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1. 发明申请

US20160060394A1 LOW DIELECTRIC CONSTANT POLYMER CONTAINING DINAPHTHYL AND HEXAFLUOROCYCLOBUTYL ETHER UNIT, PREPARATION METHOD AND USE 有权
标题翻译：含有十六烷基四氢呋喃醚的低介电常数聚合物，制备方法和用途
公开(公告)号：US20160060394A1
公开(公告)日：2016-03-03
申请号：US14785522
申请日：2013-11-20
申请人： SHANGHAI INSTITUTE OF ORGANIC CHEMISTRY, CHINESE ACADEMY OF SCIENCES
发明人： Qiang FANG , Chao YUAN , Kaikai JIN , Yinchun LIU , Shen DIAO , Kai LI
IPC分类号： C08G65/40 , C07C41/30 , C07C41/09 , C07C41/24 , C09D171/12 , C07C43/247
CPC分类号： C08G65/40 , C07C41/09 , C07C41/16 , C07C41/24 , C07C41/30 , C07C43/247 , C07C2601/04 , C08G61/12 , C08G65/007 , C08G65/4025 , C08G65/4075 , C08G65/4093 , C08G2261/146 , C08G2261/344 , C08G2261/43 , C08G2261/65 , C09D171/12 , H01L51/052 , C07C43/225
摘要： The present invention belongs to the field of preparation of high performance polymers, and specifically relates to a low dielectric constant polymer containing dinaphthyl and hexafluorocyclobutyl ether units, and preparation method and use thereof. The polymer is prepared as follows: under the effect of an alkali, 1-naphthol bromotetrafluoroethane ether is prepared from 1-naphthol and tetrafluorodibromoethane in an organic solvent, and then reduced by a zinc powder so as to obtain 1-naphthol trifluorovinyl ether. 1-naphthol trifluorovinyl ether is treated at a high temperature to obtain a bisnaphthol hexafluorocyclobutyl ether monomer. The monomer is subjected to oxidative coupling in the presence of ferric trichloride so as to obtain a thermal polymer containing dinaphthyl and hexafluorocyclobutyl structural units with a good film-forming property, and in a nitrogen atmosphere, the temperature for 5% weight loss (Td5%) of the obtained film is 437° C., and the carbon residue yield at 1000° C. is 54.24%. The dielectric constant (30 MHz) of the film is 2.33. The polymer is suitable for use in the electronic and electrical industries as an insulation coating layer and an encapsulating material for electron components.
摘要翻译：本发明属于高性能聚合物的制备领域，具体涉及含有二萘基和六氟环丁基醚单元的低介电常数聚合物及其制备方法和用途。聚合物制备如下：在碱的作用下，1-萘酚溴四氟乙醚由1-萘酚和四氟二溴乙烷在有机溶剂中制备，然后用锌粉还原，得到1-萘酚三氟乙烯醚。 1-萘酚三氟乙烯醚在高温下处理，得到双萘酚六氟环丁基醚单体。单体在三氯化铁存在下进行氧化偶合，得到含有成膜性能好的二萘基和六氟环丁基结构单元的热聚合物，在氮气气氛中，5％重量损失温度（Td5％）为437℃，1000℃下的碳残渣产率为54.24％。该膜的介电常数（30MHz）为2.33。聚合物适用于电子和电气工业中作为绝缘涂层和用于电子部件的封装材料。

2. 发明申请

US20140335440A1 MOLDED ARTICLE OF POLYMER ELECTROLYTE COMPOSITION AND SOLID POLYMER TYPE FUEL CELL USING SAME 审中-公开
标题翻译：聚合物电解质组合物和固体聚合物型燃料电池的模制品
公开(公告)号：US20140335440A1
公开(公告)日：2014-11-13
申请号：US14346684
申请日：2012-09-20
申请人： TORAY INDUSTRIES, INC.
发明人： Tomoyuki Kunita , Daisuke Izuhara , Yuka Yachi
IPC分类号： H01M8/10
CPC分类号： H01M8/1032 , C08G65/4025 , C08G65/4043 , C08G65/4056 , C08J5/2256 , C08J2371/12 , C08J2481/02 , H01B1/122 , H01M8/1025 , H01M8/1039 , H01M8/1048 , H01M8/1051 , H01M2008/1095 , H01M2300/0082 , Y02P20/582
摘要： [Summary]To provide a formed article of polymer electrolyte composition which exhibits excellent proton conductivity even under low-humidification conditions and under low-temperature conditions, which is excellent in chemical stability, mechanical strength, fuel shutoff properties, and which can achieve high output, high energy density, and excellent long-term durability when used in a polymer electrolyte fuel cell; and also to provide a polymer electrolyte fuel cell using thereof. The formed article of polymer electrolyte composition includes: a block copolymer having one or more of each of a hydrophilic segment (A1) containing an ionic group and a hydrophobic segment (A2) not containing an ionic group; and an additive, wherein the formed article forms co-continuous or lamellar phase separation structure, and the additive is hydrophilic.
摘要翻译： [摘要]提供即使在低加湿条件下和在低温条件下也具有优异的质子传导性的聚合物电解质组合物的成型体，其化学稳定性，机械强度，燃料切断性能优异，可以实现高产出，高能量密度，以及当用于聚合物电解质燃料电池时具有优异的长期耐久性; 并且还提供使用其的聚合物电解质燃料电池。聚合物电解质组合物的成型体包括：含有离子性基团的亲水性链段（A1）和不含离子性基团的疏水性链段（A2）的一个或多个的嵌段共聚物; 和添加剂，其中所形成的制品形成共连续或层状相分离结构，并且添加剂是亲水性的。

