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1. 发明授权

US07179313B2 Regenerative autothermal catalytic steam reformer 有权
标题翻译：再生自热催化蒸汽重整器
公开(公告)号：US07179313B2
公开(公告)日：2007-02-20
申请号：US10347130
申请日：2003-01-17
申请人： William B. Retallick , William A. Whittenberger
发明人： William B. Retallick , William A. Whittenberger
IPC分类号： C10J8/00 , B01J3/20 , B01J7/00 , B01J8/04 , B01J8/00
CPC分类号： B01J19/249 , B01J12/007 , B01J2219/00164 , B01J2219/2453 , B01J2219/2458 , B01J2219/2465 , B01J2219/2466 , B01J2219/247 , B01J2219/2479 , B01J2219/2493 , C01B3/384 , C01B3/48 , C01B2203/0216 , C01B2203/0283 , C01B2203/066 , C01B2203/0811 , C01B2203/1035 , C01B2203/1652 , C01B2203/169
摘要： A compact steam reformer produces hydrogen to power a fuel cell, such as can be used in a vehicle. The steam reformer includes a first channel, at least partly coated with a steam reforming catalyst, and a second channel, at least partly coated with a combustion catalyst, the channels being in thermal contact with each other. Heat from the combustion is used in the steam reforming reaction. In another embodiment, the gas streams feeding the reforming and combustion channels pass through a valve which reverses the gas streams periodically. The combustion channel becomes the reforming channel, and vice versa, so that carbon deposits in the former reforming channel are burned off. This arrangement enables the reforming reaction to continue indefinitely at peak efficiency.
摘要翻译：紧凑型蒸汽重整器产生氢气以为燃料电池供电，例如可用于车辆中。蒸汽重整器包括至少部分地涂覆有蒸汽重整催化剂的第一通道和至少部分地涂覆有燃烧催化剂的第二通道，所述通道彼此热接触。在蒸汽重整反应中使用来自燃烧的热。在另一个实施例中，供给重整和燃烧通道的气流通过一个周期性地反转气流的阀。燃烧通道成为重整通道，反之亦然，因此前一重整通道中的碳沉积物被烧掉。这种布置使重整反应在峰值效率下无限期地继续。

2. 发明授权

US06936237B2 Reforming catalysts and methods of alcohol steam reforming 失效
标题翻译：重整催化剂和醇蒸汽重整方法
公开(公告)号：US06936237B2
公开(公告)日：2005-08-30
申请号：US09788294
申请日：2001-02-16
申请人： Yong Wang , Anna Lee Y. Tonkovich , Jianli Hu
发明人： Yong Wang , Anna Lee Y. Tonkovich , Jianli Hu
IPC分类号： B01D53/22 , B01D71/02 , B01J12/00 , B01J19/00 , B01J19/24 , B01J23/60 , B01J37/02 , B01J37/03 , C01B3/38 , C01B3/48 , C01B3/50 , C01B3/56 , C01B13/02 , H01M8/06 , C01B3/26
CPC分类号： B01J37/0215 , B01J12/007 , B01J19/0093 , B01J23/60 , B01J37/031 , B01J2219/00835 , B01J2219/2453 , B01J2219/2465 , B01J2219/2474 , B01J2219/2475 , B01J2219/2479 , B01J2219/2482 , B01J2219/2497 , C01B3/38 , C01B3/501 , C01B13/0251 , C01B2203/0233 , C01B2203/0283 , C01B2203/0405 , C01B2203/041 , C01B2203/044 , C01B2203/047 , C01B2203/065 , C01B2203/066 , C01B2203/0811 , C01B2203/0833 , C01B2203/1005 , C01B2203/1011 , C01B2203/1029 , C01B2203/1035 , C01B2203/1041 , C01B2203/1052 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1094 , C01B2203/1217 , C01B2203/1223 , C01B2203/1241 , C01B2203/1276 , C01B2203/1288 , C01B2203/148 , C01B2203/1604 , C01B2203/1619 , C01B2203/1652 , C01B2203/1676 , C01B2210/0046 , H01M8/0612 , Y02P20/52
摘要： The present invention provides catalysts, reactors, and methods of steam reforming alcohols over a catalyst. Surprisingly superior results and properties obtained in methods and catalysts of the present invention are also described.
摘要翻译：本发明提供了在催化剂上蒸汽重整醇的催化剂，反应器和方法。还描述了在本发明的方法和催化剂中获得的令人惊奇的优异结果和性能。

