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1. 发明公开

US20240208811A1 PROCESS FOR SYNTHESIS OF SYNGAS COMPONENTS 审中-公开
公开(公告)号：US20240208811A1
公开(公告)日：2024-06-27
申请号：US18550752
申请日：2022-03-16
申请人： Kansas State University Research Foundation , Hydrograph Clean Power Inc.
发明人： Christopher M. Sorensen , Stefan H. Bossmann , Justin Wright , Shusil Sigdel , Jose Covarrubias , Arjun Nepal , Harold Charles Davidson
IPC分类号： C01B3/36
CPC分类号： C01B3/36 , C01B2203/0255 , C01B2203/0405 , C01B2203/1217 , C01B2203/1235 , C01B2203/1276 , C01B2203/1614 , C01B2203/169
摘要： Apparatus and processes for high-yield production of syngas components via combustion of a carbon-containing material and an oxygen-containing material are provided. Syngas components are generated in an exothermic, combustion reaction with only minor quantities of carbon dioxide, water, and elemental carbon produced.

2. 发明授权

US09527044B2 Proton conducting membranes for hydrogen production and separation 有权
标题翻译：用于氢气生产和分离的质子导电膜
公开(公告)号：US09527044B2
公开(公告)日：2016-12-27
申请号：US14502303
申请日：2014-09-30
申请人： UNIVERSITY OF FLORIDA RESEARCH FOUNDATION, INC.
发明人： Eric D. Wachsman , Hee Sung Yoon , Takkeun Oh , Jianlin Li
IPC分类号： B01J19/02 , C01B3/02 , C01B3/34 , B01D71/02 , B01D67/00 , B01J19/24 , C01B3/50 , C04B38/00 , C04B41/50
CPC分类号： B01D71/024 , B01D67/0046 , B01D2323/20 , B01D2325/00 , B01J19/02 , B01J19/2485 , B01J2219/00135 , B01J2219/0254 , C01B3/02 , C01B3/34 , C01B3/503 , C01B3/505 , C01B2203/0283 , C01B2203/0405 , C01B2203/041 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0495 , C01B2203/1205 , C01B2203/1217 , C01B2203/1235 , C01B2203/86 , C04B38/0038 , C04B41/5027 , Y02P30/30 , Y10T428/24997 , C04B35/48
摘要： In one embodiment, a membrane of proton-electron conducting ceramics that is useful for the conversion of a hydrocarbon and steam to hydrogen has a porous support coated with a film of a Perovskite-type oxide. By including the Zr and M in the oxide in place of Ce, the stability can be improved while maintaining sufficient hydrogen flux for efficient generation of hydrogen. In this manner, the conversion can be carried out by performing steam methane reforming (SMR) and/or water-gas shift reactions (WGS) at high temperature, where the conversion of CO to CO2 and H2 is driven by the removal of H2 to give high conversions.
摘要翻译：在一个实施方案中，用于将烃和蒸汽转化为氢的质子 - 电子传导陶瓷膜具有涂覆有钙钛矿型氧化物膜的多孔载体。通过将Zr和M包含在氧化物中代替Ce，可以在保持足够的氢通量以有效产生氢的同时提高稳定性。以这种方式，可以通过在高温下进行蒸汽甲烷重整（SMR）和/或水煤气变换反应（WGS）来进行转化，其中通过除去H 2来驱动CO向CO 2和H 2的转化提供高转化率。

