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1. 发明授权

US08373013B2 Process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons 有权
标题翻译：用于组合有机含氧化合物的催化转化和烃的催化转化的方法
公开(公告)号：US08373013B2
公开(公告)日：2013-02-12
申请号：US12373586
申请日：2007-07-12
申请人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
发明人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
IPC分类号： C01C1/20
CPC分类号： C10G11/05 , B01J29/084 , B01J29/46 , B01J29/80 , B01J29/90 , B01J35/0006 , C07C1/20 , C07C2521/16 , C07C2529/08 , C07C2529/70 , C07C2529/85 , C10G3/49 , C10G3/55 , C10G3/57 , C10G3/62 , C10G57/00 , C10G2300/1033 , C10G2300/1037 , C10G2300/104 , C10G2300/1055 , C10G2300/1059 , C10G2300/107 , C10G2300/1077 , C10G2300/4018 , C10G2300/701 , C10G2300/708 , Y02P20/584 , C07C11/02
摘要： A process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons: an organic oxygenate feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, and a coked catalyst and a product stream are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, a spent catalyst and a reaction oil vapor are obtained after separating the reaction stream, and the reaction oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with the organic oxygenate feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of the organic oxygenate, thus ensuring the continuous catalytic conversion of the organic oxygenate.
摘要翻译：将有机含氧化合物的催化转化和烃的催化转化与有机含氧化合物原料结合的方法与含Y-沸石的催化剂接触以产生反应流，分离反应后得到结焦催化剂和产物流流; 将烃原料与含Y-沸石的催化剂接触以产生反应物流，分离反应物流后得到废催化剂和反应油蒸气，反应油蒸气进一步分离，得到产物如气体，汽油等; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回以与有机含氧化合物原料接触。该方法不仅合理地利用烃转化的过量热能，还解决了有机含氧化合物转化的供热问题，从而确保有机含氧化合物的连续催化转化。

2. 发明申请

US20090318742A1 PROCESS FOR COMBINING THE CATALYTIC CONVERSION OF ORGANIC OXYGENATES AND THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：组合有机氧化物的催化转化和烃类催化转化的方法
公开(公告)号：US20090318742A1
公开(公告)日：2009-12-24
申请号：US12373586
申请日：2007-07-12
申请人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
发明人： Wenhua Xie , Genquan Zhu , Qiang Fu , Zhiguo Wu , Shaobing Yu , Yihua Yang , Qiang Liu , Zhiqiang Qiao , Xuhong Mu , Chaogang Xie , Yibin Luo , Jiushun Zhang , Xingtian Shu
IPC分类号： C07C11/00
CPC分类号： C10G11/05 , B01J29/084 , B01J29/46 , B01J29/80 , B01J29/90 , B01J35/0006 , C07C1/20 , C07C2521/16 , C07C2529/08 , C07C2529/70 , C07C2529/85 , C10G3/49 , C10G3/55 , C10G3/57 , C10G3/62 , C10G57/00 , C10G2300/1033 , C10G2300/1037 , C10G2300/104 , C10G2300/1055 , C10G2300/1059 , C10G2300/107 , C10G2300/1077 , C10G2300/4018 , C10G2300/701 , C10G2300/708 , Y02P20/584 , C07C11/02
摘要： A process for combining the catalytic conversion of organic oxygenates and the catalytic conversion of hydrocarbons: an organic oxygenate feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, and a coked catalyst and a product stream are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to produce a reaction stream, a spent catalyst and a reaction oil vapor are obtained after separating the reaction stream, and the reaction oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with the organic oxygenate feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of the organic oxygenate, thus ensuring the continuous catalytic conversion of the organic oxygenate.
摘要翻译：将有机含氧化合物的催化转化和烃的催化转化与有机含氧化合物原料结合的方法与含Y-沸石的催化剂接触以产生反应流，分离反应后得到结焦催化剂和产物流流; 将烃原料与含Y-沸石的催化剂接触以产生反应物流，分离反应物流后得到废催化剂和反应油蒸气，反应油蒸气进一步分离，得到产物如气体，汽油等; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回以与有机含氧化合物原料接触。该方法不仅合理地利用烃转化的过量热能，还解决了有机含氧化合物转化的供热问题，从而确保有机含氧化合物的连续催化转化。

