongation at break of the modifying polymer (C) is 100 to 500% of the tensile elongation at break of the polyamide resin (A) as well as a pneumatic tire and hose using the same.
摘要翻译：具有聚酰胺树脂（A），作为基质的聚酰胺树脂（A）和分散有聚酰胺树脂（B）的官能团（B））的改性聚合物（C）具有优异的伸长性和挠曲疲劳性的聚酰胺树脂组合物 A），其中，改性聚合物（C）的断裂拉伸应力为聚酰胺树脂（A）的断裂拉伸应力的30〜70％，改性聚合物（C）的拉伸断裂伸长率为100 至聚酰胺树脂（A）的断裂拉伸伸长率的500％，以及使用其的充气轮胎和软管。

8. 发明申请

WO2004081107A1 A METHOD FOR CONTROLLING DISPERSION SIZE OF ELASTOMER IN THERMOPLASTIC ELASTOMER COMPOSITION 审中-公开
标题翻译：用于控制热塑性弹性体组合物中弹性体分散体大小的方法
公开(公告)号：WO2004081107A1
公开(公告)日：2004-09-23
申请号：PCT/US2003/006699
申请日：2003-03-06
申请人： EXXONMOBIL CHEMICAL PATENTS, INC. , THE YOKOHAMA RUBBER CO., LTD. , TSOU, Andy, Haishung , SOEDA, Yoshihiro , HARA, Yuichi
发明人： TSOU, Andy, Haishung , SOEDA, Yoshihiro , HARA, Yuichi
IPC分类号： C08L23/28
CPC分类号： C08L77/02 , C08L23/28 , C08L23/283 , C08L77/00 , C08L77/06 , C08L2312/00 , C08L2666/20 , C08L2666/04 , C08L2666/08 , C08L2666/06
摘要： A method for controlling a dispersion size of an elastomer in a thermoplastic elastomer composition having improved durability and impermeability obtained by melt-mixing (A)a halogenated isobutylene elastomer, (B) polyamide and (C) a dispersion aid, anddynamically vulcanizing the resultant blend to form the dynamically vulcanized polymer blend, wherein the halogenated isobutylene elastomer is dispersed in the polyamide matrix at a volume-average dispersion diameter of less than 2.0 µm.
摘要翻译：通过熔融混合（A）卤化异丁烯弹性体，（B）聚酰胺和（C）分散助剂获得的具有改善的耐久性和不渗透性的热塑性弹性体组合物中控制弹性体的分散体尺寸的方法，并将所得共混物动态硫化以形成动态硫化聚合物共混物，其中卤化异丁烯弹性体以小于2.0μm的体积平均分散直径分散在聚酰胺基质中。

9. 发明申请

WO2009048472A1 EFFICIENT MIXING PROCESS FOR PRODUCING THERMOPLASTIC ELASTOMER COMPOSITION 审中-公开
标题翻译：用于生产热塑性弹性体组合物的高效混合方法
公开(公告)号：WO2009048472A1
公开(公告)日：2009-04-16
申请号：PCT/US2007/081116
申请日：2007-10-11
申请人： EXXONMOBIL CHEMICAL PATENTS INC. , THE YOKOHAMA RUBBER CO., LTD. , TSOU, Andy, Haishung , HARA, Yuichi , LYON, Michael, Kenneth , SOEDA, Yoshihiro
发明人： TSOU, Andy, Haishung , HARA, Yuichi , LYON, Michael, Kenneth , SOEDA, Yoshihiro
IPC分类号： C08L77/00 , B29C47/40 , C08G81/02 , C08L27/10 , C08L23/28
CPC分类号： C08J3/005 , B29C47/0011 , B29C47/40 , C08J2377/00 , C08L15/00 , C08L23/28 , C08L23/283 , C08L77/00 , C08L2666/02 , C08L2666/06
摘要： A durable, flexible, impermeable thermoplastic elastomer composition is produced using a dynamic vulcanization process conducted in a high shear mixer at elevated temperature. The composition comprises cured particles of a first halogenated isobutylene-containing elastomer and particles of a second elastomer having at least one functional group capable of reacting with and grafting to a polyamide, the particles of the first and second elastomers dispersed in a continuous thermoplastic polyamide matrix, said process comprising: (1) dispersing a curative in the halogenated elastomer and forming a pre-compounded, preferably pelletized composition; (2) introducing polyamide resin and optional stabilizers into the mixer and shearing and heating to melt the polyamide and form a mixture; (3) introducing a nylon plasticizer to reduce the viscosity of the polyamide mixture to substantially match that of the pre-compounded elastomer under mixing conditions; (4) introducing pellets of the pre-compounded elastomer into the mixer and initiating dynamic vulcanization of the elastomer and polyamide components; (5) introducing the second elastomer and continuing heating and shearing to disperse the second elastomer and substantially complete dynamic vulcanization; and delivering the thermoplastic elastomer composition from the mixer. Such compositions are particularly useful in applications such as tire innerliners and barrier films or layers.
摘要翻译：使用在高剪切混合器中在高温下进行的动态硫化方法制备耐用的，柔性的，不渗透的热塑性弹性体组合物。该组合物包含含有第一卤代异丁烯的弹性体的固化颗粒和具有至少一个能够与聚酰胺反应和接枝到聚酰胺上的官能团的第二弹性体颗粒，第一和第二弹性体的颗粒分散在连续的热塑性聚酰胺基质所述方法包括：（1）将固化剂分散在卤化弹性体中并形成预混合的，优选颗粒状的组合物; （2）将聚酰胺树脂和任选的稳定剂引入混合器中并剪切和加热以熔化聚酰胺并形成混合物; （3）在混合条件下引入尼龙增塑剂以降低聚酰胺混合物的粘度与预混合弹性体的粘度基本一致; （4）将预混合弹性体的颗粒引入混合器中并引发弹性体和聚酰胺组分的动态硫化; （5）引入第二弹性体并继续加热和剪切以分散第二弹性体并基本上完成动态硫化; 并从混合器输送热塑性弹性体组合物。这样的组合物特别适用于诸如轮胎内衬和阻挡膜或层的应用。

