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31. 发明授权

US08324335B2 Propylene-based polymer and method for producing the same, and propylene-based resin composition 有权
标题翻译：丙烯系聚合物及其制造方法以及丙烯系树脂组合物
公开(公告)号：US08324335B2
公开(公告)日：2012-12-04
申请号：US12514323
申请日：2007-11-16
申请人： Masaaki Ito , Hideshi Uchino , Kazuya Sakata , Masaru Aoki , Masato Nakano , Shinichi Kitade
发明人： Masaaki Ito , Hideshi Uchino , Kazuya Sakata , Masaru Aoki , Masato Nakano , Shinichi Kitade
IPC分类号： C08F210/06 , C08F210/16 , C08L23/14
CPC分类号： C08F210/06 , C08F4/65904 , C08F4/65912 , C08F4/65927 , C08F10/00 , C08F10/10 , C08F110/06 , C08L23/14 , C08L2205/02 , C08L2314/06 , C08F2/001 , C08F4/65916 , C08L2666/06 , C08F2500/01 , C08F2500/12 , C08F2500/09 , C08F2500/11 , C08F210/16
摘要： A propylene-based polymer comprising the following component (A) insoluble in p-xylene at 25° C. and component (B) soluble in p-xylene at 25° C., wherein (i) the weight average molecular weight (Mw) measured with GPC is 100,000 to 1,000,000, (ii) the content of the component insoluble in hot p-xylene is 0.3% by weight or lower, and (iii) the degree of strain hardening (λ max) in measurement of elongational viscosity is 2.0 or higher; and a method for producing the same, along with a resin composition comprising a propylene-ethylene copolymer (Z) in an amount of 50.0 to 99.9% by weight and a propylene-based polymer (M) in an amount of 0.1 to 50.0% by weight.Component (A): a component (CXIS) insoluble in p-xylene at 25° C., having requirements specified by (A1) to (A5). Component (B): a component (CXS) is soluble in p-xylene at 25° C., having requirements specified by (B1) to (B4).
摘要翻译：包含在25℃下不溶于对二甲苯的下述组分（A）和在25℃下可溶于对二甲苯的组分（B）的丙烯基聚合物，其中（i）重均分子量（Mw）使用GPC测定为100,000〜1,000,000，（ii）不溶于热对二甲苯的成分的含量为0.3重量％以下，（iii）伸长粘度测定中的应变硬化度（λmax）为2.0 或更高; 及其制造方法，以及含有50.0〜99.9重量％的丙烯 - 乙烯共聚物（Z）和丙烯系聚合物（M）的含量为0.1〜50.0％的树脂组合物，其量为0.1〜50.0％重量。组分（A）：在25℃下不溶于对二甲苯的组分（CXIS），具有（A1）至（A5）规定的要求。组分（B）：组分（CXS）在25℃下可溶于对二甲苯，具有（B1）至（B4）所规定的要求。

