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1. 发明授权

US08373013B2 Process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons 有权
标题翻译：用于组合有机含氧化合物的催化转化和烃的催化转化的方法
公开(公告)号：US08373013B2
公开(公告)日：2013-02-12
申请号：US12373586
申请日：2007-07-12
申请人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
发明人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
IPC分类号： C01C1/20
CPC分类号： C10G11/05 , B01J29/084 , B01J29/46 , B01J29/80 , B01J29/90 , B01J35/0006 , C07C1/20 , C07C2521/16 , C07C2529/08 , C07C2529/70 , C07C2529/85 , C10G3/49 , C10G3/55 , C10G3/57 , C10G3/62 , C10G57/00 , C10G2300/1033 , C10G2300/1037 , C10G2300/104 , C10G2300/1055 , C10G2300/1059 , C10G2300/107 , C10G2300/1077 , C10G2300/4018 , C10G2300/701 , C10G2300/708 , Y02P20/584 , C07C11/02
摘要： A process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons: an organic oxygenate feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, and a coked catalyst and a product stream are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, a spent catalyst and a reaction oil vapor are obtained after separating the reaction stream, and the reaction oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with the organic oxygenate feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of the organic oxygenate, thus ensuring the continuous catalytic conversion of the organic oxygenate.
摘要翻译：将有机含氧化合物的催化转化和烃的催化转化与有机含氧化合物原料结合的方法与含Y-沸石的催化剂接触以产生反应流，分离反应后得到结焦催化剂和产物流流; 将烃原料与含Y-沸石的催化剂接触以产生反应物流，分离反应物流后得到废催化剂和反应油蒸气，反应油蒸气进一步分离，得到产物如气体，汽油等; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回以与有机含氧化合物原料接触。该方法不仅合理地利用烃转化的过量热能，还解决了有机含氧化合物转化的供热问题，从而确保有机含氧化合物的连续催化转化。

2. 发明申请

US20090318742A1 PROCESS FOR COMBINING THE CATALYTIC CONVERSION OF ORGANIC OXYGENATES AND THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：组合有机氧化物的催化转化和烃类催化转化的方法
公开(公告)号：US20090318742A1
公开(公告)日：2009-12-24
申请号：US12373586
申请日：2007-07-12
申请人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
发明人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
IPC分类号： C07C11/00
CPC分类号： C10G11/05 , B01J29/084 , B01J29/46 , B01J29/80 , B01J29/90 , B01J35/0006 , C07C1/20 , C07C2521/16 , C07C2529/08 , C07C2529/70 , C07C2529/85 , C10G3/49 , C10G3/55 , C10G3/57 , C10G3/62 , C10G57/00 , C10G2300/1033 , C10G2300/1037 , C10G2300/104 , C10G2300/1055 , C10G2300/1059 , C10G2300/107 , C10G2300/1077 , C10G2300/4018 , C10G2300/701 , C10G2300/708 , Y02P20/584 , C07C11/02
摘要： A process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons: an organic oxygenate feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, and a coked catalyst and a product stream are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, a spent catalyst and a reaction oil vapor are obtained after separating the reaction stream, and the reaction oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with the organic oxygenate feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of the organic oxygenate, thus ensuring the continuous catalytic conversion of the organic oxygenate.
摘要翻译：将有机含氧化合物的催化转化和烃的催化转化与有机含氧化合物原料结合的方法与含Y-沸石的催化剂接触以产生反应流，分离反应后得到结焦催化剂和产物流流; 将烃原料与含Y-沸石的催化剂接触以产生反应物流，分离反应物流后得到废催化剂和反应油蒸气，反应油蒸气进一步分离，得到产物如气体，汽油等; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回以与有机含氧化合物原料接触。该方法不仅合理地利用烃转化的过量热能，还解决了有机含氧化合物转化的供热问题，从而确保有机含氧化合物的连续催化转化。

3. 发明授权

US08273930B2 Process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons 有权
标题翻译：从乙醇生产乙烯的方法，结合烃的催化转化
公开(公告)号：US08273930B2
公开(公告)日：2012-09-25
申请号：US12373585
申请日：2007-07-12
申请人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
发明人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
IPC分类号： C07C1/24
CPC分类号： C10G57/00 , C07C1/24 , C07C2529/08 , C10G11/05 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/04
摘要： A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol % or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol %.
摘要翻译：将乙烯的催化转化合成乙醇的方法：将乙醇原料与含Y-沸石的催化剂接触，得到产物流，分离出反应物流后得到结焦催化剂和乙烯目标产物; 将烃原料与含Y-沸石的催化剂接触，得到产物流，分离反应流后得到废催化剂和油蒸气，并进一步分离出油蒸汽，得到产物如气体，汽油和类似; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回与乙醇原料接触。这个过程不仅合理利用了烃转化的过量热能，而且解决了乙醇转化的供热问题，从而保证了乙醇的连续催化转化，产生了巨大的经济效益。对于乙醇的催化转化，气体产物中乙烯的含量为95体积％以上; 乙烯的转化率不低于99％。对于烃的催化转化，轻质烯烃的产率略微增加至少2摩尔％。