10. 发明申请

WO2008060302A1 LOW PERMEABILITY LAMINATE CONSTRUCTION 审中-公开
标题翻译：低渗透性层压结构
公开(公告)号：WO2008060302A1
公开(公告)日：2008-05-22
申请号：PCT/US2006/061042
申请日：2006-11-17
申请人： EXXONMOBIL CHEMICAL PATENTS INC. , THE YOKOHAMA RUBBER CO., LTD. , TSOU, Andy, Haishung , MEASMER, Matthew, Brian , SOEDA, Yoshihiro
发明人： TSOU, Andy, Haishung , MEASMER, Matthew, Brian , SOEDA, Yoshihiro
IPC分类号： B32B25/08 , B60C1/00 , B60C5/14 , C08L23/16 , C08L23/28 , B32B27/08
CPC分类号： C08L23/283 , B29D2030/0682 , B32B7/02 , B32B25/08 , B60C1/0008 , B60C1/0025 , B60C2005/145 , C08L21/00 , C08L23/0869 , C08L2205/03 , C08L2666/14 , C08L2666/06 , C08L2666/20 , C08L93/00 , C08L67/08 , C08L77/00
摘要： A multi-layered construction particularly useful in pneumatic tires and hoses comprising a fluid permeation prevention layer having upper and lower surfaces; a layer comprising at least one high diene rubber in laminate relation with the fluid permeation prevention layer upper surface; wherein there is present on the lower fluid permeation prevention layer surface at least one thin, substantially continuous surface or layer comprising at least one metal or metal oxide, the metal or metal oxide surface or layer in communication with the fluid; and wherein the fluid permeation prevention layer preferably comprises at least one polyamide resin composition and, preferably, a halogen-containing elastomer, preferably brominated poly(isobutylene-co-paramethylstyrene), wherein the elastomer component is vulcanized and dispersed as a discontinuous phase in a matrix of the polyamide resin composition. A thermoplastic film layer and suitable adhesives optionally can be included between the metal and/or metal oxide containing surface or layer and fluid permeation prevention layer.
摘要翻译：一种在充气轮胎和软管中特别有用的多层结构，包括具有上表面和下表面的防流体渗透层; 包含至少一种与防流液层上表面层压关系的高二烯橡胶的层; 其中在下部流体渗透防止层表面上存在至少一个薄的，基本上连续的表面或层，其包含至少一种金属或金属氧化物，与流体连通的金属或金属氧化物表面或层; 并且其中所述防流体渗透层优选包含至少一种聚酰胺树脂组合物，优选含有含卤弹性体，优选溴化聚（异丁烯 - 共 - 对甲基苯乙烯），其中所述弹性体组分以不连续相硫化和分散在聚酰胺树脂组合物的基体。可以在含金属和/或金属氧化物的表面或层和防止流体渗透层之间包含热塑性薄膜层和适当的粘合剂。

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