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1. 发明申请

US20120178833A1 PROCESS FOR THE PRODUCTION OF METHANE 有权
标题翻译：生产甲烷的方法
公开(公告)号：US20120178833A1
公开(公告)日：2012-07-12
申请号：US13388307
申请日：2010-08-02
申请人： Lloyd Anthony Clomburg, JR. , Anand Nilekar
发明人： Lloyd Anthony Clomburg, JR. , Anand Nilekar
IPC分类号： C07C27/00
CPC分类号： C07C1/0435 , C07C1/041 , C07C1/0485 , C07C2523/755 , C07C9/04
摘要： A process for the production of methane comprising reacting at least part of a feed gas containing carbon monoxide and hydrogen in an internally cooled methanation reactor containing a nickel comprising methanation catalyst to produce a product gas containing methane, cooling the internally cooled methanation reactor with water, wherein the water enters the internally cooled methanation reactor at a temperature in the range from 20-120° C. below its boiling temperature.
摘要翻译：一种生产甲烷的方法，包括在含有甲烷化催化剂的镍的内部冷却的甲烷化反应器中使至少一部分含有一氧化碳和氢气的进料气体反应，以产生含有甲烷的产物气体，用水冷却内部冷却的甲烷化反应器，其中水在低于沸点温度的20-120℃的温度范围内进入内部冷却的甲烷化反应器。

2. 发明授权

US08927610B2 Process for the production of methane 有权
标题翻译：甲烷生产工艺
公开(公告)号：US08927610B2
公开(公告)日：2015-01-06
申请号：US13388307
申请日：2010-08-02
申请人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
发明人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
IPC分类号： C07C27/00 , C07C1/04
CPC分类号： C07C1/0435 , C07C1/041 , C07C1/0485 , C07C2523/755 , C07C9/04
摘要： A process for the production of methane comprising reacting at least part of a feed gas containing carbon monoxide and hydrogen in an internally cooled methanation reactor containing a nickel comprising methanation catalyst to produce a product gas containing methane, cooling the internally cooled methanation reactor with water, wherein the water enters the internally cooled methanation reactor at a temperature in the range from 20-120° C. below its boiling temperature.
摘要翻译：一种生产甲烷的方法，包括在含有甲烷化催化剂的镍的内部冷却的甲烷化反应器中使至少部分含有一氧化碳和氢气的进料气体反应，以产生含有甲烷的产物气体，用水冷却内部冷却的甲烷化反应器，其中水在低于沸点温度的20-120℃的温度范围内进入内部冷却的甲烷化反应器。

3. 发明授权

US08470059B2 Process for producing a methane-rich gas 有权
标题翻译：富含甲烷气体的方法
公开(公告)号：US08470059B2
公开(公告)日：2013-06-25
申请号：US12649171
申请日：2009-12-29
申请人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
发明人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
IPC分类号： C01B3/24
CPC分类号： C10L3/08 , C07C1/06 , C07C9/04
摘要： A process for producing a methane-rich gas comprising the steps of: a) mixing a feed gas, comprising carbon monoxide and hydrogen, and a recycled methane-rich gas, comprising methane, to produce a gas mixture, comprising carbon monoxide, hydrogen and methane; b) reacting at least part of the carbon monoxide and hydrogen in the gas mixture in the presence of a methanation catalyst to produce a methane-rich product gas comprising methane, carbon dioxide and water; c) treating at least part of the methane-rich product gas to remove carbon dioxide to produce a methane-rich carbon dioxide-lean gas; and d) recycling at least part of the methane-rich carbon dioxide-lean gas to mixing step a) as recycled methane-rich gas.
摘要翻译：一种用于生产富甲烷气体的方法，包括以下步骤：a）将包含一氧化碳和氢气的进料气体和包含甲烷的再循环富甲烷气体混合以产生包含一氧化碳，氢气和甲烷 b）在甲烷化催化剂存在下使气体混合物中的至少一部分一氧化碳和氢气反应，以产生包含甲烷，二氧化碳和水的富含甲烷的产物气体; c）处理至少部分富甲烷产物气体以除去二氧化碳以产生富含甲烷的贫二氧化碳气体; 和d）将至少部分富含甲烷的贫二氧化碳气体再循环至混合步骤a）作为再循环的富甲烷气体。