3. 发明授权

US08273930B2 Process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons 有权
标题翻译：从乙醇生产乙烯的方法，结合烃的催化转化
公开(公告)号：US08273930B2
公开(公告)日：2012-09-25
申请号：US12373585
申请日：2007-07-12
申请人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
发明人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
IPC分类号： C07C1/24
CPC分类号： C10G57/00 , C07C1/24 , C07C2529/08 , C10G11/05 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/04
摘要： A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol % or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol %.
摘要翻译：将乙烯的催化转化合成乙醇的方法：将乙醇原料与含Y-沸石的催化剂接触，得到产物流，分离出反应物流后得到结焦催化剂和乙烯目标产物; 将烃原料与含Y-沸石的催化剂接触，得到产物流，分离反应流后得到废催化剂和油蒸气，并进一步分离出油蒸汽，得到产物如气体，汽油和类似; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回与乙醇原料接触。这个过程不仅合理利用了烃转化的过量热能，而且解决了乙醇转化的供热问题，从而保证了乙醇的连续催化转化，产生了巨大的经济效益。对于乙醇的催化转化，气体产物中乙烯的含量为95体积％以上; 乙烯的转化率不低于99％。对于烃的催化转化，轻质烯烃的产率略微增加至少2摩尔％。

4. 发明申请

US20090281363A1 PROCESS FOR PRODUCING ETHYLENE FROM ETHANOL COMBINING THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：从乙醇与乙醇催化转化合成乙烯的方法
公开(公告)号：US20090281363A1
公开(公告)日：2009-11-12
申请号：US12373585
申请日：2007-07-12
申请人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
发明人： Zhiguo Wu , Wenhua Xie , Chaogang Xie , Qiang Liu , Xuhong Mu , Jiushun Zhang , Yibin Luo , Xingtian Shu , Chenghan Yan
IPC分类号： C07C1/20
CPC分类号： C10G57/00 , C07C1/24 , C07C2529/08 , C10G11/05 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2400/20 , Y02P20/52 , Y02P20/584 , C07C11/04
摘要： A process for producing ethylene from ethanol combining the catalytic conversion of hydrocarbons: an ethanol feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, and a coked catalyst and an target product of ethylene are obtained after separating the reaction stream; a hydrocarbon feedstock is contacted with a Y-zeolite containing catalyst to give a product stream, a spent catalyst and an oil vapor are obtained after separating the reaction stream, and the oil vapor is further separated to give the products such as gas, gasoline and the like; a part or all of the coked catalyst and a part or all of the spent catalyst enter the regenerator for the coke-burning regeneration, and the regenerated catalyst is divided into two portions, wherein one portion returns to be contacted with the hydrocarbon feedstock, and the other portion, after cooling, returns to be contacted with ethanol feedstock. This process not only reasonably utilizes the excessive thermal energy of the hydrocarbon conversion, but also solves the problem of heat supply for the conversion of ethanol, thus ensuring the continuous catalytic conversion of ethanol and generating enormous economic benefits. For the catalytic conversion of the ethanol, the content of ethylene is 95 vol % or more in the gas product; and the conversion of ethylene is not less than 99%. For the catalytic conversion of the hydrocarbons, the yield for the light olefins increases slightly by at least 2 mol %.
摘要翻译：将乙烯的催化转化合成乙醇的方法：将乙醇原料与含Y-沸石的催化剂接触，得到产物流，分离出反应物流后得到结焦催化剂和乙烯目标产物; 将烃原料与含Y-沸石的催化剂接触，得到产物流，分离反应流后得到废催化剂和油蒸气，并进一步分离出油蒸汽，得到产物如气体，汽油和类似; 一部分或全部的焦化催化剂和一部分或全部废废催化剂进入再生器进行焦炭燃烧再生，再生催化剂分成两部分，其中一部分返回以与烃原料接触，和冷却后的另一部分返回与乙醇原料接触。这个过程不仅合理利用了碳氢化合物转化的过量热能，而且解决了乙醇转化的供热问题，从而确保了乙醇的连续催化转化，产生了巨大的经济效益。对于乙醇的催化转化，气体产物中乙烯的含量为95体积％以上; 乙烯的转化率不低于99％。对于烃的催化转化，轻质烯烃的产率略微增加至少2摩尔％。