3. 发明申请

US20040060238A1 Autothermal catalytic steam reformer 审中-公开
标题翻译：自热催化蒸汽重整器
公开(公告)号：US20040060238A1
公开(公告)日：2004-04-01
申请号：US10211083
申请日：2002-08-02
发明人： William B. Retallick , William A. Whittenberger
IPC分类号： C01B003/24
CPC分类号： B01J19/249 , B01J12/007 , B01J2219/00164 , B01J2219/2453 , B01J2219/2458 , B01J2219/2465 , B01J2219/2466 , B01J2219/247 , B01J2219/2479 , B01J2219/2493 , C01B3/384 , C01B3/48 , C01B2203/0216 , C01B2203/0283 , C01B2203/066 , C01B2203/0811 , C01B2203/1035 , C01B2203/1652 , C01B2203/169
摘要： A compact steam reformer produces hydrogen to power a fuel cell, such as can be used in a vehicle. The steam reformer includes a first channel, at least partly coated with a steam reforming catalyst, and a second channel, at least partly coated with a combustion catalyst, the channels being in thermal contact with each other. Heat from the combustion is used in the steam reforming reaction. The steam reformer may be provided as a stack of strips defining steam reforming channels which alternate with combustion channels. The reformer may also include a set of modules, connected in series, each module including a stack of strips as described above. The steam reformer preferably also includes a channel wherein a water-gas shift reaction occurs, to convert carbon monoxide, produced by the reformer, into carbon dioxide.
摘要翻译：紧凑型蒸汽重整器产生氢气以为燃料电池供电，例如可用于车辆中。蒸汽重整器包括至少部分地涂覆有蒸汽重整催化剂的第一通道和至少部分地涂覆有燃烧催化剂的第二通道，所述通道彼此热接触。在蒸汽重整反应中使用来自燃烧的热。蒸汽重整器可以被设置为一组条带，其限定与燃烧通道交替的蒸汽重整通道。重整器还可以包括串联连接的一组模块，每个模块包括如上所述的一堆条带。蒸汽重整器优选还包括其中发生水煤气变换反应以将由重整器产生的一氧化碳转化为二氧化碳的通道。

4. 发明授权

US06692545B2 Combined water gas shift reactor/carbon dioxide adsorber for use in a fuel cell system 有权
标题翻译：用于燃料电池系统的组合式水煤气变换反应器/二氧化碳吸附器
公开(公告)号：US06692545B2
公开(公告)日：2004-02-17
申请号：US09780079
申请日：2001-02-09
申请人： Craig S. Gittleman , Ramesh Gupta
发明人： Craig S. Gittleman , Ramesh Gupta
IPC分类号： C10K302
CPC分类号： B01D53/06 , B01D53/047 , B01D53/864 , B01D2253/102 , B01D2253/104 , B01D2253/108 , B01D2253/112 , B01D2256/16 , B01D2257/502 , B01D2257/504 , B01D2259/40052 , B01D2259/40062 , B01D2259/41 , C01B3/16 , C01B3/48 , C01B3/56 , C01B2203/0205 , C01B2203/0283 , C01B2203/0425 , C01B2203/047 , C01B2203/0475 , C01B2203/0495 , C01B2203/066 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/0883 , C01B2203/1005 , C01B2203/1047 , C01B2203/1082 , C01B2203/1223 , C01B2203/1229 , C01B2203/1241 , C01B2203/1247 , C01B2203/146 , C01B2203/1604 , C01B2203/1652 , C01B2203/82 , H01M8/0612 , H01M8/0668 , Y02C10/08 , Y02P20/128 , Y02P20/129 , Y02P20/152
摘要： An apparatus removes CO from a hydrogen-rich gas stream in a hydrogen fuel cell system. CO fouls costly catalytic particles in the membrane electrode assemblies. Both a catalyst adapted to perform a water gas shift reaction, and a carbon dioxide adsorbent are disposed in a rotating pressure swing adsorber housing. The adsorption of carbon dioxide shifts equilibrium toward carbon monoxide consumption. A second adsorbent may be disposed in the housing for adsorbing carbon monoxide at low temperatures, and is adapted to desorb carbon monoxide at high temperatures. The present invention advantageously eliminates a unit operation from a space-constrained fuel cell vehicle by combining the WGS catalyst and a CO2 adsorbent in a single reactor/housing. The apparatus further eliminates the use of a PROX reactor, by providing an apparatus which incorporates CO2 adsorption and consequent carbon monoxide consumption in the place of the PROX reactor.
摘要翻译：一种装置从氢燃料电池系统中的富氢气流中除去CO。 CO会损坏膜电极组件中昂贵的催化颗粒。适用于执行水煤气变换反应的催化剂和二氧化碳吸附剂均设置在旋转变压吸附器壳体中。二氧化碳的吸附将平衡转移到一氧化碳消耗。第二吸附剂可以设置在壳体中用于在低温下吸附一氧化碳，并且适于在高温下解吸一氧化碳。本发明通过在单个反应器/壳体中组合WGS催化剂和CO 2吸附剂有利地消除了来自空间受限的燃料电池车辆的单元操作。该设备进一步消除了使用PROX反应器，通过提供一种将CO 2吸附和随后的一氧化碳消耗引入到PROX反应器的装置中。