4. 发明申请

US20090281363A1 PROCESS FOR PRODUCING ETHYLENE FROM ETHANOL COMBINING THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：从乙醇与乙醇催化转化合成乙烯的方法
公开(公告)号：US20090281363A1
公开(公告)日：2009-11-12
申请号：US12373585
申请日：2007-07-12
申请人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
发明人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
IPC分类号： C07C1/20
CPC分类号： C10G57/00 , C07C1/24 , C07C2529/08 , C10G11/05 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/04
摘要： A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol % or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol %.
摘要翻译：将乙烯的催化转化合成乙醇的方法：将乙醇原料与含Y-沸石的催化剂接触，得到产物流，分离出反应物流后得到结焦催化剂和乙烯目标产物; 将烃原料与含Y-沸石的催化剂接触，得到产物流，分离反应流后得到废催化剂和油蒸气，并进一步分离出油蒸汽，得到产物如气体，汽油和类似; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回与乙醇原料接触。这个过程不仅合理利用了碳氢化合物转化的过量热能，而且解决了乙醇转化的供热问题，从而确保了乙醇的连续催化转化，产生了巨大的经济效益。对于乙醇的催化转化，气体产物中乙烯的含量为95体积％以上; 乙烯的转化率不低于99％。对于烃的催化转化，轻质烯烃的产率略微增加至少2摩尔％。

5. 发明申请

US20070060468A1 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US20070060468A1
公开(公告)日：2007-03-15
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J29/04
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

6. 发明授权

US07713904B2 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US07713904B2
公开(公告)日：2010-05-11
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J27/195 , B01J29/06
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

7. 发明授权

US08349756B2 Noble metal-containing titanosilicate material and its preparation method 有权
标题翻译：贵金属含钛硅酸盐材料及其制备方法
公开(公告)号：US08349756B2
公开(公告)日：2013-01-08
申请号：US12594008
申请日：2008-03-27
申请人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
发明人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
IPC分类号： B01J29/89
CPC分类号： B01J35/002 , B01J23/38 , B01J23/40 , B01J23/44 , B01J29/89 , B01J35/0046 , B01J35/006 , B01J2229/20 , C07D301/08 , Y02P20/52
摘要： A noble metal-containing titanosilicate material, characterized in that said material is represented with the oxide form of xTiO2.100SiO2.yEOm.zE, wherein x ranges from 0.001 to 50.0; (y+z) ranges from 0.0001 to 20.0 and y/z
摘要翻译：一种含贵金属的钛硅酸盐材料，其特征在于，所述材料用xTiO2.1··O·SiO 2·yO·m·zE的氧化物形式表示，其中x为0.001-50.0; （y + z）为0.0001〜20.0，y / z <5。 E表示选自Ru，Rh，Pd，Re，Os，Ir，Pt，Ag和Au中的一种或多种贵金属; m是满足E的氧化态的数。所述材料的晶粒含有中空结构或下垂结构。在所述材料中，增强了贵金属和钛硅酸盐之间的协同效应。与现有技术相比，在氧化反应中，反应产物的选择性，催化活性和稳定性明显增加。通过丙烯环氧化制备环氧丙烷的反应。

8. 发明申请

US20100105542A1 NOBLE METAL-CONTAINING TITANOSILICATE MATERIAL AND ITS PREPARATION METHOD 有权
标题翻译：含金属的钛酸盐材料及其制备方法
公开(公告)号：US20100105542A1
公开(公告)日：2010-04-29
申请号：US12594008
申请日：2008-03-27
申请人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
发明人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
IPC分类号： B01J29/068
CPC分类号： B01J35/002 , B01J23/38 , B01J23/40 , B01J23/44 , B01J29/89 , B01J35/0046 , B01J35/006 , B01J2229/20 , C07D301/08 , Y02P20/52
摘要： A noble metal-containing titanosilicate material, characterized in that said material is represented with the oxide form of xTiO2.100SiO2.yEOm.zE, wherein x ranges from 0.001 to 50.0; (y+z) ranges from 0.0001 to 20.0 and y/z
摘要翻译：一种含贵金属的钛硅酸盐材料，其特征在于，所述材料用xTiO2.1··O·SiO 2·yO·m·zE的氧化物形式表示，其中x为0.001-50.0; （y + z）为0.0001〜20.0，y / z <5。 E表示选自Ru，Rh，Pd，Re，Os，Ir，Pt，Ag和Au中的一种或多种贵金属; m是满足E的氧化态的数。所述材料的晶粒含有中空结构或下垂结构。在所述材料中，增强了贵金属和钛硅酸盐之间的协同效应。与现有技术相比，在氧化反应中，反应产物的选择性，催化活性和稳定性明显增加。通过丙烯环氧化制备环氧丙烷的反应。