32. 发明申请

US20110230622A1 METALLOCENE COMPLEX AND POLYMERIZATION METHOD OF OLEFIN 有权
标题翻译：烯烃复合物和烯烃聚合方法
公开(公告)号：US20110230622A1
公开(公告)日：2011-09-22
申请号：US13131301
申请日：2009-12-14
申请人： Masato Nakano , Hideshi Uchino , Naoshi Iwama , Masami Kashimoto , Tomohiro Kato
发明人： Masato Nakano , Hideshi Uchino , Naoshi Iwama , Masami Kashimoto , Tomohiro Kato
IPC分类号： C08F299/00 , C08F4/76 , C07F7/08 , B01J31/14 , B01J21/16
CPC分类号： C07F17/00 , C08F4/65912 , C08F10/00 , C08F10/06 , C08F110/06 , C08F210/06 , C08F4/65927 , C08F4/65916 , C08F2/001 , C08F2500/01 , C08F210/16 , C08F210/08
摘要： A metallocene complex by which high uptake efficiency of ethylene and/or α-olefin can be obtained compared with the conventional metallocene catalyst, and rubber component having high molecular weight can be polymerized, and polymerization method of olefin.Metallocene complex (metallocene complex having furyl or thienyl group in which substituent exists at 5-position of indenyl ring, and substituent may exist at 2-position of indenyl ring, and the like) represented by the general formula [I], the catalyst for olefin polymerization characterized by comprising said metallocene complex, and polymerization method of olefin characterized in that polymerization or copolymerization of olefin is carried out using said polymerization catalyst for olefin, and the like.
摘要翻译：与常规茂金属催化剂相比，可以获得乙烯和/或α-烯烃的高吸收效率的茂金属络合物，可以聚合具有高分子量的橡胶组分，以及烯烃的聚合方法。茂金属络合物（具有呋喃基或噻吩基的茂金属络合物，其中在茚基环的5-位存在取代基，并且取代基可以存在于通式[I]表示的茚基环的2-位，等等），催化剂其特征在于包含所述茂金属络合物和烯烃聚合方法，其特征在于使用所述烯烃聚合催化剂等进行烯烃的聚合或共聚。

33. 发明申请

US20110009303A1 AUTOMATIC DISHWASHING COMPOSITION CONTAINING A SULFONATED COPOLYMER 有权
标题翻译：自动洗涤组合物含有磺化共聚物
公开(公告)号：US20110009303A1
公开(公告)日：2011-01-13
申请号：US12863844
申请日：2009-03-27
申请人： Takahiro Tsumori , Masato Nakano
发明人： Takahiro Tsumori , Masato Nakano
IPC分类号： C11D3/37 , C11D17/00 , C11D17/06
CPC分类号： C11D3/2086 , C08J3/14 , C08L33/00 , C08L33/14 , C08L35/00 , C08L41/00 , C11D3/33 , C11D3/34 , C11D3/3757 , C11D3/378 , C11D3/3902 , C11D3/3942 , C11D3/3947 , C11D7/265 , C11D7/34 , C08L2666/04
摘要： An ADW composition comprising a builder and a water-soluble copolymer which comprises: (a) from about 30 to 60 mol % of the copolymer having a structural unit originating from a monoethylenic unsaturated dicarboxylic acid (or dicarboxylate) monomer having 4 to 6 carbon atoms or its anhydride at; (b) from about 30 to 60 mol % of the copolymer having a structural unit originating from a monoethylenic unsaturated monocarboxylic acid (or monocarboxylate) monomer having 3 to 8 carbon atoms; and (c) from about 5 to 15 mol % of the polymer having a structural unit originating from a monoethylenic unsaturated monomer having a sulfonic (or sulfonate) group; wherein the water-soluble copolymer has a weight average molecular weight of from about 1,000 to about 50,000 wherein the copolymer is polymerized with hydrogen peroxide.
摘要翻译：一种包含助洗剂和水溶性共聚物的ADW组合物，其包含：（a）约30至60摩尔％的具有来自具有4-6个碳原子的单烯属不饱和二羧酸（或二羧酸酯）单体的结构单元的共聚物或其酸酐在（b）具有来自具有3-8个碳原子的单烯属不饱和一元羧酸（或单羧酸酯）单体的结构单元的共聚物的约30至60mol％; 和（c）约5至15摩尔％的具有源自具有磺酸（或磺酸盐）基团的单烯属不饱和单体的结构单元的聚合物; 其中所述水溶性共聚物的重均分子量为约1,000至约50,000，其中所述共聚物与过氧化氢聚合。