3. 发明授权

US08859672B2 Poly(arylene ether)-poly(hydroxy ether) block copolymer and method of making 有权
标题翻译：聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物及其制备方法
公开(公告)号：US08859672B2
公开(公告)日：2014-10-14
申请号：US13169122
申请日：2011-06-27
申请人： Edward Norman Peters
发明人： Edward Norman Peters
IPC分类号： C08G59/04 , C08G59/06 , C08G65/48 , C08K7/14 , C08L71/10 , C08G65/40 , C08G65/38 , C08G65/42 , C08G65/34 , C08L71/12 , C08G65/44
CPC分类号： C08G65/48 , C08G65/34 , C08G65/38 , C08G65/40 , C08G65/4006 , C08G65/4012 , C08G65/4018 , C08G65/4025 , C08G65/4031 , C08G65/4043 , C08G65/4056 , C08G65/4075 , C08G65/42 , C08G65/44 , C08G81/00 , C08G2261/126 , C08G2650/56 , C08K7/14 , C08L71/10 , C08L71/12 , C08L71/123 , C08L71/126 , C08L2205/05 , C08L63/00
摘要： A poly(arylene ether)-poly(hydroxy ether) block copolymer includes at least one poly(hydroxy ether) block and at least one poly(arylene ether) block, and the mole ratio of poly(hydroxy ether) blocks to poly(arylene ether) blocks is 0.95:1 to about 1.00:1. The poly(arylene ether)-poly(hydroxy ether) block copolymer can be prepared by reacting a telechelic poly(arylene ether) having terminal hydroxyl groups with a telechelic poly(hydroxy ether) epoxy resin having terminal epoxy groups, wherein the mole ratio of the telechelic poly(hydroxy ether) to the telechelic poly(arylene ether) is 0.95:1 to 1.00:1. The poly(arylene ether)-poly(hydroxy ether) block copolymer can be shaped into an article by extrusion, thermoforming, or molding, and is a compatibilizing agent for non-polar and polar polymers.
摘要翻译：聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物包括至少一个聚（羟基醚）嵌段和至少一个聚（亚芳基醚）嵌段，以及聚（羟基醚）嵌段与聚（亚芳基）嵌段的摩尔比醚）嵌段为0.95：1至约1.00：1。聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物可以通过使具有末端羟基的遥爪聚（亚芳基醚）与具有末端环氧基的遥爪聚（羟基醚）环氧树脂反应来制备，其中摩尔比遥爪聚（羟基醚）与遥爪聚（亚芳基醚）的比例为0.95:1-1.00:1。聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物可以通过挤出，热成型或模塑成型成制品，并且是非极性和极性聚合物的相容剂。

