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1. 发明授权

US09789445B2 Composite oxygen ion transport membrane 有权
公开(公告)号：US09789445B2
公开(公告)日：2017-10-17
申请号：US14853157
申请日：2015-09-14
申请人： Jonathan A. Lane , Zigui Lu , Pawel J. Plonczak
发明人： Jonathan A. Lane , Zigui Lu , Pawel J. Plonczak
IPC分类号： B01D53/22 , B01D71/02 , B01D69/02 , B01D69/12 , B01D69/10 , C01B13/02 , B01D67/00
CPC分类号： B01D71/024 , B01D53/228 , B01D67/0046 , B01D69/02 , B01D69/10 , B01D69/12 , B01D2325/023 , B01D2325/04 , B01D2325/26 , C01B13/0255
摘要： A composite oxygen ion transport membrane having a dense layer, a porous support layer, an optional intermediate porous layer located between the porous support layer and the dense layer and an optional surface exchange layer, overlying the dense layer. The dense layer has electronic and ionic phases. The ionic phase is composed of scandia doped, yttrium or cerium stabilized zirconia. The electronic phase is composed of a metallic oxide containing lanthanum, strontium, chromium, iron and cobalt. The porous support layer is composed of zirconia partially stabilized with yttrium, scandium, aluminum or cerium or mixtures thereof. The intermediate porous layer, if used, contains the same ionic and electronic phases as the dense layer. The surface exchange layer is formed of an electronic phase of a metallic oxide of lanthanum and strontium that also contains chromium, iron and cobalt and an ionic phase of scandia doped zirconia stabilized with yttrium or cerium.

2. 发明授权

US09592469B2 Oxygen separation device for a pressure swing adsorption system 有权
标题翻译：用于变压吸附系统的氧气分离装置
公开(公告)号：US09592469B2
公开(公告)日：2017-03-14
申请号：US14416066
申请日：2013-07-19
申请人： KONINKLIJKE PHILIPS N.V.
发明人： Mareike Klee , Rainer Hilbig , Robert William Murdoch , Achim Gerhard Rolf Koerber , Wilhelmus Cornelis Keur , Paul Van Der Sluis
IPC分类号： B01D53/22 , B01D53/047 , B01D69/10 , B01D71/02 , A61M16/10 , B01D53/02 , B01J20/18 , B01J20/28 , C01B13/02
CPC分类号： B01D53/229 , A61M16/101 , B01D53/02 , B01D53/047 , B01D53/228 , B01D69/10 , B01D69/105 , B01D71/028 , B01D2053/221 , B01D2253/108 , B01D2253/25 , B01D2256/12 , B01D2257/102 , B01D2259/4533 , B01D2325/12 , B01J20/18 , B01J20/28033 , C01B13/0255 , C01B13/0259 , C01B2203/025 , Y10T29/49789
摘要： The present invention refers to an oxygen separation device (12, 14) for a pressure swing adsorption system. In order to provide at least one of improved maintenance behavior, longer lifetime and improved energy consumption, the oxygen separation device (12, 14) comprises a gas inlet (18, 22) at a primary side for guiding a flow of oxygen comprising gas into the oxygen separation device (12, 14) and a gas outlet (28, 30) at a secondary side for guiding a flow of oxygen enriched gas out of the oxygen separation device (12, 14), an oxygen separation membrane (78) comprising an oxygen separation sorbent being capable of separating oxygen from an oxygen comprising gas by sorbing at least one component of the oxygen comprising gas apart from oxygen, and a support structure (80) for supporting the oxygen separation membrane (78), wherein the support structure (80) comprises a plurality of support bars (82) being fixed to the oxygen separation membrane (78). The invention further relates to an oxygen separator (10) and to a method of generating an oxygen separation device (12, 14) for a pressure swing adsorption system.
摘要翻译：本发明涉及一种用于变压吸附系统的氧气分离装置（12,14）。为了提供改进的维护行为，更长的寿命和改善的能量消耗中的至少一个，氧分离装置（12,14）包括在初级侧的气体入口（18,22），用于将包含气体的氧气流引导到氧分离装置（12,14）和二次侧的气体出口（28,30），用于将富氧气体流引导出氧分离装置（12,14）;氧分离膜（78），包括氧分离吸附剂，其能够通过吸附除了氧以外的含氧气体的至少一种成分以及用于支撑氧分离膜（78）的支撑结构（80），从含氧气体中分离出氧气，其中所述支撑结构（80）包括固定到氧分离膜（78）的多个支撑杆（82）。本发明还涉及氧分离器（10）以及用于产生用于变压吸附系统的氧分离装置（12,14）的方法。