5. 发明申请

US20030187310A1 Fuel for fuel cell system 审中-公开
标题翻译：燃料电池系统燃料
公开(公告)号：US20030187310A1
公开(公告)日：2003-10-02
申请号：US10297934
申请日：2003-05-27
发明人： Kenichirou Saitou , Iwao Anzai , Osamu Sadakane , Michiro Matsubara
IPC分类号： C10L003/00
CPC分类号： C01B3/583 , C01B3/38 , C01B3/48 , C01B2203/0233 , C01B2203/0261 , C01B2203/0283 , C01B2203/044 , C01B2203/047 , C01B2203/066 , C01B2203/085 , C01B2203/1064 , C01B2203/1205 , C01B2203/1223 , C01B2203/1235 , C01B2203/1288 , C01B2203/1652 , C10L3/00 , H01M8/0612
摘要： A fuel for a fuel cell system comprises wherein said fuel comprises 5 mol. % or more of hydrocarbons, 0.5-20 mass % of oxygenates therein in terms of an oxygen content batsed on the whole fuel and 5 mol. % or less of hydrocarbons having carbon numbers of 2 or less, 90 mol. % or more of hydrocarbons having carbon numbers of 3 and 4 in total, 5 mol. % or less of hydrocarbons having carbon numbers of 5 or more and is a gaseous phase under normal temperature and pressure. The fuel for a fuel cell system has a high power generation quantity per weight, a high power generation quantity per CO2 emission, a low fuel consumption, a small evaporative gas (evapo-emission), small deterioration of a fuel cell system comprising such as a reforming catalyst, a water gas shift reaction catalyst, a carbon monoxide removal catalyst, fuel cell stacks and the like to maintain the initial performances for a long duration, good handling properties in view of storage stability and inflammability, and a low preheating heat quantity.
摘要翻译：用于燃料电池系统的燃料包括其中所述燃料包含5mol。以上，全部燃料中含有的氧含量为5〜5质量％，含有0.5-20质量％的含氧化合物。碳数为2以下的烃的％以下为90摩尔％以下。总共有碳数为3和4的烃的5％以上。碳数为5以上的烃的％以下为常温常压下的气相。用于燃料电池系统的燃料具有每重量的高发电量，每二氧化碳排放的高发电量，低燃料消耗量，小蒸发气体（蒸发发射），燃料电池系统的劣化，包括例如重整催化剂，水煤气变换反应催化剂，一氧化碳去除催化剂，燃料电池堆等，以保持长时间的初始性能，考虑到储存稳定性和易燃性，处理性能好，预热热量低。