34. 发明申请

US20100298526A1 COPOLYMER COMPOSITION AND METHOD OF PRODUCING THE COMPOSITION 审中-公开
标题翻译：共聚物组合物及其制备方法
公开(公告)号：US20100298526A1
公开(公告)日：2010-11-25
申请号：US12740954
申请日：2008-10-31
申请人： Takahiro Tsumori , Masato Nakano
发明人： Takahiro Tsumori , Masato Nakano
IPC分类号： C08G75/00
CPC分类号： C11D3/378 , C08F2/10 , C08F2/38 , C08F220/04 , C08F220/38 , C08F222/02
摘要： Provided are a copolymer composition which can achieve a high level of compatibility between clay dispersibility under water having high hardness and an anti-iron deposition ability and is suitable for an additive for a detergent, and a method of producing the composition. The copolymer composition of the present invention includes a copolymer (P) which has a weight average molecular weight of 10,000 to 50,000 and contains a structural unit originating from a monoethylenic unsaturated dicarboxylic acid (or dicarboxylate) monomer (a) at 30 to 60 mol %, a structural unit originating from a monoethylenic unsaturated monocarboxylic acid (or monocarboxylate) monomer (b), and a structural unit originating from a sulfonic acid (or sulfonate) group-containing monomer (c) free of an ester bond and an amide bond, and a remaining monoethylenic unsaturated dicarboxylic acid (or dicarboxylate) monomer a content of which in terms of an acid is less than 12,000 ppm.
摘要翻译：提供一种共聚物组合物，其可以实现在具有高硬度和抗铁沉积能力的水下的粘土分散性之间的高水平的相容性，并且适用于洗涤剂用添加剂和制备该组合物的方法。本发明的共聚物组合物包含重均分子量为10,000〜50,000的共聚物（P），含有以30〜60摩尔％的单烯属不饱和二羧酸（或二羧酸酯）单体（a）的结构单元，，来自单烯属不饱和一元羧酸（或单羧酸酯）单体（b）的结构单元和源自不含酯键和酰胺键的含磺酸（或磺酸酯）基团的单体（c）的结构单元，和剩余的单烯属不饱和二羧酸（或二羧酸酯）单体的含量以酸计小于12,000ppm。

35. 发明申请

US20100292122A1 SULFONIC GROUP-CONTAINING, MALEIC ACID-BASED, WATER-SOLUBLE COPOLYMER AQUEOUS SOLUTION AND POWDER OBTAINED BY DRYING THE AQUEOUS SOLUTION 有权
标题翻译：含硫酸基，基于酸性的水溶性共聚物水溶液和粉末通过干燥水溶液获得
公开(公告)号：US20100292122A1
公开(公告)日：2010-11-18
申请号：US12863865
申请日：2009-03-27
申请人： Takahiro Tsumori , Masato Nakano
发明人： Takahiro Tsumori , Masato Nakano
IPC分类号： C08K3/20 , C02F5/10 , C11D3/39
CPC分类号： C11D3/2086 , C08J3/14 , C08L33/00 , C08L33/14 , C08L35/00 , C08L41/00 , C11D3/33 , C11D3/34 , C11D3/3757 , C11D3/378 , C11D3/3902 , C11D3/3942 , C11D3/3947 , C11D7/265 , C11D7/34 , C08L2666/04
摘要： Provided is a copolymer aqueous solution which exerts a high calcium carbonate-deposition suppressing ability even under high hardness condition, has excellent storage stability, and suppresses coloring of a detergent to yellow even when used as a detergent raw material. The water-soluble copolymer aqueous solution includes a water-soluble copolymer and hydrogen peroxide as essential components, in which: the water-soluble copolymer at least includes, as its structure, a structural unit originating from a monoethylenic unsaturated dicarboxylic acid (or dicarboxylate) monomer having 4 to 6 carbon atoms or its anhydride (a) at 30 to 60 mol %, a structural unit originating from a monoethylenic unsaturated monocarboxylic acid (or monocarboxylate) monomer having 3 to 8 carbon atoms (b), and a structural unit originating from a monoethylenic unsaturated monomer having a sulfonic (or sulfonate) group (c); the water-soluble copolymer has a weight average molecular weight of 1,000 or more and 50,000 or less; the water-soluble copolymer aqueous solution has a weight ratio of the hydrogen peroxide of 10 ppm to 50,000 ppm with respect to a solid content of the water-soluble copolymer aqueous solution; and the water-soluble copolymer aqueous solution has a weight ratio of water of 33% to 99%.
摘要翻译：提供即使在高硬度条件下也具有高碳酸钙沉积抑制能力的共聚物水溶液，具有优异的储存稳定性，并且即使用作洗涤剂原料也能抑制洗涤剂的着色。水溶性共聚物水溶液包含水溶性共聚物和过氧化氢作为必要成分，其中：水溶性共聚物至少包含来自单烯属不饱和二羧酸（或二羧酸酯）的结构单元作为其结构，具有4-6个碳原子的单体或其酸酐（a）的含量为30至60摩尔％，源自具有3-8个碳原子的单烯属不饱和一元羧酸（或单羧酸酯）单体（b）的结构单元，以及起始于来自具有磺酸（或磺酸）基团（c）的单烯属不饱和单体; 该水溶性共聚物的重均分子量为1000以上且50,000以下，相对于水溶性共聚物水溶液的固体成分，水溶性共聚物水溶液的过氧化氢重量比为10ppm〜50,000ppm; 水溶性共聚物水溶液的重量比为33〜99％。