3. 发明授权

US09199847B2 Method and arrangement for generating oxygen 有权
标题翻译：产生氧气的方法和装置
公开(公告)号：US09199847B2
公开(公告)日：2015-12-01
申请号：US14002213
申请日：2012-02-27
申请人： Rainer Hilbig , Achim Gerhard Rolf Koerber , Mareike Klee , Wilco Cornelis Keur
发明人： Rainer Hilbig , Achim Gerhard Rolf Koerber , Mareike Klee , Wilco Cornelis Keur
IPC分类号： B01D53/22 , C01B13/02 , B01D71/02 , B01D53/047
CPC分类号： C01B13/0251 , B01D53/047 , B01D53/22 , B01D53/229 , B01D71/024 , B01D2256/12 , B01D2259/402 , B01D2325/027 , C01B13/0255 , C01B13/0259 , C01B13/027 , Y02P20/126
摘要： The invention relates to a method of generating oxygen. The method comprises the steps of: intermittently guiding a stream of oxygen comprising gas through at least one adsorption chamber (12) being equipped with an oxygen separation adsorbent (16), thereby defining an adsorption mode and a desorption mode of the at least one adsorption chamber (12), and thereby enriching the oxygen comprising gas with respect to oxygen, guiding the enriched oxygen comprising gas to a primary side of a dense membrane (52), heating the dense membrane(52) to a temperature at which it is permeable for oxygen, generating an oxygen flow through the dense membrane (52) to its secondary side, thereby separating the oxygen from the enriched oxygen comprising gas and forming a stream of oxygen. According to the invention, the invention further comprises the step of guiding at least a part of the generated oxygen through the at least one adsorption chamber (12) being in desorption mode. The method according to the invention allows generating oxygen in a high purity, thereby being energy saving, cost saving and being performable in a compact device.
摘要翻译：本发明涉及一种产生氧气的方法。该方法包括以下步骤：间歇地引导包含气体的氧气通过装有氧分离吸附剂（16）的至少一个吸附室（12），从而限定至少一种吸附剂的吸附模式和解吸模式（12），从而使相对于氧气的包含气体的氧富集，将富含氧气的气体引导到致密膜（52）的初级侧，将致密膜（52）加热至可渗透的温度用于氧气，产生通过致密膜（52）到其次级侧的氧气流，从而将氧气与富氧的含氧气体分离并形成氧气流。根据本发明，本发明还包括通过处于解吸模式的至少一个吸附室（12）引导至少一部分产生的氧的步骤。根据本发明的方法允许产生高纯度的氧，从而在紧凑的装置中节能，成本节约和可执行。