3. 发明授权

US09496565B2 Architectures for electrochemical systems 有权
标题翻译：电化学系统的结构
公开(公告)号：US09496565B2
公开(公告)日：2016-11-15
申请号：US12526008
申请日：2008-02-06
申请人： Reinder J. Boersma , Scott C. Rackey , Jack A. Shindle
发明人： Reinder J. Boersma , Scott C. Rackey , Jack A. Shindle
IPC分类号： H01M8/06 , C25B1/02 , B01J8/00 , C01B3/02 , H01M8/04 , C01B3/34 , C01B3/36 , C01B3/38 , C10J3/00
CPC分类号： H01M8/04014 , C01B3/34 , C01B3/36 , C01B3/382 , C01B2203/0233 , C01B2203/025 , C01B2203/0283 , C01B2203/04 , C01B2203/06 , C01B2203/0883 , C01B2203/1217 , C01B2203/1235 , C01B2203/142 , C01B2203/84 , C10J3/00 , C10J2300/1646 , C10J2300/1684 , H01M8/04089 , H01M8/04119 , H01M8/04291 , H01M8/0612 , H01M8/0618 , H01M8/0631 , H01M8/0656 , H01M8/0662 , H01M8/0668 , Y02E60/364 , Y02E60/50
摘要： The present invention generally relates to electrochemical systems for producing hydrogen and/or power. Various aspects of the invention are directed to reactor designs for producing hydrogen and/or power from a fuel and water, conducting ceramics and other materials for such systems, including mixed ionically and electrically conducting ceramics which can be used for hydrogen gas generation, control systems for such systems, and methods of operating such systems.
摘要翻译：本发明一般涉及用于产生氢和/或电力的电化学系统。本发明的各个方面涉及从燃料和水生产氢和/或电力的反应器设计，用于这种系统的导电陶瓷和其它材料，包括可用于氢气产生的混合离子和导电陶瓷，控制系统对于这样的系统，以及操作这种系统的方法。

4. 发明申请

US20160297844A1 DEHYDROGENATION CATALYST, AND CARBONYL COMPOUND AND HYDROGEN PRODUCTION METHOD USING SAID CATALYST 有权
标题翻译：脱氢催化剂和碳化合物和使用催化剂的氢生产方法
公开(公告)号：US20160297844A1
公开(公告)日：2016-10-13
申请号：US15183490
申请日：2016-06-15
申请人： Kanto Kagaku Kabushiki Kaisha
发明人： Ryohei Yamaguchi , Ken-ichi Fujita
IPC分类号： C07F17/02 , C07C45/00 , C07C201/12 , B01J7/02 , C07C51/16 , C07B41/06 , C07B41/08 , C01B3/32 , B01J31/22 , C07J13/00
CPC分类号： C07F17/02 , B01J7/02 , B01J31/2295 , B01J2231/763 , B01J2231/766 , B01J2531/827 , C01B3/0015 , C01B3/06 , C01B3/22 , C01B3/326 , C01B2203/02 , C01B2203/0227 , C01B2203/0277 , C01B2203/1041 , C01B2203/1064 , C01B2203/1205 , C01B2203/1211 , C01B2203/1217 , C01B2203/1223 , C01B2203/1229 , C07B41/06 , C07B41/08 , C07C45/002 , C07C51/16 , C07C201/12 , C07C2601/08 , C07C2601/14 , C07J13/007 , Y02E60/328 , Y02E60/36 , Y02P20/132 , C07C47/02 , C07C47/06 , C07C47/32 , C07C47/52 , C07C49/04 , C07C49/213 , C07C49/395 , C07C49/403
摘要： Objects of the present invention are to provide a novel dehydrogenation reaction catalyst, to provide a method that can produce a ketone, an aldehyde, and a carboxylic acid with high efficiency from an alcohol, and to provide a method for efficiently producing hydrogen from an alcohol, formic acid, or a formate, and they are accomplished by a catalyst containing an organometallic compound of Formula (1).