5. 发明授权

US08900445B2 Process for the catalytic conversion of hydrocarbons 有权
标题翻译：碳氢化合物的催化转化方法
公开(公告)号：US08900445B2
公开(公告)日：2014-12-02
申请号：US12439309
申请日：2006-09-28
申请人： Chaogang Xie , Genquan Zhu , Yihua Yang , Yibin Luo , Jun Long , Xingtian Shu , Jiushun Zhang
发明人： Chaogang Xie , Genquan Zhu , Yihua Yang , Yibin Luo , Jun Long , Xingtian Shu , Jiushun Zhang
IPC分类号： C10G11/02 , B01J29/80 , B01J29/76 , B01J29/78 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18 , B01J29/40 , B01J29/60 , B01J29/70 , B01J37/00
CPC分类号： B01J29/80 , B01J29/084 , B01J29/18 , B01J29/40 , B01J29/60 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2300/4093 , C10G2300/807 , C10G2400/02 , C10G2400/04 , C10G2400/20
摘要： A process for the catalytic conversion of hydrocarbons to convert petroleum hydrocarbons in a higher yield for light olefins, particularly propylene is disclosed, the process involving a hydrocarbon-converting catalyst comprising zeolite, phosphorous and a transition metal, as defined herein.
摘要翻译：公开了一种用于轻质烯烃，特别是丙烯，以较高产率转化石油烃的方法，该方法涉及包含如本文所定义的沸石，磷和过渡金属的烃转化催化剂。

6. 发明申请

US20090264693A1 PROCESS FOR THE CATALYTIC CONVERSION OF HYDROCARBONS 有权
标题翻译：烃类催化转化方法
公开(公告)号：US20090264693A1
公开(公告)日：2009-10-22
申请号：US12439309
申请日：2006-09-28
申请人： Chaogang Xie , Genquan Zhu , Yihua Yang , Yibin Luo , Jun Long , Xingtian Shu , Jiushun Zhang
发明人： Chaogang Xie , Genquan Zhu , Yihua Yang , Yibin Luo , Jun Long , Xingtian Shu , Jiushun Zhang
IPC分类号： C07C4/06
CPC分类号： B01J29/80 , B01J29/084 , B01J29/18 , B01J29/40 , B01J29/60 , B01J29/7057 , B01J29/7615 , B01J29/7815 , B01J37/0045 , B01J2229/18 , B01J2229/42 , C10G11/02 , C10G11/05 , C10G11/14 , C10G11/16 , C10G11/18 , C10G2300/1033 , C10G2300/104 , C10G2300/1044 , C10G2300/1055 , C10G2300/107 , C10G2300/1074 , C10G2300/1077 , C10G2300/4018 , C10G2300/4093 , C10G2300/807 , C10G2400/02 , C10G2400/04 , C10G2400/20
摘要： A process for the catalytic conversion of hydrocarbons, said process comprising the following steps: a feedstock of hydrocarbons is contacted with a hydrocarbon-converting catalyst to conduct a catalytic cracking reaction in a reactor, then the reaction products are taken from said reactor and fractionated to give light olefins, gasoline, diesel, heavy oil and other saturated hydrocarbons with low molecular weight, wherein said hydrocarbon-converting catalyst comprises, based on the total weight of the catalyst, 1-60 wt % of a zeolite mixture, 5-99 wt % of a thermotolerant inorganic oxide and 0-70 wt % of clay, wherein said zeolite mixture comprises, based on the total weight of said zeolite mixture, 1-75 wt % of a zeolite beta modified with phosphorus and a transition metal M, 25-99 wt % of a zeolite having a MFI structure and 0-74 wt % of a large pore zeolite, wherein the anhydrous chemical formula of the zeolite beta modified with phosphorus and the transition metal M is represented in the mass percent of the oxides as (0-0.3)Na2O.(0.5-10)Al2O3.(1.3-10)P2O5.(0.7-15)MxOy.(64-97)SiO2, in which the transition metal M is one or more selected from the group consisting of Fe, Co, Ni, Cu, Mn, Zn and Sn; x represents the atom number of the transition metal M, and y represents a number needed for satisfying the oxidation state of the transition metal M. The process of the present invention has a higher ability to convert petroleum hydrocarbon in a higher yield for light olefins, particularly for propylene.
摘要翻译：一种用于烃的催化转化的方法，所述方法包括以下步骤：烃的原料与烃转化催化剂接触以在反应器中进行催化裂化反应，然后将反应产物从所述反应器中取出并分馏成给出轻质烯烃，汽油，柴油，重油和其他具有低分子量的饱和烃，其中所述烃转化催化剂基于催化剂的总重量包含1-60重量％的沸石混合物，5-99重量％％的耐热无机氧化物和0-70重量％的粘土，其中所述沸石混合物基于所述沸石混合物的总重量包含1-75重量％的用磷和过渡金属M，25 -99重量％的具有MFI结构的沸石和0-74重量％的大孔沸石，其中表示用磷和过渡金属M改性的沸石β的无水化学式被表示氧化物的质量百分比为（0-0.3）Na2O。（0.5-10）Al2O3。（1.3-10）P2O5。（0.7-15）MxOy。（64-97）SiO2，其中过渡金属M为选自Fe，Co，Ni，Cu，Mn，Zn和Sn中的一种或多种; x表示过渡金属M的原子数，y表示满足过渡金属M的氧化态所需的数。本发明的方法具有较高的轻质烯烃转化石油烃的能力，特别是对于丙烯。

