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1. 发明申请

US20120330065A1 PRODUCTION OF MYRTANAL FROM BETA-PINENE EPOXIDE 有权
标题翻译：由环戊二烯环氧化物生产木质素
公开(公告)号：US20120330065A1
公开(公告)日：2012-12-27
申请号：US13517403
申请日：2010-12-17
申请人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
发明人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
IPC分类号： C07C45/58
CPC分类号： B01J29/7615 , B01J29/7057 , B01J29/7815 , B01J35/002 , C01B39/02 , C07C45/58 , C07C47/347
摘要： The present invention refers to a process for the production of myrtanal from β-pinene epoxide that comprises at least of putting this epoxide in contact with a microporous and crystalline catalyst with pores of a diameter of at least 0.52 nm with an empirical formula for the calcinated and dehydrated form of Hw(MwTixSnyZrzSi1-w-x-y-z)O2 where M is at least a metal with valence+3 selected from Al, B, Ga, Fe, Cr and combinations of these; w is a molar fraction of M with a value of between 0 and 2(x+y+z); x is a molar fraction of titanium and has a value of between 0 and 0.06; y is a molar fraction of tin and has a value of between 0 and 0.06; z is a molar fraction of zirconium and has a value of between 0 and 0.06; and where at least one of the three values “x”, “y” or “z” is different from zero. In the present invention, the microporous and crystalline catalyst preferably has pores of at least 0.52 nm and has a crystalline structure with an X-ray diffractogram of a zeolite beta.
摘要翻译：本发明涉及一种从环氧丙烷生产木药的方法，该方法至少包括使该环氧化物与直径为至少0.52nm的孔的微孔和结晶催化剂接触，其经验公式为煅烧和脱水形式的Hw（MwTixSnyZrzSi1-wxyz）O2，其中M至少为选自Al，B，Ga，Fe，Cr的价数+3的金属及其组合; w是0至2（x + y + z）之间的M的摩尔分数; x是钛的摩尔分数，其值在0和0.06之间; y是锡的摩尔分数，其值在0和0.06之间; z是锆的摩尔分数，其值在0和0.06之间; 并且其中三个值x，y或z中的至少一个不同于零。在本发明中，微孔和结晶催化剂优选具有至少0.52nm的孔，并具有具有β沸石的X射线衍射图的晶体结构。

2. 发明授权

US09199955B2 Production of liquid fuels (sylvan-liquid-fuels) from 2-methylfuran 有权
标题翻译：从2-甲基呋喃生产液体燃料（乙醇 - 液体燃料）
公开(公告)号：US09199955B2
公开(公告)日：2015-12-01
申请号：US13491910
申请日：2012-06-08
申请人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
发明人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
IPC分类号： C10G1/00 , C07C27/00 , C10L1/00 , C07D307/38 , C10G3/00
CPC分类号： C07D307/38 , C10G3/42 , C10G3/45 , C10G3/47 , C10G3/50 , Y02P30/20
摘要： The present invention describes a procedure for the production of liquid fuel having a content high in alkanes and low in oxygenated compounds, comprising as a minimum: a first step of alkylation of 2-methylfuran (commonly denominated Sylvan) with a furan alcohol 2 having the formula: (2), wherein R1 is H or an aliphatic or aromatic or heteroaromatic moiety, R2 is H or an aliphatic or aromatic or heteroaromatic moiety, and R3 is H, hydroxymethyl or an aliphatic or aromatic or heteroaromatic moiety, in the presence of a catalyst, a second step of hydrogenation and dehydration of the compound obtained in step 1 in the presence of hydrogen, utilizing suitable hydrogenation and dehydration catalysts.
摘要翻译：本发明描述了生产具有高烷烃含量和低氧化合物含量低的液体燃料的方法，该方法至少包括：将呋喃醇2与2-甲基呋喃（通常称为Sylvan）烷基化的第一步骤式（2）其中R 1为H或脂族或芳族或杂芳族部分，R 2为H或脂族或芳族或杂芳族部分，且R 3为H，羟甲基或脂族或芳族或杂芳族部分，催化剂，在氢存在下，使用合适的氢化和脱水催化剂氢化和脱水步骤1中获得的化合物的第二步骤。