36. 发明授权

US07427623B2 4-Amino-2,3-disubstituted thieno[2,3-d]pyrimidines and pharmacetical compositions thereof 失效
标题翻译： 4-氨基-2,3-二取代噻吩并[2,3-d]嘧啶及其药物组合物
公开(公告)号：US07427623B2
公开(公告)日：2008-09-23
申请号：US10489052
申请日：2002-09-10
申请人： Jerry Leroy Adams , Deborah Lynne Bryan , Yanhong Feng , Shinichiro Matsunaga , Yutaka Maeda , Yasushi Miyazaki , Masato Nakano , Jean-Philippe Rocher , Hideyuki Sato , Marcus Semones , Domingos J. Silva , Jun Tang
发明人： Jerry Leroy Adams , Deborah Lynne Bryan , Yanhong Feng , Shinichiro Matsunaga , Yutaka Maeda , Yasushi Miyazaki , Masato Nakano , Jean-Philippe Rocher , Hideyuki Sato , Marcus Semones , Domingos J. Silva , Jun Tang
IPC分类号： A61K31/519 , C07D495/04 , A61P35/00 , A61P9/00
CPC分类号： C07D491/04 , C07D495/04
摘要： Furo- and thienopyrimidine derivatives, which are useful as TIE-2 and/or VEGFR-2 inhibitors are described herein. The described invention also includes methods of making such furo- and thienopyrimidine derivatives as well as methods of using the same in the treatment of hyperproliferative diseases.
摘要翻译：本文描述了可用作TIE-2和/或VEGFR-2抑制剂的呋喃和噻吩并嘧啶衍生物。所述的发明还包括制备这些呋喃并噻吩并嘧啶衍生物的方法以及使用它们在治疗过度增殖性疾病中的方法。