4. 发明申请

US20150328582A1 ELECTRODE-SUPPORT TYPE OF GAS-SEPARATION MEMBRANE MODULE, TUBULAR STRUCTURE OF SAME, PRODUCTION METHOD FOR TUBULAR STRUCTURE, AND HYDROCARBON REFORMING METHOD USING SAME 有权
标题翻译：气体分离膜模块的电极支撑型，其管状结构，管状结构的生产方法和使用相同的烃改性方法
公开(公告)号：US20150328582A1
公开(公告)日：2015-11-19
申请号：US14410587
申请日：2013-10-31
申请人： KOREA INSTITUTE OF ENERGY RESEARCH
发明人： Jong Hoon JOO , Ji Haeng YU , Chung-Yul YOO
IPC分类号： B01D53/22 , B01D69/02 , B01D71/02 , C01B13/02 , B01D63/06 , C01B3/36 , C01B3/50 , B01D53/32 , B01D67/00
CPC分类号： B01D53/228 , B01D53/22 , B01D53/229 , B01D53/323 , B01D63/061 , B01D67/0083 , B01D69/02 , B01D71/024 , B01D2256/12 , B01D2256/16 , B01D2319/02 , B01D2323/08 , B01D2325/22 , B01D2325/24 , B01D2325/26 , B01D2325/30 , C01B3/36 , C01B3/503 , C01B13/0255 , C01B2203/025 , C01B2203/1241 , C01B2203/1282
摘要： The present invention provides: an electrode-supporting type of gas-separation membrane module for selectively effecting the passage of a gas via an electron exchange reaction due to a coupling-material layer and gas exchange via an ion-conducting separation layer; a tubular structure of same; a production method for the tubular structure; and a hydrocarbon-reforming method using the gas-separation membrane module. The present invention is advantageous in that outstanding chemical and mechanical durability can be ensured by using a fluorite-based ion-conducting membrane which is chemically stable in CO2 and H2O atmospheres in particular, at high temperature, and in that a pure gas can be produced inexpensively since the passage of gas occurs due to an internal circuit even without applying a voltage from the outside.
摘要翻译：本发明提供一种电极支撑型气体分离膜组件，用于通过离子传导分离层，由于耦合材料层和气体交换而选择性地进行通过电子交换反应的气体的通过; 其管状结构; 一种用于管状结构的生产方法; 和使用气体分离膜组件的烃重整法。本发明的优点在于，可以通过使用在特别是在高温下在CO 2和H 2 O气氛中化学稳定的萤石基离子导电膜来确保优异的化学和机械耐久性，并且可以生产纯气体即使没有从外部施加电压，由于内部电路由于气体的通过而成本低廉。

5. 发明申请

US20150306549A1 Organosiloxane Films for Gas Separations 有权
公开(公告)号：US20150306549A1
公开(公告)日：2015-10-29
申请号：US14792255
申请日：2015-07-06
申请人： Applied Membrane Technology, Inc.
发明人： Ashok K. Sharma
IPC分类号： B01D69/12 , B01D63/02 , C01B13/02 , B01D71/70 , C01B21/04 , B05D1/00 , B01D67/00
CPC分类号： B01D69/125 , B01D53/228 , B01D63/02 , B01D67/0037 , B01D67/0072 , B01D69/02 , B01D69/08 , B01D71/70 , B01D2256/10 , B01D2257/504 , B01D2325/20 , B05D1/62 , C01B13/0255 , C01B21/0444 , Y02C10/10 , Y02P70/38
摘要： A semipermeable gas separation membrane is plasma deposited from liquid organosiloxane monomer having at least three silicon atoms and an alpha hydrogen atom. The semipermeable membrane may be employed as a gas-selective membrane in combination with a porous substrate.

6. 发明授权

US09061929B2 Glass melting furnace 有权
标题翻译：玻璃熔化炉
公开(公告)号：US09061929B2
公开(公告)日：2015-06-23
申请号：US13389164
申请日：2010-08-05
申请人： Francois Bioul , Olivier Douxchamps
发明人： Francois Bioul , Olivier Douxchamps
IPC分类号： F23C10/08 , C03B5/235 , C01B13/02
CPC分类号： C03B5/2353 , C01B13/0255 , C01B2210/0046 , Y02P20/13 , Y02P40/55
摘要： The present invention relates to a furnace (12) for melting heated glass using burners (13), wherein the combustion energy is at least partially produced by oxy-fuel combustion, and wherein at least a portion of the oxygen used is produced by separation, on a ceramic separation membrane (18), from a gaseous mixture including oxygen.
摘要翻译：本发明涉及一种用于使用燃烧器（13）熔化加热玻璃的炉子（12），其中燃烧能量至少部分地由氧 - 燃料燃烧产生，并且其中所用的氧气的至少一部分通过分离产生，在陶瓷分离膜（18）上，从包含氧的气体混合物中。