4. 发明授权

US08461216B2 Process for the co-production of superheated steam and methane 有权
标题翻译：共同生产过热蒸汽和甲烷的方法
公开(公告)号：US08461216B2
公开(公告)日：2013-06-11
申请号：US13388311
申请日：2010-08-02
申请人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
发明人： Lloyd Anthony Clomburg, Jr. , Anand Nilekar
IPC分类号： C07C27/00
CPC分类号： C07C1/0435 , C07C1/041 , C07C1/0485 , C07C2523/755 , C07C9/04
摘要： A process for the co-production of superheated steam and methane includes reacting a gas containing carbon monoxide and hydrogen in a series of methanation regions to produce a product gas containing methane The gas containing carbon monoxide and hydrogen flows, in passing through the series of methanation regions, successively through at least a first internally cooled methanation region and a second internally cooled methanation region, cooling the first and second internally cooled methanation region with water, which water is vaporized in the first internally cooled methanation region to produce steam and which steam is subsequently superheated in the second internally cooled methanation region to produce superheated steam The internally cooled methanation regions include tubes filled with a methanation catalyst and a space surrounding the tubes The gas containing carbon monoxide and hydrogen and/or product gas flows through the tubes and the water flows through the space surrounding the tubes.
摘要翻译：共同生产过热蒸汽和甲烷的方法包括在一系列甲烷化区域中使含有一氧化碳和氢气的气体反应以产生含有甲烷的产物气体含有一氧化碳和氢气的气体在经过一系列甲烷化作用区域，依次通过至少第一内部冷却的甲烷化区域和第二内部冷却的甲烷化区域，用水冷却第一和第二内部冷却的甲烷化区域，该水在第一内部冷却的甲烷化区域中蒸发以产生蒸汽，随后在第二内部冷却的甲烷化区域中过热以产生过热蒸汽。内部冷却的甲烷化区域包括填充有甲烷化催化剂的管和围绕管的空间。含有一氧化碳和氢气和/或产物气体的气体流过管和水流过空间环绕管子。

5. 发明申请

US20120148481A1 PROCESS FOR THE CO-PRODUCTION OF SUPERHEATED STEAM AND METHANE 有权
标题翻译：过热蒸汽和甲烷的共同生产工艺
公开(公告)号：US20120148481A1
公开(公告)日：2012-06-14
申请号：US13388311
申请日：2010-08-02
申请人： Lloyd Anthony Clomburg, JR. , Anand Nilekar
发明人： Lloyd Anthony Clomburg, JR. , Anand Nilekar
IPC分类号： C01B5/00
CPC分类号： C07C1/0435 , C07C1/041 , C07C1/0485 , C07C2523/755 , C07C9/04
摘要： A process for the co-production of superheated steam and methane includes reacting a gas containing carbon monoxide and hydrogen in a series of methanation regions to produce a product gas containing methane. The gas containing carbon monoxide and hydrogen flows, in passing through the series of methanation regions, successively through at least a first internally cooled methanation region and a second internally cooled methanation region, cooling the first and second internally cooled methanation region with water, which water is vaporized in the first internally cooled methanation region to produce steam and which steam is subsequently superheated in the second internally cooled methanation region to produce superheated steam. The internally cooled methanation regions include tubes filled with a methanation catalyst and a space surrounding the tubes. The gas containing carbon monoxide and hydrogen and/or product gas flows through the tubes and the water flows through the space surrounding the tubes.
摘要翻译：用于共生产过热蒸汽和甲烷的方法包括在一系列甲烷化区域中使含有一氧化碳和氢气的气体反应以产生含有甲烷的产物气体。含有一氧化碳和氢气的气体在通过一系列甲烷化区域时依次通过至少第一内部冷却的甲烷化区域和第二内部冷却的甲烷化区域，用水冷却第一和第二内部冷却的甲烷化区域，该水在第一内部冷却的甲烷化区域中蒸发以产生蒸汽，并且随后将蒸汽在第二内部冷却的甲烷化区域中过热以产生过热蒸汽。内部冷却的甲烷化区域包括填充有甲烷化催化剂的管和围绕管的空间。含有一氧化碳和氢气和/或产物气体的气体流过管，水流过管周围的空间。