6. 发明申请

US20030017105A1 Catalyst and method of steam reforming 有权
标题翻译：催化剂和蒸汽重整方法
公开(公告)号：US20030017105A1
公开(公告)日：2003-01-23
申请号：US10076881
申请日：2002-02-13
发明人： Yong Wang , Anna Lee Tonkovich , David P. Vanderwiel
IPC分类号： C01B003/26
CPC分类号： B01J12/007 , B01J19/0093 , B01J21/005 , B01J21/10 , B01J23/005 , B01J23/40 , B01J23/464 , B01J23/58 , B01J27/22 , B01J35/06 , B01J37/0207 , B01J37/0225 , B01J37/0244 , B01J37/0248 , B01J2219/00788 , B01J2219/00826 , B01J2219/00835 , B01J2219/00873 , B01J2219/00891 , B01J2219/00961 , B01J2219/2453 , B01J2219/2465 , B01J2219/2474 , B01J2219/2475 , B01J2219/2479 , B01J2219/2482 , B01J2219/2497 , C01B3/38 , C01B3/40 , C01B3/501 , C01B13/0251 , C01B2203/0233 , C01B2203/0283 , C01B2203/0405 , C01B2203/041 , C01B2203/044 , C01B2203/047 , C01B2203/065 , C01B2203/066 , C01B2203/0811 , C01B2203/0816 , C01B2203/0833 , C01B2203/1005 , C01B2203/1011 , C01B2203/1029 , C01B2203/1035 , C01B2203/1041 , C01B2203/1052 , C01B2203/1058 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1094 , C01B2203/1217 , C01B2203/1223 , C01B2203/1241 , C01B2203/1247 , C01B2203/1276 , C01B2203/1288 , C01B2203/148 , C01B2203/1604 , C01B2203/1619 , C01B2203/1652 , C01B2203/1676 , C01B2203/169 , C01B2203/80 , H01M8/0612 , Y02P20/52
摘要： The present invention provides a method of steam reforming a hydrocarbon over a catalyst at short residence times or short contact times. The present invention also provides spinel-containing catalysts. Surprisingly superior results and properties obtained in methods and catalysts of the present invention are also described.
摘要翻译：本发明提供一种在短的停留时间或短的接触时间下在催化剂上蒸汽重整烃的方法。本发明还提供了含尖晶石的催化剂。还描述了在本发明的方法和催化剂中获得的令人惊奇的优异结果和性能。

7. 发明授权

US09452402B2 Integrated reactors, methods of making same, and methods of conducting simultaneous exothermic and endothermic reactions 有权
公开(公告)号：US09452402B2
公开(公告)日：2016-09-27
申请号：US14053500
申请日：2013-10-14
申请人： Battelle Memorial Institute
发明人： Anna Lee Tonkovich , Gary Roberts , Steven T. Perry , Sean P. Fitzgerald , Robert S. Wegeng , Yong Wang , David Vanderwiel , Jennifer L. Marco
IPC分类号： B01J19/00 , B01J19/24 , B01J10/00 , B01J12/00 , B01J14/00 , B01J15/00 , B01J16/00 , C01B3/38 , B01J8/02 , C01B3/50 , C01B13/02 , F23C13/00 , F23N1/00 , C01B3/00 , C01B3/02 , C01B3/32 , C01B3/34 , H01M8/06
CPC分类号： B01J8/0285 , B01J12/007 , B01J19/0093 , B01J19/249 , B01J2208/00309 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00833 , B01J2219/00835 , B01J2219/00844 , B01J2219/0086 , B01J2219/00873 , B01J2219/00891 , B01J2219/2453 , B01J2219/2458 , B01J2219/2459 , B01J2219/2465 , B01J2219/247 , B01J2219/2471 , B01J2219/2474 , B01J2219/2475 , B01J2219/2479 , B01J2219/2482 , B01J2219/2497 , B01J2219/2498 , C01B3/38 , C01B3/384 , C01B3/501 , C01B13/0251 , C01B2203/0233 , C01B2203/0244 , C01B2203/0261 , C01B2203/0283 , C01B2203/041 , C01B2203/0495 , C01B2203/0811 , C01B2203/0822 , C01B2203/0827 , C01B2203/0833 , C01B2203/0844 , C01B2203/0883 , C01B2203/1005 , C01B2203/1029 , C01B2203/1035 , C01B2203/1041 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1205 , C01B2203/1241 , C01B2203/1276 , C01B2203/1288 , C01B2203/141 , C01B2203/142 , C01B2203/148 , C01B2203/1604 , C01B2203/1619 , C01B2203/1633 , C01B2203/1652 , C01B2203/1676 , C01B2203/169 , C01B2203/1695 , C01B2203/82 , F23C13/00 , F23N1/007 , H01M8/0631 , Y02E60/324 , Y02P20/128 , Y02P20/52 , Y02P70/56 , Y10T29/49826
摘要： Integrated Combustion Reactors (ICRs) and methods of making ICRs are described in which combustion chambers (or channels) are in direct thermal contact to reaction chambers for an endothermic reaction. Superior results were achieved for combustion chambers which contained a gap for free flow through the chamber. Particular reactor designs are also described. Processes of conducting reactions in integrated combustion reactors are described and results presented. Some of these processes are characterized by unexpected and superior results.