4. 发明申请

US20120329939A1 POLY(ARYLENE ETHER)-POLY(HYDROXY ETHER) BLOCK COPOLYMER AND METHOD OF MAKING 有权
标题翻译：聚（亚乙基醚） - 聚（羟基醚）嵌段共聚物及其制备方法
公开(公告)号：US20120329939A1
公开(公告)日：2012-12-27
申请号：US13169122
申请日：2011-06-27
申请人： Edward Norman Peters
发明人： Edward Norman Peters
IPC分类号： C08L71/10 , C08K7/14 , C08G65/48
CPC分类号： C08G65/48 , C08G65/34 , C08G65/38 , C08G65/40 , C08G65/4006 , C08G65/4012 , C08G65/4018 , C08G65/4025 , C08G65/4031 , C08G65/4043 , C08G65/4056 , C08G65/4075 , C08G65/42 , C08G65/44 , C08G81/00 , C08G2261/126 , C08G2650/56 , C08K7/14 , C08L71/10 , C08L71/12 , C08L71/123 , C08L71/126 , C08L2205/05 , C08L63/00
摘要： A poly(arylene ether)-poly(hydroxy ether) block copolymer includes at least one poly(hydroxy ether) block and at least one poly(arylene ether) block, and the mole ratio of poly(hydroxy ether) blocks to poly(arylene ether) blocks is 0.95:1 to about 1.00:1. The poly(arylene ether)-poly(hydroxy ether) block copolymer can be prepared by reacting a telechelic poly(arylene ether) having terminal hydroxyl groups with a telechelic poly(hydroxy ether) epoxy resin having terminal epoxy groups, wherein the mole ratio of the telechelic poly(hydroxy ether) to the telechelic poly(arylene ether) is 0.95:1 to 1.00:1. The poly(arylene ether)-poly(hydroxy ether) block copolymer can be shaped into an article by extrusion, thermoforming, or molding, and is a compatibilizing agent for non-polar and polar polymers.
摘要翻译：聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物包括至少一个聚（羟基醚）嵌段和至少一个聚（亚芳基醚）嵌段，以及聚（羟基醚）嵌段与聚（亚芳基）嵌段的摩尔比醚）嵌段为0.95：1至约1.00：1。聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物可以通过使具有末端羟基的遥爪聚（亚芳基醚）与具有末端环氧基的遥爪聚（羟基醚）环氧树脂反应来制备，其中摩尔比遥爪聚（羟基醚）与遥爪聚（亚芳基醚）的比例为0.95:1-1.00:1。聚（亚芳基醚） - 聚（羟基醚）嵌段共聚物可以通过挤出，热成型或模塑成型成制品，并且是非极性和极性聚合物的相容剂。

5. 发明授权

US08273499B2 Membrane-electrode assembly for solid polymer electrolyte fuel cell 有权
标题翻译：固体聚合物电解质燃料电池膜电极组件
公开(公告)号：US08273499B2
公开(公告)日：2012-09-25
申请号：US12474828
申请日：2009-05-29
申请人： Takaki Nakagawa , Ryohei Ishimaru
发明人： Takaki Nakagawa , Ryohei Ishimaru
IPC分类号： H01M8/10
CPC分类号： C08G61/12 , C08G65/4006 , C08G65/4025 , C08G65/4037 , C08G75/23 , C08J5/2256 , C08J2371/12 , C08J2381/06 , H01M4/921 , H01M4/926 , H01M8/0289 , H01M8/1004 , H01M8/1027 , H01M8/103 , H01M8/1032 , H01M8/1039
摘要： A membrane-electrode assembly for a solid polymer electrolyte fuel cell is provided that uses a proton conductive membrane having high proton conductivity and also superior heat resistance and chemical durability. A membrane-electrode assembly for a solid polymer electrolyte fuel cell is provided with an anode on one side of a proton conductive membrane and a cathode on another side thereof, and the proton conductive membrane is a sulfonated polyarylene containing a structure expressed by the general formula (1) below: —Rs—Z—Rh (1) In the formula (1), Z represents at least one structure selected from the group consisting of —CO—, —SO2—, and —SO—; Rs represents a direct bond or any divalent organic group; and Rh represents a nitrogen-containing heterocyclic group.
摘要翻译：提供了一种固体聚合物电解质燃料电池的膜 - 电极组件，其使用具有高质子传导性和优异的耐热性和化学耐久性的质子传导膜。用于固体聚合物电解质燃料电池的膜 - 电极组件在质子传导膜的一侧和另一侧的阴极上设置有阳极，质子传导膜是含有由通式表示的结构的磺化聚亚芳基（1）-Rs-Z-Rh（1）式（1）中，Z表示选自-CO - ， - SO 2 - 和-SO - 的至少一种结构。 Rs表示直接键或任何二价有机基团; 而Rh表示含氮杂环基。