6. 发明授权

US07846413B2 Systems and processes for producing hydrogen and carbon dioxide 有权
标题翻译：用于生产氢气和二氧化碳的系统和方法
公开(公告)号：US07846413B2
公开(公告)日：2010-12-07
申请号：US11946747
申请日：2007-11-28
申请人： Lloyd Anthony Clomburg, Jr. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
发明人： Lloyd Anthony Clomburg, Jr. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
IPC分类号： C01B31/20 , C01B3/24 , C01B3/26 , C01B3/16
CPC分类号： C01B3/384 , B01J8/0285 , B01J2208/00274 , B01J2208/00504 , B01J2219/00006 , C01B3/382 , C01B3/48 , C01B3/501 , C01B3/56 , C01B2203/0233 , C01B2203/0288 , C01B2203/0294 , C01B2203/0405 , C01B2203/041 , C01B2203/043 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0495 , C01B2203/0811 , C01B2203/0883 , C01B2203/1041 , C01B2203/1047 , C01B2203/1058 , C01B2203/1076 , C01B2203/1241 , C01B2203/1294 , C01B2203/142 , C01B2203/146 , C01B2203/148 , C01B2203/1623 , C01B2203/82
摘要： A process and a system are provided for producing and separating hydrogen and carbon dioxide from a hydrocarbon and steam. A hydrocarbon and steam are steam reformed and the reformed gas is shift reacted to produce a shift gas. Hydrogen is removed from the shift gas, and the hydrogen-depleted gas is reformed and shift reacted again to produce more hydrogen and carbon dioxide. The hydrogen and carbon dioxide are then separated.
摘要翻译：提供了用于从烃和蒸汽中生产和分离氢气和二氧化碳的方法和系统。将烃和蒸汽进行蒸汽重整，重整气体发生反应以产生换档气体。从移动气体中除去氢气，并且将贫氢气体重整并再次反应以产生更多的氢气和二氧化碳。然后分离氢气和二氧化碳。

7. 发明授权

US08088185B2 System for producing hydrogen and carbon dioxide 失效
标题翻译：生产氢气和二氧化碳的系统
公开(公告)号：US08088185B2
公开(公告)日：2012-01-03
申请号：US12939014
申请日：2010-11-03
申请人： Lloyd Anthony Clomburg, Jr. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
发明人： Lloyd Anthony Clomburg, Jr. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
IPC分类号： B01J8/00
CPC分类号： C01B3/384 , B01J8/0285 , B01J2208/00274 , B01J2208/00504 , B01J2219/00006 , C01B3/382 , C01B3/48 , C01B3/501 , C01B3/56 , C01B2203/0233 , C01B2203/0288 , C01B2203/0294 , C01B2203/0405 , C01B2203/041 , C01B2203/043 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0495 , C01B2203/0811 , C01B2203/0883 , C01B2203/1041 , C01B2203/1047 , C01B2203/1058 , C01B2203/1076 , C01B2203/1241 , C01B2203/1294 , C01B2203/142 , C01B2203/146 , C01B2203/148 , C01B2203/1623 , C01B2203/82
摘要： A system is provided for producing and separating hydrogen and carbon dioxide from a hydrocarbon and steam. A hydrocarbon and steam are steam reformed and the reformed gas is shift reacted to produce a shift gas in the system. Hydrogen is removed from the shift gas, and the hydrogen-depleted gas is reformed and shift reacted again to produce more hydrogen and carbon dioxide in the system. The hydrogen and carbon dioxide are then separated.
摘要翻译：提供一种用于从烃和蒸汽中生产和分离氢气和二氧化碳的系统。蒸汽重整碳氢化合物和蒸汽，并且重整气体被移动反应以在系统中产生换档气体。从移动气体中除去氢气，并且将贫氢气体重整并再次反应以在系统中产生更多的氢和二氧化碳。然后分离氢气和二氧化碳。

8. 发明申请

US20110044861A1 SYSTEM FOR PRODUCING HYDROGEN AND CARBON DIOXIDE 失效
标题翻译：生产二氧化碳和二氧化碳的系统
公开(公告)号：US20110044861A1
公开(公告)日：2011-02-24
申请号：US12939014
申请日：2010-11-03
申请人： Lloyd Anthony CLOMBURG, JR. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
发明人： Lloyd Anthony CLOMBURG, JR. , Andreas Nicholas Matzakos , Peter Veenstra , Scott Lee Wellington
IPC分类号： B01J8/00
CPC分类号： C01B3/384 , B01J8/0285 , B01J2208/00274 , B01J2208/00504 , B01J2219/00006 , C01B3/382 , C01B3/48 , C01B3/501 , C01B3/56 , C01B2203/0233 , C01B2203/0288 , C01B2203/0294 , C01B2203/0405 , C01B2203/041 , C01B2203/043 , C01B2203/047 , C01B2203/0475 , C01B2203/048 , C01B2203/0495 , C01B2203/0811 , C01B2203/0883 , C01B2203/1041 , C01B2203/1047 , C01B2203/1058 , C01B2203/1076 , C01B2203/1241 , C01B2203/1294 , C01B2203/142 , C01B2203/146 , C01B2203/148 , C01B2203/1623 , C01B2203/82
摘要： A system is provided for producing and separating hydrogen and carbon dioxide from a hydrocarbon and steam. A hydrocarbon and steam are steam reformed and the reformed gas is shift reacted to produce a shift gas in the system. Hydrogen is removed from the shift gas, and the hydrogen-depleted gas is reformed and shift reacted again to produce more hydrogen and carbon dioxide in the system. The hydrogen and carbon dioxide are then separated.
摘要翻译：提供一种用于从烃和蒸汽中生产和分离氢气和二氧化碳的系统。蒸汽重整碳氢化合物和蒸汽，并且重整气体被移动反应以在系统中产生换档气体。从移动气体中除去氢气，并且将贫氢气体重整并再次反应以在系统中产生更多的氢和二氧化碳。然后分离氢气和二氧化碳。