5. 发明申请

US20160244555A1 PROCESS FOR PRODUCING A STREAM COMPRISING ETHYLENE GLYCOL 审中-公开
标题翻译：生产包含乙烯甘油的流程的方法
公开(公告)号：US20160244555A1
公开(公告)日：2016-08-25
申请号：US15025980
申请日：2014-10-16
申请人： BIOCHEMTEX S.P.A.
发明人： Marco BERNARDI , Daniela TODARO , Chiara DORATI
IPC分类号： C08G63/183 , B01J21/18 , B01J21/04 , C01B3/32 , B01J23/42 , B01J23/46 , B01J23/755
CPC分类号： C08G63/183 , B01J21/04 , B01J21/18 , B01J23/42 , B01J23/462 , B01J23/755 , C01B3/323 , C01B3/326 , C01B2203/0233 , C01B2203/06 , C01B2203/065 , C01B2203/1217 , C07C29/00 , C07C29/132 , C07C29/60 , Y02P20/145 , Y02P20/52 , C07C31/18 , C07C31/202 , C07C31/205 , C07C31/225
摘要： It is disclosed a process for producing a low boiling mixture comprising ethylene glycol and propylene glycol from a liquid sugar stream derived from a ligno-cellulosic biomass feedstock. The liquid sugar stream is catalytically converted in the presence of hydrogen to a mixture, which is separated into at least a high boiling mixture, comprising glycerol, and the low boiling mixture. The high boiling mixture is converted to hydrogen by reforming and the reforming hydrogen is used in the catalytical steps. Preferably, all the hydrogen used in the conversion process is generated by aqueous phase reforming of the high boiling polyols mixture.
摘要翻译：公开了一种从源自木质纤维素生物质原料的液体糖流中生产包含乙二醇和丙二醇的低沸点混合物的方法。将液体糖流在氢存在下催化转化成混合物，将其分离成至少包含甘油的高沸点混合物和低沸点混合物。通过重整将高沸点混合物转化为氢，并且在催化步骤中使用重整氢。优选地，转化过程中使用的所有氢通过高沸点多元醇混合物的水相重整产生。

6. 发明授权

US09314771B2 Use of lanthanide oxides to reduce sintering of catalysts 有权
标题翻译：使用镧系元素氧化物来减少催化剂的烧结
公开(公告)号：US09314771B2
公开(公告)日：2016-04-19
申请号：US14312105
申请日：2014-06-23
申请人： SABIC Global Technologies B.V.
发明人： Lawrence D'Souza , Vinu Viswanath
IPC分类号： C01B3/38 , C07C1/02 , B01J23/00 , B01J23/02 , B01J23/08 , B01J23/10 , B01J23/40 , B01J23/42 , B01J23/44 , B01J23/56 , B01J23/58 , B01J23/60 , B01J23/70 , B01J23/72 , B01J23/74 , B01J21/00 , B01J21/04 , B01J21/16 , B01J23/63 , C01B3/26 , B01J37/02 , B01J23/83 , B01J35/00 , C01B3/32
CPC分类号： B01J33/00 , B01J21/04 , B01J21/16 , B01J23/005 , B01J23/02 , B01J23/10 , B01J23/42 , B01J23/63 , B01J23/83 , B01J35/0046 , B01J35/006 , B01J37/0242 , B01J37/0244 , C01B3/26 , C01B3/326 , C01B3/382 , C01B3/386 , C01B3/40 , C01B2203/0233 , C01B2203/0238 , C01B2203/0261 , C01B2203/04 , C01B2203/0405 , C01B2203/062 , C01B2203/1041 , C01B2203/107 , C01B2203/1082 , C01B2203/1211 , C01B2203/1217 , C01B2203/1241 , C01B2203/1247 , C01B2203/148 , Y02P20/142 , Y02P20/52
摘要： Disclosed is a lanthanide oxide coated catalyst, and methods for its use, that includes a supported catalyst comprising a support material, a catalytic material, and a lanthanide oxide, wherein the lanthanide oxide is attached to at least a portion of the surface of the supported catalyst.
摘要翻译：公开了一种氧化镧氧化物涂覆的催化剂及其使用方法，其包括载体催化剂，其包含载体材料，催化材料和镧系元素氧化物，其中所述镧系元素氧化物附着至所述载体的氧化物表面的至少一部分催化剂。