37. 发明授权

US07019157B2 Metallocene compounds, production process for olefin polymers using catalysts containing them and olefin polymers produced by the production process 有权
标题翻译：茂金属化合物，使用含有催化剂的烯烃聚合物的生产方法和通过生产方法生产的烯烃聚合物
公开(公告)号：US07019157B2
公开(公告)日：2006-03-28
申请号：US10210394
申请日：2002-08-02
申请人： Toshihiro Uwai , Masato Nakano , Tsutomu Ushioda , Masami Kimura , Tsuyoshi Yahata
发明人： Toshihiro Uwai , Masato Nakano , Tsutomu Ushioda , Masami Kimura , Tsuyoshi Yahata
IPC分类号： C07F17/00 , C08F4/76 , C08F4/52
CPC分类号： C08F297/08 , C07F17/00 , C08F4/65912 , C08F4/65916 , C08F10/06 , C08F210/06 , Y10S526/943 , C08F4/65927 , C08F210/16 , C08F2500/12 , C08F2500/03
摘要： The present invention provides metallocene compounds which exhibit high polymerization activity for production of highly stereoregular polymers, as well as a production process for olefin polymers which employs olefin polymerization catalysts containing the compounds, and olefin polymers obtained by the production process. A metallocene compound of the present invention is represented by the following general formula (1): YKLMX2 (1) wherein M represents a titanium atom, zirconium atom or hafnium atom; K and L are fused rings coordinated to M and each independently represents a fused ring of a cyclopentadienyl ring and a 5-membered ring, a fused ring of a cyclopentadienyl ring and a 6-membered ring or a fused ring of a cyclopentadienyl ring and a 7-membered ring; Y is a bridge group crosslinking K and L; and each X is bonded to M; and K and L have a 2-furyl group, substituted 2-furyl group, 2-thienyl group, substituted 2-thienyl group, 2-furfuryl group or substituted 2-furfuryl group on at least one position among each of the 2-positions, 4-positions and 5-positions.
摘要翻译：本发明提供了表现出高聚合活性的茂金属化合物，用于生产高立体规则聚合物，以及使用含有该化合物的烯烃聚合催化剂的烯烃聚合物的制备方法，以及通过该方法得到的烯烃聚合物。本发明的茂金属化合物由以下通式（1）表示：<？in-line-formula description =“In-line formula”end =“lead”？> YKLMX＆lt; 2＆gt;（ 1）<？in-line-formula description =“In-line Formulas”end =“tail”？>其中M表示钛原子，锆原子或铪原子; K和L是与M配位的稠合环，并且各自独立地表示环戊二烯基环和5元环的稠环，环戊二烯基环的稠环和6元环或环戊二烯基环的稠环和 7元环; Y是交联K和L的桥组; 并且每个X与M键合; K和L在2-位中的至少一个位置具有2-呋喃基，取代的2-呋喃基，2-噻吩基，取代的2-噻吩基，2-糠基或取代的2-糠基 4个职位和5个职位。

38. 发明授权

US06635733B2 Elastomeric polypropylene 失效
标题翻译：弹性聚丙烯
公开(公告)号：US06635733B2
公开(公告)日：2003-10-21
申请号：US09850152
申请日：2001-05-08
申请人： Tsuyoshi Yahata , Masato Nakano , Yoshiyuki Ohgi , Tsutomu Ushioda
发明人： Tsuyoshi Yahata , Masato Nakano , Yoshiyuki Ohgi , Tsutomu Ushioda
IPC分类号： C08F21006
CPC分类号： C08F110/06 , C08F4/65912 , C08F10/00 , Y10S526/943 , C08F4/65925 , C08F2500/15 , C08F2500/12 , C08F2500/03 , C08F2500/21
摘要： An elastomeric polypropylene wherein (a) an isotactic pentad (I5) is 0.150-0.749, (b) a different bond due to a 2,1-insertion reaction is 0.11-20 mol %, (c) a different bond due to a 1,3-insertion reaction is 0-10 mol % and (d) a melting point (Tm) is 50-160° C., (a) to (c) being determined from 13C NMR spectra, which is obtainable by the polymerization of propylene using any one of a metallocene catalyst (I) comprising a metallocene compound (A), an activating compound (B) and if desired, an organoaluminum compound (C), a supported metallocene catalyst (II) prepared by supporting the metallocene catalyst (I) on a finely particulate support (D), and a supported metallocene catalyst (III) prepared by adding an organoaluminum compound (E) to the supported metallocene catalyst (II). In particular, it has excellent transparency and elastic characteristics.
摘要翻译：一种弹性体聚丙烯，其中（a）全同立构五单元组（I5）为0.150-0.749，（b）由于2,1-插入反应引起的不同键为0.11-20摩尔％，（c）由于1 ，3-插入反应为0-10摩尔％，（d）熔点（Tm）为50-160℃，（a）至（c）由13 C NMR谱确定，可通过使用包含茂金属化合物（A）的茂金属催化剂（I），活化化合物（B）和如果需要的话，使用有机铝化合物（C），负载金属茂催化剂（II）在精细颗粒载体（D）上的金属茂催化剂（I）和通过将有机铝化合物（E）加入到负载的茂金属催化剂（II）中制备的负载金属茂催化剂（III）。特别是具有优异的透明性和弹性特性。