7. 发明申请

US20150098868A1 CERAMIC OXYGEN TRANSPORT MEMBRANE ARRAY REACTOR AND REFORMING METHOD 有权
标题翻译：陶瓷氧运输膜阵列反应器和改造方法
公开(公告)号：US20150098868A1
公开(公告)日：2015-04-09
申请号：US14508344
申请日：2014-10-07
申请人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
发明人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
IPC分类号： B01J8/00
CPC分类号： B01J8/009 , B01J8/065 , B01J8/067 , B01J12/007 , B01J19/242 , B01J19/2425 , B01J19/243 , B01J19/2475 , B01J2208/00309 , B01J2208/00938 , B01J2219/00006 , B01J2219/0004 , B01J2219/0006 , B01J2219/00117 , C01B3/382 , C01B3/384 , C01B13/0255 , C01B2203/0233 , C01B2203/0244 , C01B2203/0894 , C01B2203/127 , F22B1/003 , F22B1/16 , Y02P20/129
摘要： The invention relates to a commercially viable modular ceramic oxygen transport membrane reforming reactor configured using repeating assemblies of oxygen transport membrane tubes and catalytic reforming reactors.
摘要翻译：本发明涉及一种商业上可行的模块化陶瓷氧传输膜重整反应器，其配置为使用氧传输膜管和催化重整反应器的重复组件。

8. 发明申请

US20150096506A1 CERAMIC OXYGEN TRANSPORT MEMBRANE ARRAY REACTOR AND REFORMING METHOD 有权
标题翻译：陶瓷氧运输膜阵列反应器和改造方法
公开(公告)号：US20150096506A1
公开(公告)日：2015-04-09
申请号：US14508326
申请日：2014-10-07
申请人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
发明人： Sean M. Kelly , Gervase Maxwell Christie , Charles Robinson , Jamie R. Wilson , Javier E. Gonzalez , Uttam R. Doraswami
IPC分类号： F22B1/00 , F22B1/16
CPC分类号： B01J8/009 , B01J8/065 , B01J8/067 , B01J12/007 , B01J19/242 , B01J19/2425 , B01J19/243 , B01J19/2475 , B01J2208/00309 , B01J2208/00938 , B01J2219/00006 , B01J2219/0004 , B01J2219/0006 , B01J2219/00117 , C01B3/382 , C01B3/384 , C01B13/0255 , C01B2203/0233 , C01B2203/0244 , C01B2203/0894 , C01B2203/127 , F22B1/003 , F22B1/16 , Y02P20/129
摘要： The invention relates to a commercially viable modular ceramic oxygen transport membrane system for utilizing heat generated in reactively-driven oxygen transport membrane tubes to generate steam, heat process fluid and/or provide energy to carry out endothermic chemical reactions. The system provides for improved thermal coupling of oxygen transport membrane tubes to steam generation tubes or process heater tubes or reactor tubes for efficient and effective radiant heat transfer.
摘要翻译：本发明涉及一种商业可行的模块化陶瓷氧输送膜系统，用于利用在反应驱动的氧传输膜管中产生的热产生蒸汽，加热过程流体和/或提供能量以进行吸热化学反应。该系统提供氧传输膜管与蒸汽发生管或过程加热器管或反应管的热耦合，用于有效和有效的辐射热传递。

9. 发明授权

US08999039B2 Oxygen separation membrane 有权
标题翻译：氧分离膜
公开(公告)号：US08999039B2
公开(公告)日：2015-04-07
申请号：US13581870
申请日：2011-02-04
申请人： Rainer Hilbig , Joachim Opitz
发明人： Rainer Hilbig , Joachim Opitz
IPC分类号： B01D53/22 , B01D69/10 , B01D65/02 , B01D69/02 , B01D71/02 , C01B13/02
CPC分类号： B01D53/228 , B01D65/02 , B01D69/02 , B01D71/02 , B01D2256/12 , B01D2259/4533 , B01D2313/22 , B01D2321/32 , B01D2325/22 , B01D2325/26 , C01B13/0255 , C01B2210/0046
摘要： The invention relates to membranes, in particular oxygen separation membranes, which enable improved gas separation conditions with respect to cost, price, size, weight, and noise. The membrane, in particular oxygen separation membrane, according to the invention comprises a support layer (28) and a separation layer (30), wherein the separation layer (30) is permeable for oxygen and has a sorptive affinity for at least one other gas, in particular for nitrogen, wherein the membrane (20) is designed such that substantially only the separation layer (30) is heatable by a heating device.
摘要翻译：本发明涉及膜，特别是氧分离膜，其能够在成本，价格，尺寸，重量和噪声方面改善气体分离条件。根据本发明的膜，特别是氧分离膜包括支撑层（28）和分离层（30），其中分离层（30）对于氧可渗透并且对至少一种其它气体具有吸附亲和力，特别是氮气，其中膜（20）被设计成使得基本上只有分离层（30）可被加热装置加热。