7. 发明申请

US20160083251A1 HYDROGEN GENERATION ASSEMBLIES 审中-公开
标题翻译：氢气发电装置
公开(公告)号：US20160083251A1
公开(公告)日：2016-03-24
申请号：US14961529
申请日：2015-12-07
申请人： Element 1 Corp.
发明人： David J. Edlund , Robert Schluter
IPC分类号： C01B3/32
CPC分类号： C01B3/32 , C01B3/501 , C01B2203/0233 , C01B2203/0283 , C01B2203/0405 , C01B2203/043 , C01B2203/044 , C01B2203/0445 , C01B2203/047 , C01B2203/0811 , C01B2203/1217 , C01B2203/1235 , C01B2203/1633 , C01B2203/1647 , C01B2203/169
摘要： Hydrogen generation assemblies and methods of generating hydrogen are disclosed. In some embodiments, the method may include receiving a feed stream in a fuel processing assembly of the hydrogen generation assembly; and generating a product hydrogen stream in the fuel processing assembly from the received feed stream. Generating a product hydrogen stream may, in some embodiments, include generating an output stream in a hydrogen generating region from the received feed stream, and generating the product hydrogen stream in a purification region from the output stream. The method may additionally include receiving the generated product hydrogen stream in a buffer tank of the hydrogen generation assembly; and detecting pressure in the buffer tank via a tank sensor assembly. The method may further include stopping generation of the product hydrogen stream in the fuel processing assembly when the detected pressure in the buffer tank is above a predetermined maximum pressure.
摘要翻译：公开了氢生成组件和产生氢气的方法。在一些实施例中，该方法可包括在氢气产生组件的燃料处理组件中接收进料流; 以及从所接收的进料流在燃料处理组件中产生产物氢气流。在一些实施方案中，产生产物氢气流可以包括在所接收的进料流中在氢气产生区域中产生输出流，以及在来自输出流的净化区域中产生产物氢气流。该方法可以另外包括在氢发生组件的缓冲罐中接收生成的产物氢流; 以及经由油箱传感器组件检测缓冲罐中的压力。该方法可以进一步包括当缓冲罐中的检测压力高于预定最大压力时停止在燃料处理组件中产生产物氢气流。

8. 发明申请

US20160016794A1 METHODS OF PRODUCING HYDROGEN AND SOLID CARBON 有权
标题翻译：生产氢和固体碳的方法
公开(公告)号：US20160016794A1
公开(公告)日：2016-01-21
申请号：US14775946
申请日：2014-03-12
申请人： SEERSTONE LLC
发明人： Dallas B. Noyes
IPC分类号： C01B3/40
CPC分类号： C01B3/40 , C01B3/38 , C01B32/05 , C01B2203/0233 , C01B2203/0435 , C01B2203/047 , C01B2203/0811 , C01B2203/0833 , C01B2203/1047 , C01B2203/1058 , C01B2203/1217 , C01B2203/1241 , C01B2203/1258 , C01B2203/148
摘要： A method for producing hydrogen, includes heating a process feed gas stream, flowing the process feed gas stream into a first reaction zone, flowing the intermediate gas stream into a second reaction zone, removing the solid carbon product from the second reaction zone, removing the tail gas stream from the second reaction zone, and removing hydrogen from the tail gas stream. The process gas stream includes methane and steam. The first reaction zone contains a first catalyst, and at least a portion of the process feed gas stream is converted into an intermediate gas stream in the first reaction zone. The second reaction zone contains a second catalyst, and at least a portion of the intermediate gas stream is converted into a tail gas stream and a solid carbon product in the second reaction zone.
摘要翻译：一种生产氢的方法包括加热工艺原料气流，将工艺进料气流流入第一反应区，将中间气流流入第二反应区，从第二反应区除去固体碳产物，除去来自第二反应区的尾气流，并从尾气流中除去氢。工艺气流包括甲烷和蒸汽。第一反应区含有第一催化剂，并且至少一部分工艺原料气流在第一反应区转化为中间气流。第二反应区含有第二催化剂，并且至少一部分中间气流在第二反应区转化成尾气流和固体碳产物。