6. 发明授权

US08168742B2 Crosslinkable fluorinated aromatic prepolymer and its uses 有权
标题翻译：可交联的氟化芳族预聚物及其用途
公开(公告)号：US08168742B2
公开(公告)日：2012-05-01
申请号：US12631123
申请日：2009-12-04
申请人： Shunsuke Yokotsuka , Masahiro Ito , Kaori Tsuruoka
发明人： Shunsuke Yokotsuka , Masahiro Ito , Kaori Tsuruoka
IPC分类号： C08G65/38 , C08G63/78 , C08G61/10 , H01L21/02 , H01L21/70
CPC分类号： C08G65/4025 , H01L21/0212 , H01L21/02282 , H01L21/3127
摘要： To provide a crosslinkable fluorinated aromatic prepolymer which is capable of forming a cured product having a low relative permittivity, high heat resistance, low birefringence and high flexibility, and its uses.A crosslinkable fluorinated aromatic prepolymer which is obtained by subjecting a compound (Y-1) having a crosslinkable functional group (A) and a phenolic hydroxyl group and/or a compound (Y-2) having a crosslinkable functional group (A) and a fluorinated aromatic ring, to a condensation reaction in the presence of a HF-removing agent, with a fluorinated aromatic compound (B) represented by the formula (1): (wherein n is an integer of from 0 to 2, each of a and b which are independent of each other, is an integer of 0 to 3, and each of Rf1 and Rf2 represents a fluorinated alkyl group having at most 8 carbon atoms and a compound (C) having at least 3 phenolic hydroxyl groups, and which has crosslinkable functional groups (A) and ether bonds and has a number average molecular weight of from 1×103 to 5×105.
摘要翻译：提供能够形成具有低相对介电常数，高耐热性，低双折射性和高柔性的固化产物的可交联的含氟芳族预聚物及其用途。通过使具有交联性官能团（A）的化合物（Y-1）和酚羟基和/或具有交联性官能团（A）的化合物（Y-2）和氟化芳香环与HF除去剂的存在下的缩合反应与式（1）表示的含氟芳香族化合物（B）：（其中，n为0〜2的整数，a和 b彼此独立，为0〜3的整数，Rf1和Rf2分别表示碳原子数最多为8的氟代烷基和至少3个酚羟基的化合物（C），并且具有交联官能团（A）和醚键，数均分子量为1×10 3〜5×10 5。

7. 发明申请

US20070032628A1 CROSSLINKED COMPOSITIONS COMPRISING A POLY(ARYLENE ETHER) AND A NONLINEAR OPTICAL CHROMOPHORE, AND DEVICES INCORPORATING SAME 失效
标题翻译：包含聚（亚乙基醚）和非线性光学色谱的交联组合物和与其相同的装置
公开(公告)号：US20070032628A1
公开(公告)日：2007-02-08
申请号：US11424946
申请日：2006-06-19
申请人： Diyun Huang , Timothy Londergan
发明人： Diyun Huang , Timothy Londergan
IPC分类号： C08G61/02
CPC分类号： C09K11/06 , C08G18/4879 , C08G65/40 , C08G65/4025 , C08G65/48 , C08J3/24 , C08J3/246 , C08J2371/10 , C08L71/10 , C09K2211/1433 , G03F7/0388 , C08L2666/02
摘要： Crosslinked polymer blends comprising a poly(arylene ether) and a nonlinear optical chromophore. Also featured are electro-optic devices incorporating these blends.
摘要翻译：包含聚（亚芳基醚）和非线性光学发色团的交联聚合物共混物。还有一些结合了这些混合物的电光装置。

8. 发明申请

US20060173129A1 Crosslinkable fluorinated aromatic prepolymer and its uses 审中-公开
标题翻译：可交联的氟化芳族预聚物及其用途
公开(公告)号：US20060173129A1
公开(公告)日：2006-08-03
申请号：US11392727
申请日：2006-03-30
申请人： Shunsuke Yokotsuka , Masahiro Ito , Kaori Tsuruoka
发明人： Shunsuke Yokotsuka , Masahiro Ito , Kaori Tsuruoka
IPC分类号： C08L69/00 , C08G63/78
CPC分类号： C08G65/4025 , H01L21/0212 , H01L21/02282 , H01L21/3127
摘要： To provide a crosslinkable fluorinated aromatic prepolymer which is capable of forming a cured product having a low relative permittivity, high heat resistance, low birefringence and high flexibility, and its uses. A crosslinkable fluorinated aromatic prepolymer which is obtained by subjecting a compound (Y-1) having a crosslinkable functional group (A) and a phenolic hydroxyl group and/or a compound (Y-2) having a crosslinkable functional group (A) and a fluorinated aromatic ring, to a condensation reaction in the presence of a HF-removing agent, with a fluorinated aromatic compound (B) represented by the formula (1): (wherein n is an integer of from 0 to 2, each of a and b which are independent of each other, is an integer of 0 to 3, and each of Rf1 and Rf2 represents a fluorinated alkyl group having at most 8 carbon atoms and a compound (C) having at least 3 phenolic hydroxyl groups, and which has crosslinkable functional groups (A) and ether bonds and has a number average molecular weight of from 1×103 to 5×105.
摘要翻译：提供能够形成具有低相对介电常数，高耐热性，低双折射性和高柔性的固化产物的可交联的含氟芳族预聚物及其用途。通过使具有交联性官能团（A）的化合物（Y-1）和酚羟基和/或具有交联性官能团（A）的化合物（Y-2）和氟化芳香环与HF除去剂的存在下的缩合反应与式（1）表示的含氟芳香族化合物（B）：（其中，n为0〜2的整数，a和 b彼此独立，为0〜3的整数，Rf 1〜R 2各自表示碳原子数为8以下的氟代烷基，具有至少3个酚羟基的化合物（C），并具有交联官能团（A）和醚键，并且具有1×10 3至5×10 5的数均分子量， / SUP>。