10. 发明申请

US20140311346A1 COMPOSITE OXYGEN TRANSPORT MEMBRANE 有权
标题翻译：复合氧运输膜
公开(公告)号：US20140311346A1
公开(公告)日：2014-10-23
申请号：US14322981
申请日：2014-07-03
申请人： Gervase Maxwell Christie , Jonathan A. Lane
发明人： Gervase Maxwell Christie , Jonathan A. Lane
IPC分类号： B01D53/22
CPC分类号： B01D53/228 , B01D67/0041 , B01D69/02 , B01D69/12 , B01D71/024 , B01D71/028 , B01D2255/402 , B01D2255/407 , B01D2255/902 , B01D2256/12 , B01D2257/104 , B01D2258/06 , B01D2325/023 , C01B13/0255 , C04B35/01 , C04B35/016 , C04B35/2633 , C04B35/42 , C04B35/44 , C04B35/462 , C04B35/488 , C04B38/00 , C04B2111/00612 , C04B2111/00801 , C04B2111/0081 , C04B2235/3208 , C04B2235/3217 , C04B2235/3222 , C04B2235/3224 , C04B2235/3225 , C04B2235/3227 , C04B2235/3229 , C04B2235/3232 , C04B2235/3234 , C04B2235/3243 , C04B2235/3246 , C04B2235/3262 , C04B2235/3268 , C04B2235/3272 , C04B2235/3274 , C04B2235/3275 , C04B2235/5445 , C04B2235/768 , C04B2235/80 , Y10T428/1314 , Y10T428/24997 , Y10T428/24999 , C04B35/48 , C04B38/0074 , C04B35/443 , C04B35/04
摘要： A method of producing a composite oxygen ion membrane and a composite oxygen ion membrane in which a porous fuel oxidation layer and a dense separation layer and optionally, a porous surface exchange layer are formed on a porous support from mixtures of (Ln1-xAx)wCr1-yByO3-δ and a doped zirconia. In the porous fuel oxidation layer and the optional porous surface exchange layer, A is Calcium and in the dense separation layer A is not Calcium and, preferably is Strontium. Preferred materials are (La0.8Ca0.2)0.95Cr0.5Mn0.5O3-δ for the porous fuel oxidation and optional porous surface exchange layers and (La0.8Sr0.2)0.95Cr0.5Fe0.5O3-δ for the dense separation layer. The use of such materials allows the membrane to sintered in air and without the use of pore formers to reduce membrane manufacturing costs. The use of materials, as described herein, for forming the porous layers have application for forming any type of porous structure, such as a catalyst support.
摘要翻译：一种制备复合氧离子膜和复合氧离子膜的方法，其中多孔燃料氧化层和致密分离层以及任选的多孔表面交换层由（Ln1-xAx）wCr1的混合物形成在多孔载体上 -yByO3-δ和掺杂的氧化锆。在多孔燃料氧化层和任选的多孔表面交换层中，A为钙，密实分离层A不为钙，优选为锶。优选的材料是（La0.8Ca0.2）0.95Cr0.5Mn0.5O3-δ用于多孔燃料氧化和任选的多孔表面交换层和（La0.8Sr0.2）0.95Cr0.5Fe0.5O3-δ用于致密分离层。使用这种材料允许膜在空气中烧结而不使用成孔剂来降低膜的制造成本。如本文所述用于形成多孔层的材料的使用具有用于形成任何类型的多孔结构例如催化剂载体的应用。

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