9. 发明申请

US20150352528A1 PROCESS FOR PRODUCTION OF HYDROGEN 有权
标题翻译：生产氢过程
公开(公告)号：US20150352528A1
公开(公告)日：2015-12-10
申请号：US14655487
申请日：2014-01-09
申请人： CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE , UNIVERSITE LILLE 1
发明人： Louise DUHAMEL , Wenhao FANG , Sebastien PAUL , Franck DUMEIGNIL
IPC分类号： B01J23/83 , B01J37/14 , C01B3/32 , B01J37/03 , B01J37/00
CPC分类号： B01J23/83 , B01J35/002 , B01J35/023 , B01J35/1014 , B01J35/1019 , B01J37/009 , B01J37/03 , B01J37/14 , B01J37/18 , C01B3/326 , C01B2203/0233 , C01B2203/1058 , C01B2203/1217 , C01B2203/1229 , Y02P20/52
摘要： The present invention relates to a process for production of hydrogen at low temperature starting from alcohols without formation of carbon using an oxyhydride material based on cerium and nickel and to the use of such a material as catalyst for transformation of alcohols to hydrogen.
摘要翻译：本发明涉及一种使用基于铈和镍的氢氧化物材料从醇形成低温生产氢的方法，以及使用这种材料作为用于将醇转化成氢的催化剂的方法。

10. 发明授权

US09073043B2 Hydrogen production catalyst, production method of the same and hydrogen production method 有权
标题翻译：氢气生产催化剂，生产方法相同，氢气生产方法
公开(公告)号：US09073043B2
公开(公告)日：2015-07-07
申请号：US12675716
申请日：2007-11-19
申请人： Katutoshi Nagaoka , Yuusaku Takita , Katutoshi Satou , Hiroyasu Nishiguti
发明人： Katutoshi Nagaoka , Yuusaku Takita , Katutoshi Satou , Hiroyasu Nishiguti
IPC分类号： C01B3/26 , B01J23/63 , B01J23/00 , B01J23/10 , B01J23/83 , C01B3/40 , H01M8/06 , B01J37/02 , B01J37/03
CPC分类号： B01J23/63 , B01J23/002 , B01J23/10 , B01J23/83 , B01J37/0201 , B01J37/031 , B01J2523/00 , C01B3/40 , C01B2203/0238 , C01B2203/0261 , C01B2203/0283 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/107 , C01B2203/1082 , C01B2203/1211 , C01B2203/1217 , C01B2203/1229 , C01B2203/1241 , C01B2203/1247 , C01B2203/1258 , H01M8/0618 , Y02E60/50 , Y02P20/52 , B01J2523/36 , B01J2523/3712 , B01J2523/48
摘要： The drive of direct-heat-supply type reforming of hydrocarbon at ordinary temperature is necessary in order to realize a self-sustaining, on-site reforming type fuel cell system which does not necessitate the supply of energy from the outside. According to the invention, an oxide, CeO2 or Pr6O11, or a Ce/Zr or Ce/Zr/Y double oxide is used as the oxide containing a rare earth element capable of changing the oxidation number with an active metal and oxygen defects are introduced into the oxide or double oxide by activating the oxide or double oxide with a reducing gas at high temperature. When a reaction gas containing hydrocarbon and oxygen is passed though the catalyst at low temperature, the oxygen defects react with oxygen and thereby return to the original oxide. Since this return reaction is an exothermic reaction, the catalyst itself is heated, which acts as the driving force for advancing the combustion of the hydrocarbon, whereby the catalyst layer is further heated and the reforming is advanced to from hydrogen. Thus, the hydrogen-producing reaction can be driven even at low temperature, particularly ordinary temperature.
摘要翻译：为了实现不需要从外部供应能量的自持式现场重整型燃料电池系统，需要在常温下直接进行碳氢化合物的重整的驱动。根据本发明，使用氧化物CeO 2或Pr 6 O 11或Ce / Zr或Ce / Zr / Y双氧化物作为含有能够用活性金属改变氧化数的稀土元素的氧化物，并引入氧缺陷通过在高温下还原气体活化氧化物或双氧化物而进入氧化物或双氧化物。当含有烃和氧的反应气体在低温下通过催化剂时，氧缺陷与氧反应，从而返回到原始氧化物。由于该返回反应是放热反应，所以催化剂本身被加热，其作为促进烃的燃烧的驱动力，由此催化剂层进一步加热并且重整进行到氢。因此，即使在低温，特别是常温也可以驱动制氢反应。

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