8. 发明授权

US08497042B2 Fuel cell system 有权
标题翻译：燃料电池系统
公开(公告)号：US08497042B2
公开(公告)日：2013-07-30
申请号：US12673876
申请日：2008-09-08
申请人： Kazufumi Takeuchi , Hiromichi Miwa , Masaharu Hatano , Keiko Kushibiki , Dong Song
发明人： Kazufumi Takeuchi , Hiromichi Miwa , Masaharu Hatano , Keiko Kushibiki , Dong Song
IPC分类号： H01M8/06
CPC分类号： H01M8/04179 , C01B3/34 , C01B3/382 , C01B2203/0233 , C01B2203/0244 , C01B2203/025 , C01B2203/0266 , C01B2203/066 , C01B2203/1258 , C01B2203/1276 , C01B2203/143 , C01B2203/148 , C01B2203/1652 , C01B2203/1685 , C01B2203/1695 , H01M8/04014 , H01M8/04089 , H01M8/04164 , H01M8/04365 , H01M8/04373 , H01M8/04388 , H01M8/04708 , H01M8/04835 , H01M8/0618 , H01M2008/1293
摘要： Disclosed is a fuel cell system comprising a reformer and a fuel cell body to which a fuel gas reformed through the reformer and air are supplied and in which the supplied fuel gas and air are separated from each other and caused to flow and contact on respective electrodes to perform electric power generation. A moisture quantity adjustment device is configured to adjustably separate a portion of moisture included in the fuel gas supplied from the reformer in order for the moisture included in the fuel gas to be supplied to the fuel cell body in an appropriate quantity.
摘要翻译：公开了一种燃料电池系统，其包括重整器和燃料电池体，燃料气体通过重整器和空气被重整而供给到燃料电池体中，并且供给的燃料气体和空气彼此分离并使其在各个电极上流动和接触进行发电。水分量调节装置被配置为可调节地分离供应到重整器中的燃料气体中包含的一部分水分，以使包含在燃料气体中的水分以适当的量供应到燃料电池体。