39. 发明授权

US06479646B1 Metallocene compounds having indenyl ligand and catalysts for olefin polymerization containing the same 失效
标题翻译：具有茚基配体的茂金属化合物和含有它们的烯烃聚合催化剂
公开(公告)号：US06479646B1
公开(公告)日：2002-11-12
申请号：US09686619
申请日：2000-10-12
申请人： Masato Nakano , Tsutomu Ushioda , Seiki Mitani , Hiroshi Yamazaki
发明人： Masato Nakano , Tsutomu Ushioda , Seiki Mitani , Hiroshi Yamazaki
IPC分类号： B05J3100
CPC分类号： C07F17/00 , C08F4/65908 , C08F4/65912 , C08F10/06 , C08F110/06 , C08F4/65925 , C08F2500/17 , C08F2500/03
摘要： A metallocene compound having an indenyl ligand substituted by a heteroaromatic group, which is useful as an olefin polymerization catalyst. The metallocene compound has the following structure wherein M is a transition metal atom; each Ra is a monocyclic or polycyclic heteroaromatic group; each R1 is halogen, a hydrocarbon group of 1-20 carbons, a halogenated hydrocarbon group of 1-20 carbons, etc., or adjacent R1's may be joined together to form a ring of 6-8 carbons; p and q are each 1-7; n and l are each 0 or 1-6; and each X is halogen, a hydrocarbon group of 1-20 carbons, a halogenated hydrocarbon group of 1-20 carbons, etc.
摘要翻译：具有被杂芳基取代的茚基配位体的茂金属化合物，其可用作烯烃聚合催化剂。金属茂化合物具有以下结构，其中M是过渡金属原子;每个R a是单环或多环杂芳族基团;每个R 1是卤素，1-20个碳的烃基，1-20个碳的卤代烃基等，或相邻的R1可以连接在一起形成6-8个碳环; p和q各自为1-7; n和l各自为0或1-6;并且各X为卤素，1-20个碳的烃基，1-20个碳的卤代烃基等

40. 发明授权

US06169051A Metallocene compounds, processes for the preparation thereof, catalyst components for olefin polymerization, and processes for the production of olefin polymers 有权
公开(公告)号：US06169051A
公开(公告)日：2001-01-02
申请号：US09236322
申请日：1999-01-25
申请人： Seiki Mitani , Masato Nakano , Jun Saito , Hiroshi Yamazaki , Keisuke Kimura
发明人： Seiki Mitani , Masato Nakano , Jun Saito , Hiroshi Yamazaki , Keisuke Kimura
IPC分类号： B01J3100
CPC分类号： C08F10/00 , C07F17/00 , C08F4/65904 , C08F4/65912 , C08F4/65916 , C08F110/06 , Y10S526/943 , C08F4/6592 , C08F4/65927 , C08F2500/03 , C08F2500/15
摘要： A metallocene compound is provided wherein to a transition metal compound is bonded a multidentate compound wherein a substituted cycloalkadienyl ring CA1 having therein a heteroaromatic group Ra containing an oxygen, sulfur or nitrogen atom on a cycloalkadienyl ring, preferably the five-membered ring thereof, and an unsubstituted or substituted cycloalkadienyl group CA2 or —(R1)N—, —O—, —S— or —(R1)P—, preferably CA2, more preferably a substituted cycloalkadienyl group identical with CA1 are bonded through a divalent linking group. The metallocene compound is suitable as a principal ingredient of a catalyst for the polymerization of olefins, particularly achieving a very high effect in making the molecular weight of a polypropylene higher.

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