7. 发明授权

US07713904B2 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US07713904B2
公开(公告)日：2010-05-11
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J27/195 , B01J29/06
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

8. 发明申请

US20070060468A1 Composition for desulfurization 有权
标题翻译：脱硫组成
公开(公告)号：US20070060468A1
公开(公告)日：2007-03-15
申请号：US10562965
申请日：2004-06-24
申请人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
发明人： Baoning Zong , Jinyu Zheng , Wenhua Xie , Yong Xu , Xuhong Mu , Yibin Luo , Minggang Li , Xingtian Shu
IPC分类号： B01J29/04
CPC分类号： B01J29/84 , B01J29/084 , B01J29/088 , B01J29/40 , B01J29/405 , B01J29/80 , B01J2229/42 , C10G45/12 , C10G47/20
摘要： This invention relates to a composition with desulfurization property, in which the desulfurization component is a kind of molecular sieves with incorporation of vanadium into the skeleton. The composition has high hydrothermal stability and the vanadium is hard to lose.
摘要翻译：本发明涉及具有脱硫性质的组合物，其中脱硫组分是一种将钒掺入骨架中的分子筛。该组合物具有很高的水热稳定性，钒难以失去。

9. 发明授权

US08349756B2 Noble metal-containing titanosilicate material and its preparation method 有权
标题翻译：贵金属含钛硅酸盐材料及其制备方法
公开(公告)号：US08349756B2
公开(公告)日：2013-01-08
申请号：US12594008
申请日：2008-03-27
申请人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
发明人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
IPC分类号： B01J29/89
CPC分类号： B01J35/002 , B01J23/38 , B01J23/40 , B01J23/44 , B01J29/89 , B01J35/0046 , B01J35/006 , B01J2229/20 , C07D301/08 , Y02P20/52
摘要： A noble metal-containing titanosilicate material, characterized in that said material is represented with the oxide form of xTiO2.100SiO2.yEOm.zE, wherein x ranges from 0.001 to 50.0; (y+z) ranges from 0.0001 to 20.0 and y/z
摘要翻译：一种含贵金属的钛硅酸盐材料，其特征在于，所述材料用xTiO2.1··O·SiO 2·yO·m·zE的氧化物形式表示，其中x为0.001-50.0; （y + z）为0.0001〜20.0，y / z <5。 E表示选自Ru，Rh，Pd，Re，Os，Ir，Pt，Ag和Au中的一种或多种贵金属; m是满足E的氧化态的数。所述材料的晶粒含有中空结构或下垂结构。在所述材料中，增强了贵金属和钛硅酸盐之间的协同效应。与现有技术相比，在氧化反应中，反应产物的选择性，催化活性和稳定性明显增加。通过丙烯环氧化制备环氧丙烷的反应。

10. 发明申请

US20100105542A1 NOBLE METAL-CONTAINING TITANOSILICATE MATERIAL AND ITS PREPARATION METHOD 有权
标题翻译：含金属的钛酸盐材料及其制备方法
公开(公告)号：US20100105542A1
公开(公告)日：2010-04-29
申请号：US12594008
申请日：2008-03-27
申请人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
发明人： Min Lin , Chunfeng Shi , Jun Long , Bin Zhu , Xingtian Shu , Xuhong Mu , Yibin Luo , Xieqing Wang , Yingchun Ru
IPC分类号： B01J29/068
CPC分类号： B01J35/002 , B01J23/38 , B01J23/40 , B01J23/44 , B01J29/89 , B01J35/0046 , B01J35/006 , B01J2229/20 , C07D301/08 , Y02P20/52
摘要： A noble metal-containing titanosilicate material, characterized in that said material is represented with the oxide form of xTiO2.100SiO2.yEOm.zE, wherein x ranges from 0.001 to 50.0; (y+z) ranges from 0.0001 to 20.0 and y/z
摘要翻译：一种含贵金属的钛硅酸盐材料，其特征在于，所述材料用xTiO2.1··O·SiO 2·yO·m·zE的氧化物形式表示，其中x为0.001-50.0; （y + z）为0.0001〜20.0，y / z <5。 E表示选自Ru，Rh，Pd，Re，Os，Ir，Pt，Ag和Au中的一种或多种贵金属; m是满足E的氧化态的数。所述材料的晶粒含有中空结构或下垂结构。在所述材料中，增强了贵金属和钛硅酸盐之间的协同效应。与现有技术相比，在氧化反应中，反应产物的选择性，催化活性和稳定性明显增加。通过丙烯环氧化制备环氧丙烷的反应。

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