9. 发明申请

US20120115966A1 Process for Preparing Methanol, Dimethyl Ether, and Low Carbon Olefins from Syngas 有权
标题翻译：从合成气中制备甲醇，二甲醚和低碳烯烃的方法
公开(公告)号：US20120115966A1
公开(公告)日：2012-05-10
申请号：US13131028
申请日：2009-11-26
申请人： Qiang Fu , Xiaoxin Zhang , Yibin Luo , Xuhong Mu , Baoning Zong
发明人： Qiang Fu , Xiaoxin Zhang , Yibin Luo , Xuhong Mu , Baoning Zong
IPC分类号： C07C27/06
CPC分类号： C07C41/01 , B01J23/78 , B01J23/80 , B01J23/825 , B01J23/835 , B01J23/8472 , B01J23/868 , B01J23/8892 , B01J25/00 , B01J29/46 , B01J35/002 , B01J37/0009 , B01J37/03 , B01J37/06 , C07C1/043 , C07C29/154 , C07C2521/02 , C07C2521/04 , C07C2521/06 , C07C2523/02 , C07C2523/06 , C07C2523/10 , C07C2523/22 , C07C2523/26 , C07C2523/34 , C07C2523/72 , C07C2523/745 , C07C2523/755 , C07C2529/40 , C07C2529/85 , Y02P20/52 , C07C31/04 , C07C43/043 , C07C11/04 , C07C11/06
摘要： The present invention provides a process for preparing methanol, dimethyl ether, and low carbon olefins from syngas, wherein the process comprises the step of contacting syngas with a catalyst under the conditions for converting the syngas into methanol, dimethyl ether, and low carbon olefins, characterized in that, the catalyst contains an amorphous alloy consisting of a first component Al and a second component, said second component being one or more elements or oxides thereof selected from Group IA, IIIA, IVA, VA, IB, IIB, IVB, VB, VIIB, VIIB, VIII, and Lanthanide series of the Periodic Table of Elements, and said second component being different from the first component Al. According to the present process, the syngas can be converted into methanol, dimethyl ether, and low carbon olefins in a high CO conversion, a high selectivity of the target product, and high carbon availability.
摘要翻译：本发明提供从合成气制备甲醇，二甲醚和低碳烯烃的方法，其中该方法包括在合成气转化为甲醇，二甲醚和低碳烯烃的条件下使合成气与催化剂接触的步骤，其特征在于，所述催化剂含有由第一成分Al和第二成分组成的非晶合金，所述第二成分为选自IA，IIIA，IVA，VA，IB，IIB，IVB，VB中的一种或多种元素或氧化物，VIIB，VIIB，VIII和元素周期表的镧系元素，所述第二成分与第一成分Al不同。根据本方法，合成气可以在高CO转化率，目标产物的高选择性和高碳可利用性下转化为甲醇，二甲醚和低碳烯烃。

10. 发明申请

US20120083539A1 Process for Preparing Methanol, Dimethyl Ether, and Low Carbon Olefins from Syngas 有权
标题翻译：从合成气中制备甲醇，二甲醚和低碳烯烃的方法
公开(公告)号：US20120083539A1
公开(公告)日：2012-04-05
申请号：US13139513
申请日：2009-12-15
申请人： Qiang Fu , Xiaoxin Zhang , Yibin Luo , Xuhong Mu , Baoning Zong
发明人： Qiang Fu , Xiaoxin Zhang , Yibin Luo , Xuhong Mu , Baoning Zong
IPC分类号： C07C27/06
CPC分类号： C07C41/01 , C07C1/043 , C07C29/153 , C07C2521/06 , C07C2523/14 , C07C2523/22 , C07C2523/26 , C07C2523/34 , C07C2523/745 , C07C2523/75 , C07C2523/755 , C07C2523/83 , Y02P20/52 , C07C11/02 , C07C31/04 , C07C43/043
摘要： The present invention provides a process for preparing methanol, dimethyl ether, and low carbon olefins from syngas, wherein the process comprises the step of contacting syngas with a catalyst under the conditions for converting the syngas into methanol, dimethyl ether, and low carbon olefins, characterized in that, the catalyst contains an amorphous alloy consisting of components M and X wherein the component X represents an element B and/or P, the component M represents two or more elements selected from Group IIIA, IVA, VA, IB, IIB, IVB, VB, VIB, VIIB, VIII and Lanthanide series of the Periodic Table of Elements. According to the present process, the syngas can be converted into methanol, dimethyl ether, and low carbon olefins in a high CO conversion, a high selectivity of the target product, and high carbon availability.
摘要翻译：本发明提供从合成气制备甲醇，二甲醚和低碳烯烃的方法，其中该方法包括在合成气转化为甲醇，二甲醚和低碳烯烃的条件下使合成气与催化剂接触的步骤，其特征在于，催化剂含有由成分M和X组成的非晶合金，其中成分X表示元素B和/或P，成分M表示选自IIIA，IVA，VA，IB，IIB， IVB，VB，VIB，VIIB，VIII和元素周期表的镧系元素。根据本方法，合成气可以在高CO转化率，目标产物的高选择性和高碳可利用性下转化为甲醇，二甲醚和低碳烯烃。

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