9. 发明授权

US06678082B2 Electro-optical component including a fluorinated poly(phenylene ether ketone) protective coating and related methods 失效
标题翻译：电光组件包括氟化聚（苯醚酮）保护涂层及相关方法
公开(公告)号：US06678082B2
公开(公告)日：2004-01-13
申请号：US09952456
申请日：2001-09-12
申请人： Randy T. Pike , Calvin Lee Adkins , Charles E. Bryant
发明人： Randy T. Pike , Calvin Lee Adkins , Charles E. Bryant
IPC分类号： G02F103
CPC分类号： C08G65/4025 , C09D171/00 , Y10S359/90
摘要： A method for applying a protective coating to an electro-optical component includes positioning the electro-optical component in a chamber and applying a coating composition to at least one surface of the electro-optical component to form the protective coating thereon. The coating composition may include fluorinated poly(phenylene ether ketone) and an anti-reflection agent. The anti-reflection agent may include at least one of an inorganic salt, an organofunctionalized additive, and an erbium dopant, for example.
摘要翻译：将保护涂层施加到电光部件的方法包括将电光部件定位在腔室中，并将涂层组合物施加到电光部件的至少一个表面上以在其上形成保护涂层。涂料组合物可以包括氟化聚（苯醚酮）和抗反射剂。防反射剂可以包括例如无机盐，有机官能化添加剂和铒掺杂剂中的至少一种。

10. 发明申请

US20020188097A1 Halogenated aromatic compound, polymer thereof, and proton-conductive membrane comprising same 有权
标题翻译：卤化芳族化合物，其聚合物和包含其的质子传导膜
公开(公告)号：US20020188097A1
公开(公告)日：2002-12-12
申请号：US10105213
申请日：2002-03-26
申请人： JSR CORPORATION
发明人： Kohei Goto , Masayuki Takahashi , Yoshitaka Yamakawa , Makoto Higami
IPC分类号： C08G061/00 , C08G073/24 , C08F283/06
CPC分类号： H01B1/122 , C07C45/71 , C07C49/84 , C07C317/22 , C08G61/12 , C08G65/40 , C08G65/4018 , C08G65/4025 , C08G75/23 , C08J5/2256 , C08J2381/06 , H01M6/181 , H01M2300/0082
摘要： A polymer which has a flexible structure in its main chain and thus exhibits a high toughness and can difficultly be deteriorated in its mechanical properties and thermal properties even when sulfonated, a sulfonic acid group-containing polymer obtained by the sulfonation of the polymer, and a proton-conductive membrane having an excellent mechanical strength and durability made of the sulfonic acid group-containing polymer. A novel halogenated aromatic compound represented by the following general formula (1m) is provided: 1 wherein A independently represents an electron-withdrawing group; B independently represents an electron-donating atom or group; X represents a chlorine atom, iodine atom or bromine atom; R1 to R8 may be the same or different and each represent a hydrogen atom, fluorine atom or alkyl group; and n represents an integer of 2 or more.
摘要翻译：一种聚合物，其主链具有柔性结构，因此即使在磺化时也显示出高的韧性，并且其机械性能和热性能难以降低，通过聚合物的磺化获得的含磺酸基的聚合物和质子传导膜具有优异的机械强度和耐久性，由含磺酸基的聚合物制成。提供由以下通式（1m）表示的新型卤代芳族化合物：其中A独立地表示吸电子基团; B独立地表示给电子原子或基团; X表示氯原子，碘原子或溴原子; R 1至R 8可以相同或不同，各自表示氢原子，氟原子或烷基; n表示2以上的整数。

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