9. 发明授权

US08231857B2 Catalysts and methods for reforming oxygenated compounds 有权
标题翻译：用于重整含氧化合物的催化剂和方法
公开(公告)号：US08231857B2
公开(公告)日：2012-07-31
申请号：US12158635
申请日：2006-12-18
申请人： Randy D. Cortright , Nicholas W. Vollendorf , Charles C. Hornemann , Shawn P. McMahon
发明人： Randy D. Cortright , Nicholas W. Vollendorf , Charles C. Hornemann , Shawn P. McMahon
IPC分类号： C01B3/22 , B01J21/18 , C07C1/20
CPC分类号： B01J23/8896 , B01J21/18 , B01J23/656 , B01J23/6567 , B01J23/889 , B01J37/0201 , B01J37/0205 , B01J37/0207 , C01B3/326 , C01B2203/0233 , C01B2203/0805 , C01B2203/1041 , C01B2203/1047 , C01B2203/1064 , C01B2203/107 , C01B2203/1217 , C01B2203/1652 , C01B2203/1676 , C07C1/20 , C07C2523/656 , C10G3/45 , C10G3/47 , C10G3/48 , C10G2300/1011 , C10G2400/28 , Y02P20/52 , Y02P30/20 , C07C9/00
摘要： Disclosed are catalysts and methods that can reform aqueous solutions of oxygenated compounds such as ethylene glycol, glycerol, sugar alcohols, and sugars to generate products such as hydrogen and alkanes. In some embodiments, aqueous solutions containing at least 20 wt % of the oxygenated compounds can be reformed over a catalyst comprising a Group VIII transition metal and a Group VIIB transition metal, preferably supported on an activated carbon-supported catalyst. In other embodiments, catalysts are provided for the production of hydrogen or alkanes at reaction temperatures less than 300° C.
摘要翻译：公开了可以改造含氧化合物如乙二醇，甘油，糖醇和糖的水溶液以产生诸如氢和烷烃的产物的催化剂和方法。在一些实施方案中，含有至少20重量％的氧化化合物的水溶液可以通过包含第VIII族过渡金属和第VIIB族过渡金属的催化剂进行改性，优选负载在活性炭负载的催化剂上。在其它实施方案中，提供催化剂用于在低于300℃的反应温度下生产氢或烷烃。

10. 发明申请

US20060067861A1 Chemical reactor and method for gas phase reactant catalytic reactions 有权
公开(公告)号：US20060067861A1
公开(公告)日：2006-03-30
申请号：US11282423
申请日：2005-11-18
申请人： Anna Tonkovich , Yong Wang , Sean Fitzgerald , Jennifer Marco , Gary Roberts , David Vanderwiel , Robert Wegeng
发明人： Anna Tonkovich , Yong Wang , Sean Fitzgerald , Jennifer Marco , Gary Roberts , David Vanderwiel , Robert Wegeng
IPC分类号： B01J8/02 , B01J8/04
CPC分类号： C01B3/384 , B01J12/007 , B01J19/0093 , B01J23/58 , B01J23/60 , B01J35/04 , B01J37/0215 , B01J37/031 , B01J2219/00159 , B01J2219/00783 , B01J2219/00822 , B01J2219/00824 , B01J2219/00835 , B01J2219/00844 , B01J2219/00873 , B01J2219/00907 , B01J2219/00984 , B01J2219/2453 , B01J2219/2465 , B01J2219/2474 , B01J2219/2475 , B01J2219/2479 , B01J2219/2482 , B01J2219/2497 , C01B3/38 , C01B3/501 , C01B13/0251 , C01B2203/0233 , C01B2203/0283 , C01B2203/0405 , C01B2203/041 , C01B2203/044 , C01B2203/047 , C01B2203/065 , C01B2203/066 , C01B2203/0811 , C01B2203/0822 , C01B2203/0833 , C01B2203/0838 , C01B2203/1005 , C01B2203/1011 , C01B2203/1029 , C01B2203/1035 , C01B2203/1041 , C01B2203/1047 , C01B2203/1052 , C01B2203/1064 , C01B2203/1076 , C01B2203/1082 , C01B2203/1094 , C01B2203/1217 , C01B2203/1223 , C01B2203/1241 , C01B2203/1258 , C01B2203/1276 , C01B2203/1288 , C01B2203/148 , C01B2203/1604 , C01B2203/1619 , C01B2203/1652 , C01B2203/1676 , C01B2210/0046 , H01M8/0612 , Y02P20/128 , Y02P20/52
摘要： The present invention is a chemical reactor and method for catalytic chemical reactions having gas phase reactants. The chemical reactor has reactor microchannels for flow of at least one reactant and at least one product, and a catalyst material wherein the at least one reactant contacts the catalyst material and reacts to form the at least one product. The improvement, according to the present invention is: the catalyst material is on a porous material having a porosity that resists bulk flow therethrough and permits molecular diffusion therein. The porous material further has a length, a width and a thickness, the porous material defining at least a portion of one wall of a bulk flow path through which the at least one reactant passes.

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