9. 发明申请

US20100162627A1 PROCESS FOR PRODUCING A METHANE-RICH GAS 有权
标题翻译：生产甲烷气的方法
公开(公告)号：US20100162627A1
公开(公告)日：2010-07-01
申请号：US12649171
申请日：2009-12-29
申请人： Lloyd Anthony CLOMBURG, JR. , Anand Nilekar
发明人： Lloyd Anthony CLOMBURG, JR. , Anand Nilekar
IPC分类号： C10L3/10
CPC分类号： C10L3/08 , C07C1/06 , C07C9/04
摘要： A process for producing a methane-rich gas comprising the steps of: a) mixing a feed gas, comprising carbon monoxide and hydrogen, and a recycled methane-rich gas, comprising methane, to produce a gas mixture, comprising carbon monoxide, hydrogen and methane; b) reacting at least part of the carbon monoxide and hydrogen in the gas mixture in the presence of a methanation catalyst to produce a methane-rich product gas comprising methane, carbon dioxide and water; c) treating at least part of the methane-rich product gas to remove carbon dioxide to produce a methane-rich carbon dioxide-lean gas; and d) recycling at least part of the methane-rich carbon dioxide-lean gas to mixing step a) as recycled methane-rich gas.
摘要翻译：一种用于生产富甲烷气体的方法，包括以下步骤：a）将包含一氧化碳和氢气的进料气体和包含甲烷的再循环富甲烷气体混合以产生包含一氧化碳，氢气和甲烷 b）在甲烷化催化剂存在下使气体混合物中的至少一部分一氧化碳和氢气反应，以产生包含甲烷，二氧化碳和水的富含甲烷的产物气体; c）处理至少部分富甲烷产物气体以除去二氧化碳以产生富含甲烷的贫二氧化碳气体; 和d）将至少部分富含甲烷的贫二氧化碳气体再循环至混合步骤a）作为再循环的富甲烷气体。

10. 发明申请

US20100162626A1 ADIABATIC REACTOR AND A PROCESS AND A SYSTEM FOR PRODUCING A METHANE-RICH GAS IN SUCH ADIABATIC REACTOR 审中-公开
标题翻译：自动反应器和一种在这样的自动反应器中生产甲烷气体的方法和系统
公开(公告)号：US20100162626A1
公开(公告)日：2010-07-01
申请号：US12649150
申请日：2009-12-29
申请人： Lloyd Anthony CLOMBURG, JR. , Anand NILEKAR
发明人： Lloyd Anthony CLOMBURG, JR. , Anand NILEKAR
IPC分类号： C10L3/10 , B01J19/00
CPC分类号： B01J8/0285 , B01J8/062 , B01J8/067 , B01J12/007 , B01J19/249 , B01J2208/00212 , B01J2208/00309 , B01J2219/2453 , B01J2219/2458 , B01J2219/2465 , B01J2219/2481 , C10J2300/0916 , C10J2300/092 , C10J2300/093 , C10J2300/1662 , C10K1/101 , C10K3/04 , C10L3/08
摘要： An adiabatic reactor comprising a first inlet and a first outlet defining a first flowpath between the first inlet and the first outlet and a second inlet and a second outlet defining a second flowpath between the second inlet and the second outlet, wherein the first flowpath and the second flowpath are directed in opposite directions; wherein both the first flowpath and the second flowpath comprise a catalyst; and wherein at least part of the first flowpath and at least part of the second flowpath are thermally connected via a wall separating the first flowpath from the second flowpath.In addition a methanation process and system using the adiabatic reactor is provided.
摘要翻译：一种绝热反应器，包括限定第一入口和第一出口之间的第一流路的第一入口和第一出口以及限定第二入口和第二出口之间的第二流路的第二入口和第二出口，其中第一流路和第二流路沿相反方向导向; 其中所述第一流路和所述第二流路都包括催化剂; 并且其中所述第一流动路径的至少一部分和所述第二流动路径的至少一部分经由将所述第一流动路径与所述第二流动路径分开的壁热连接。此外，还提供了使用绝热反应器的甲烷化方法和系统。

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