3. 发明申请

US20120316372A1 PRODUCTION OF LIQUID FUELS (SYLVAN-LIQUID-FUELS) FROM 2-METHYLFURAN 有权
标题翻译：二甲苯的液体燃料（SYLVAN-LIQUID-FUELS）的生产
公开(公告)号：US20120316372A1
公开(公告)日：2012-12-13
申请号：US13491910
申请日：2012-06-08
申请人： Avelino CORMA CANÓS , Michael RENZ , Olalla DE LA TORRE ALFARO
发明人： Avelino CORMA CANÓS , Michael RENZ , Olalla DE LA TORRE ALFARO
IPC分类号： C07C1/247
CPC分类号： C07D307/38 , C10G3/42 , C10G3/45 , C10G3/47 , C10G3/50 , Y02P30/20
摘要： The present invention describes a procedure for the production of liquid fuel having a content high in alkanes and low in oxygenated compounds, comprising as a minimum: —a first step of alkylation of 2-methylfuran (commonly denominated Sylvan) with a furan alcohol 2 having the formula: (2), wherein R1 is H or an aliphatic or aromatic or heteroaromatic moiety, R2 is H or an aliphatic or aromatic or heteroaromatic moiety, and R3 is H, hydroxymethyl or an aliphatic or aromatic or heteroaromatic moiety, in the presence of a catalyst, —a second step of hydrogenation and dehydration of the compound obtained in step 1 in the presence of hydrogen, utilising suitable hydrogenation and dehydration catalysts.
摘要翻译：本发明描述了一种制备具有高烷烃含量和低氧化合物含量低的液体燃料的方法，其至少包括： - 第一步是将2-甲基呋喃（通常称为Sylvan）烷基化，其中呋喃醇2具有式（2）其中R 1为H或脂族或芳族或杂芳族部分，R 2为H或脂族或芳族或杂芳族部分，R 3为H，羟甲基或脂族或芳族或杂芳族部分，的催化剂， - 在氢的存在下，利用合适的氢化和脱水催化剂，在步骤1中获得的化合物氢化和脱水的第二步骤。

4. 发明授权

US08633338B2 Production of myrtanal from beta-pinene epoxide 有权
标题翻译：从β-蒎烯环氧化物生产米尔那那
公开(公告)号：US08633338B2
公开(公告)日：2014-01-21
申请号：US13517403
申请日：2010-12-17
申请人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
发明人： Avelino Corma Canós , Michael Renz , Olalla De La Torre Alfaro
IPC分类号： C07C45/58
CPC分类号： B01J29/7615 , B01J29/7057 , B01J29/7815 , B01J35/002 , C01B39/02 , C07C45/58 , C07C47/347
摘要： The present invention refers to a process for the production of myrtanal from β-pinene epoxide that comprises at least of putting this epoxide in contact with a microporous and crystalline catalyst with pores of a diameter of at least 0.52 nm with an empirical formula for the calcinated and dehydrated form of Hw(MwTixSnyZrzSi1-w-x-y-z)O2 where M is at least a metal with valence+3 selected from Al, B, Ga, Fe, Cr and combinations of these; w is a molar fraction of M with a value of between 0 and 2(x+y+z); x is a molar fraction of titanium and has a value of between 0 and 0.06; y is a molar fraction of tin and has a value of between 0 and 0.06; z is a molar fraction of zirconium and has a value of between 0 and 0.06; and where at least one of the three values “x”, “y” or “z” is different from zero. In the present invention, the microporous and crystalline catalyst preferably has pores of at least 0.52 nm and has a crystalline structure with an X-ray diffractogram of a zeolite beta.
摘要翻译：本发明涉及一种由β-蒎烯环氧化物制备米糠醛的方法，该方法至少包括使该环氧化物与具有至少0.52nm直径的孔的微孔和结晶催化剂接触，其煅烧的经验式和Hw（MwTixSnyZrzSi1-wxyz）O2的脱水形式，其中M至少为选自Al，B，Ga，Fe，Cr的价数+3的金属及其组合; w是0至2（x + y + z）之间的M的摩尔分数; x是钛的摩尔分数，其值在0和0.06之间; y是锡的摩尔分数，其值在0和0.06之间; z是锆的摩尔分数，其值在0和0.06之间; 并且三个值“x”，“y”或“z”中的至少一个与零不同。在本发明中，微孔和结晶催化剂优选具有至少0.52nm的孔，并具有具有β沸石的X射线衍射图的晶体结构。

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